From 5aa09cfee8266903bb77986ebea5b8671a383ea5 Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Mon, 5 Jun 2023 16:52:50 -0700 Subject: [PATCH 01/73] Confirmed CASCI with Open-Shell (O2 Triplet), added guards around untested code paths --- tests/standalone_driver.cxx | 15 +++++++++++++-- 1 file changed, 13 insertions(+), 2 deletions(-) diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index f2b537bb..6d2aaa18 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -85,7 +85,7 @@ int main(int argc, char** argv) { auto nalpha = input.getData("CI.NALPHA"); auto nbeta = input.getData("CI.NBETA"); - if(nalpha != nbeta) throw std::runtime_error("NALPHA != NBETA"); + //if(nalpha != nbeta) throw std::runtime_error("NALPHA != NBETA"); // Read FCIDUMP File size_t norb = macis::read_fcidump_norb(fcidump_fname); @@ -230,6 +230,9 @@ int main(int argc, char** argv) { // MP2 Guess Orbitals if(mp2_guess) { + if( nalpha != nbeta ) + throw std::runtime_error("MP2 Guess only implemented for closed-shell"); + console->info("Calculating MP2 Natural Orbitals"); size_t nocc_canon = n_inactive + nalpha; size_t nvir_canon = norb - nocc_canon; @@ -291,7 +294,7 @@ int main(int argc, char** argv) { auto det_logger = world_rank ? spdlog::null_logger_mt("determinants") : spdlog::stdout_color_mt("determinants"); - det_logger->info("Print leading determinants > {:.12f}", + det_logger->info("Print leading determinants > {:.2e}", determinants_threshold); auto dets = macis::generate_hilbert_space( n_active, nalpha, nbeta); @@ -304,6 +307,10 @@ int main(int argc, char** argv) { } } else { + + if(nalpha != nbeta) + throw std::runtime_error("ASCI Only Implemented for Closed-Shell"); + // Generate the Hamiltonian Generator generator_t ham_gen( macis::matrix_span(T_active.data(), n_active, n_active), @@ -376,6 +383,10 @@ int main(int argc, char** argv) { // MCSCF } else if(job == Job::MCSCF) { + + if( nalpha != nbeta ) + throw std::runtime_error("MCSCF Only Implemented for Closed-Shells"); + // Possibly read active RDMs if(rdm_fname.size()) { console->info(" * RDMFILE = {}", rdm_fname); From bd1091ac6817749a85211fe3a492977427e7a534 Mon Sep 17 00:00:00 2001 From: Clang Robot Date: Mon, 5 Jun 2023 23:54:33 +0000 Subject: [PATCH 02/73] Committing clang-format changes --- tests/standalone_driver.cxx | 10 ++++------ 1 file changed, 4 insertions(+), 6 deletions(-) diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index 6d2aaa18..3d0deb32 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -85,7 +85,7 @@ int main(int argc, char** argv) { auto nalpha = input.getData("CI.NALPHA"); auto nbeta = input.getData("CI.NBETA"); - //if(nalpha != nbeta) throw std::runtime_error("NALPHA != NBETA"); + // if(nalpha != nbeta) throw std::runtime_error("NALPHA != NBETA"); // Read FCIDUMP File size_t norb = macis::read_fcidump_norb(fcidump_fname); @@ -230,7 +230,7 @@ int main(int argc, char** argv) { // MP2 Guess Orbitals if(mp2_guess) { - if( nalpha != nbeta ) + if(nalpha != nbeta) throw std::runtime_error("MP2 Guess only implemented for closed-shell"); console->info("Calculating MP2 Natural Orbitals"); @@ -307,9 +307,8 @@ int main(int argc, char** argv) { } } else { - if(nalpha != nbeta) - throw std::runtime_error("ASCI Only Implemented for Closed-Shell"); + throw std::runtime_error("ASCI Only Implemented for Closed-Shell"); // Generate the Hamiltonian Generator generator_t ham_gen( @@ -383,8 +382,7 @@ int main(int argc, char** argv) { // MCSCF } else if(job == Job::MCSCF) { - - if( nalpha != nbeta ) + if(nalpha != nbeta) throw std::runtime_error("MCSCF Only Implemented for Closed-Shells"); // Possibly read active RDMs From b75ff55244c3a0d11ed77cea93b5b1b22ed4381d Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Tue, 6 Jun 2023 11:28:53 -0700 Subject: [PATCH 03/73] Validated Open Shell CASSCF --- tests/standalone_driver.cxx | 2 -- 1 file changed, 2 deletions(-) diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index 3d0deb32..3408a0de 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -382,8 +382,6 @@ int main(int argc, char** argv) { // MCSCF } else if(job == Job::MCSCF) { - if(nalpha != nbeta) - throw std::runtime_error("MCSCF Only Implemented for Closed-Shells"); // Possibly read active RDMs if(rdm_fname.size()) { From 6cfb79ae520ac201f53ad052c3973e2fdd595883 Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Tue, 6 Jun 2023 11:51:54 -0700 Subject: [PATCH 04/73] Minor --- tests/standalone_driver.cxx | 1 - 1 file changed, 1 deletion(-) diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index 3408a0de..32cfd240 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -283,7 +283,6 @@ int main(int argc, char** argv) { using generator_t = macis::DoubleLoopHamiltonianGenerator; if(ci_exp == CIExpansion::CAS) { std::vector C_local; - // TODO: VERIFY MPI + CAS E0 = macis::CASRDMFunctor::rdms( mcscf_settings, NumOrbital(n_active), nalpha, nbeta, T_active.data(), V_active.data(), active_ordm.data(), From 6a5528ebd457fbac4b27dc4b9945ab3ca68d962b Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Tue, 6 Jun 2023 15:27:21 -0700 Subject: [PATCH 05/73] Adding open-shell logic to ASCI --- include/macis/asci/determinant_search.hpp | 13 +++++++++---- 1 file changed, 9 insertions(+), 4 deletions(-) diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index d5332b79..4a14cce1 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -226,7 +226,12 @@ asci_contrib_container> asci_contributions_constraint( const auto n_sing_alpha = n_occ_alpha * n_vir_alpha; const auto n_doub_alpha = (n_sing_alpha * (n_sing_alpha - norb + 1)) / 4; - logger->info(" * NS = {} ND = {}", n_sing_alpha, n_doub_alpha); + const auto n_occ_beta = cdets_begin->count() - n_occ_alpha; + const auto n_vir_beta = norb - n_occ_beta; + const auto n_sing_beta = n_occ_beta * n_vir_beta; + const auto n_doub_beta = (n_sing_beta * (n_sing_beta - norb + 1)) / 4; + + //logger->info(" * NS = {} ND = {}", n_sing_alpha, n_doub_alpha); // Generate mask constraints if(!world_rank) { @@ -261,9 +266,9 @@ asci_contrib_container> asci_contributions_constraint( logger->info(" * GEN_DUR = {:.2e} ms", gen_c_dur.count()); size_t max_size = std::min(asci_settings.pair_size_max, - ncdets * (2 * n_sing_alpha + // AA + BB - 2 * n_doub_alpha + // AAAA + BBBB - n_sing_alpha * n_sing_alpha // AABB + ncdets * (n_sing_alpha + n_sing_beta +// AA + BB + n_doub_alpha + n_sing_beta +// AAAA + BBBB + n_sing_alpha * n_sing_beta // AABB )); asci_pairs.reserve(max_size); From 385a5b5432e185add468049dd00b611a7848b210 Mon Sep 17 00:00:00 2001 From: Clang Robot Date: Wed, 7 Jun 2023 17:55:07 +0000 Subject: [PATCH 06/73] Committing clang-format changes --- include/macis/asci/determinant_search.hpp | 15 ++++++++------- tests/standalone_driver.cxx | 1 - 2 files changed, 8 insertions(+), 8 deletions(-) diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index 4a14cce1..35dd3309 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -226,12 +226,12 @@ asci_contrib_container> asci_contributions_constraint( const auto n_sing_alpha = n_occ_alpha * n_vir_alpha; const auto n_doub_alpha = (n_sing_alpha * (n_sing_alpha - norb + 1)) / 4; - const auto n_occ_beta = cdets_begin->count() - n_occ_alpha; + const auto n_occ_beta = cdets_begin->count() - n_occ_alpha; const auto n_vir_beta = norb - n_occ_beta; const auto n_sing_beta = n_occ_beta * n_vir_beta; const auto n_doub_beta = (n_sing_beta * (n_sing_beta - norb + 1)) / 4; - //logger->info(" * NS = {} ND = {}", n_sing_alpha, n_doub_alpha); + // logger->info(" * NS = {} ND = {}", n_sing_alpha, n_doub_alpha); // Generate mask constraints if(!world_rank) { @@ -265,11 +265,12 @@ asci_contrib_container> asci_contributions_constraint( duration_type gen_c_dur = gen_c_en - gen_c_st; logger->info(" * GEN_DUR = {:.2e} ms", gen_c_dur.count()); - size_t max_size = std::min(asci_settings.pair_size_max, - ncdets * (n_sing_alpha + n_sing_beta +// AA + BB - n_doub_alpha + n_sing_beta +// AAAA + BBBB - n_sing_alpha * n_sing_beta // AABB - )); + size_t max_size = + std::min(asci_settings.pair_size_max, + ncdets * (n_sing_alpha + n_sing_beta + // AA + BB + n_doub_alpha + n_sing_beta + // AAAA + BBBB + n_sing_alpha * n_sing_beta // AABB + )); asci_pairs.reserve(max_size); // Process ASCI pair contributions for each constraint diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index 32cfd240..532f317f 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -381,7 +381,6 @@ int main(int argc, char** argv) { // MCSCF } else if(job == Job::MCSCF) { - // Possibly read active RDMs if(rdm_fname.size()) { console->info(" * RDMFILE = {}", rdm_fname); From 1bf63c889f51dc1a576ae88e3fe684add458dfdc Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Wed, 16 Aug 2023 10:24:58 -0700 Subject: [PATCH 07/73] Separate numerator / denominator in ASCI scores to allow for reuse in PT2 calculation --- .../macis/asci/determinant_contributions.hpp | 17 ++++++++++------- include/macis/asci/determinant_search.hpp | 19 +++++++++++-------- include/macis/asci/determinant_sort.hpp | 6 +++--- include/macis/asci/mask_constraints.hpp | 12 ++++++------ tests/asci.cxx | 1 + 5 files changed, 31 insertions(+), 24 deletions(-) diff --git a/include/macis/asci/determinant_contributions.hpp b/include/macis/asci/determinant_contributions.hpp index 7b3315f3..041979bb 100644 --- a/include/macis/asci/determinant_contributions.hpp +++ b/include/macis/asci/determinant_contributions.hpp @@ -16,7 +16,10 @@ namespace macis { template struct asci_contrib { WfnT state; - double rv; + double c_times_matel; + double h_diag; + + auto rv() const { return c_times_matel / h_diag; } }; template @@ -57,10 +60,10 @@ void append_singles_asci_contributions( // Calculate fast diagonal matrix element auto h_diag = ham_gen.fast_diag_single(eps_same[i], eps_same[a], i, a, root_diag); - h_el /= (E0 - h_diag); + //h_el /= (E0 - h_diag); // Append to return values - asci_contributions.push_back({ex_det, coeff * h_el}); + asci_contributions.push_back({ex_det, coeff * h_el, E0 - h_diag}); } // Loop over single extitations } @@ -110,10 +113,10 @@ void append_ss_doubles_asci_contributions( auto h_diag = ham_gen.fast_diag_ss_double(eps_same[i], eps_same[j], eps_same[a], eps_same[b], i, j, a, b, root_diag); - h_el /= (E0 - h_diag); + //h_el /= (E0 - h_diag); // Append {det, c*h_el} - asci_contributions.push_back({ex_det, coeff * h_el}); + asci_contributions.push_back({ex_det, coeff * h_el, E0 - h_diag}); } // Restricted BJ loop } // AI Loop @@ -152,9 +155,9 @@ void append_os_doubles_asci_contributions( auto h_diag = ham_gen.fast_diag_os_double(eps_alpha[i], eps_beta[j], eps_alpha[a], eps_beta[b], i, j, a, b, root_diag); - h_el /= (E0 - h_diag); + //h_el /= (E0 - h_diag); - asci_contributions.push_back({ex_det, coeff * h_el}); + asci_contributions.push_back({ex_det, coeff * h_el, E0 - h_diag}); } // BJ loop } // AI loop } diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index 7d66813c..03cc9b9d 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -27,7 +27,7 @@ template struct asci_contrib_topk_comparator { using type = asci_contrib; constexpr bool operator()(const type& a, const type& b) const { - return std::abs(a.rv) > std::abs(b.rv); + return std::abs(a.rv()) > std::abs(b.rv()); } }; @@ -122,7 +122,7 @@ asci_contrib_container> asci_contributions_standard( // Remove small contributions auto it = std::partition( asci_pairs.begin(), asci_pairs.end(), [=](const auto& x) { - return std::abs(x.rv) > asci_settings.rv_prune_tol; + return std::abs(x.rv()) > asci_settings.rv_prune_tol; }); asci_pairs.erase(it, asci_pairs.end()); logger->info(" * Pruning at DET = {} NSZ = {}", i, asci_pairs.size()); @@ -356,7 +356,7 @@ asci_contrib_container> asci_contributions_constraint( // Remove small contributions auto it = std::partition( asci_pairs.begin(), asci_pairs.end(), [=](const auto& x) { - return std::abs(x.rv) > asci_settings.rv_prune_tol; + return std::abs(x.rv()) > asci_settings.rv_prune_tol; }); asci_pairs.erase(it, asci_pairs.end()); @@ -527,7 +527,10 @@ std::vector> asci_search( auto keep_large_st = clock_type::now(); // Finalize scores - for(auto& x : asci_pairs) x.rv = -std::abs(x.rv); + for(auto& x : asci_pairs) { + x.c_times_matel = -std::abs(x.c_times_matel); + x.h_diag = std::abs(x.h_diag); + } // Insert all dets with their coefficients as seeds for(size_t i = 0; i < ncdets; ++i) { @@ -540,7 +543,7 @@ std::vector> asci_search( keep_only_largest_copy_asci_pairs(asci_pairs); asci_pairs.erase(std::partition(asci_pairs.begin(), asci_pairs.end(), - [](const auto& p) { return p.rv < 0.0; }), + [](const auto& p) { return p.rv() < 0.0; }), asci_pairs.end()); // Only do top-K on (ndets_max - ncdets) b/c CDETS will be added later @@ -569,7 +572,7 @@ std::vector> asci_search( // Strip scores std::vector scores(asci_pairs.size()); std::transform(asci_pairs.begin(), asci_pairs.end(), scores.begin(), - [](const auto& p) { return std::abs(p.rv); }); + [](const auto& p) { return std::abs(p.rv()); }); // Determine kth-ranked scores auto kth_score = @@ -579,8 +582,8 @@ std::vector> asci_search( // Partition local pairs into less / eq batches auto [g_begin, e_begin, l_begin, _end] = leg_partition( asci_pairs.begin(), asci_pairs.end(), kth_score, - [=](const auto& p, const auto& s) { return std::abs(p.rv) > s; }, - [=](const auto& p, const auto& s) { return std::abs(p.rv) == s; }); + [=](const auto& p, const auto& s) { return std::abs(p.rv()) > s; }, + [=](const auto& p, const auto& s) { return std::abs(p.rv()) == s; }); // Determine local counts size_t n_greater = std::distance(g_begin, e_begin); diff --git a/include/macis/asci/determinant_sort.hpp b/include/macis/asci/determinant_sort.hpp index 829f7240..dccb1a45 100644 --- a/include/macis/asci/determinant_sort.hpp +++ b/include/macis/asci/determinant_sort.hpp @@ -65,8 +65,8 @@ PairIterator sort_and_accumulate_asci_pairs(PairIterator pairs_begin, // Accumulate else { - cur_it->rv += it->rv; - it->rv = 0; // Zero out to expose potential bugs + cur_it->c_times_matel += it->c_times_matel; + it->c_times_matel = 0; // Zero out to expose potential bugs } } @@ -108,7 +108,7 @@ void keep_only_largest_copy_asci_pairs( // Keep only max value else { - cur_it->rv = std::max(cur_it->rv, it->rv); + cur_it->c_times_matel = std::max(cur_it->c_times_matel, it->c_times_matel); } } diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index c9907e09..af32fcd2 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -283,9 +283,9 @@ void generate_constraint_singles_contributions_ss( // Compute Fast Diagonal Matrix Element auto h_diag = ham_gen.fast_diag_single(eps[i], eps[a], i, a, root_diag); - h_el /= (E0 - h_diag); + //h_el /= (E0 - h_diag); - asci_contributions.push_back({ex_det, coeff * h_el}); + asci_contributions.push_back({ex_det, coeff * h_el, E0 - h_diag}); } } } @@ -336,9 +336,9 @@ void generate_constraint_doubles_contributions_ss( // Evaluate fast diagonal matrix element auto h_diag = ham_gen.fast_diag_ss_double(eps[i], eps[j], eps[a], eps[b], i, j, a, b, root_diag); - h_el /= (E0 - h_diag); + //h_el /= (E0 - h_diag); - asci_contributions.push_back({full_ex, coeff * h_el}); + asci_contributions.push_back({full_ex, coeff * h_el, E0 - h_diag}); } } } @@ -394,9 +394,9 @@ void generate_constraint_doubles_contributions_os( auto h_diag = ham_gen.fast_diag_os_double(eps_same[i], eps_othr[j], eps_same[a], eps_othr[b], i, j, a, b, root_diag); - h_el /= (E0 - h_diag); + //h_el /= (E0 - h_diag); - asci_contributions.push_back({ex_det, coeff * h_el}); + asci_contributions.push_back({ex_det, coeff * h_el, E0 - h_diag}); } // BJ } // A diff --git a/tests/asci.cxx b/tests/asci.cxx index 5542db83..03358cb5 100644 --- a/tests/asci.cxx +++ b/tests/asci.cxx @@ -254,6 +254,7 @@ TEST_CASE("ASCI") { asci_settings, mcscf_settings, E0, std::move(dets), std::move(C), ham_gen, norb MACIS_MPI_CODE(, MPI_COMM_WORLD)); + std::cout << E0 - -8.542926243842e+01 << std::endl; REQUIRE(E0 == Approx(-8.542926243842e+01)); REQUIRE(dets.size() == 10000); REQUIRE(C.size() == 10000); From f33f0f396e5593ef95080f1919756152c7ba81cf Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Wed, 16 Aug 2023 17:42:26 -0700 Subject: [PATCH 08/73] Initial implementation of EN-PT2 --- include/macis/asci/determinant_sort.hpp | 2 +- include/macis/asci/mask_constraints.hpp | 4 +- include/macis/asci/pt2.hpp | 231 ++++++++++++++++++++++++ tests/standalone_driver.cxx | 22 ++- 4 files changed, 253 insertions(+), 6 deletions(-) create mode 100644 include/macis/asci/pt2.hpp diff --git a/include/macis/asci/determinant_sort.hpp b/include/macis/asci/determinant_sort.hpp index dccb1a45..9d37ce18 100644 --- a/include/macis/asci/determinant_sort.hpp +++ b/include/macis/asci/determinant_sort.hpp @@ -66,7 +66,7 @@ PairIterator sort_and_accumulate_asci_pairs(PairIterator pairs_begin, // Accumulate else { cur_it->c_times_matel += it->c_times_matel; - it->c_times_matel = 0; // Zero out to expose potential bugs + it->c_times_matel = NAN; // Zero out to expose potential bugs } } diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index af32fcd2..5430b00b 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -258,11 +258,11 @@ void generate_constraint_singles_contributions_ss( const size_t LDV2 = LDV * LDV; for(int ii = 0; ii < no; ++ii) { const auto i = fls(o); - o.flip(i); + o.flip(i); // Disable "i"-bit so it's not used in FLS next iteration auto v_cpy = v; for(int aa = 0; aa < nv; ++aa) { const auto a = fls(v_cpy); - v_cpy.flip(a); + v_cpy.flip(a); // Disable "a"-bit so it's not used in FLS next iteration double h_el = T_pq[a + i * LDT]; const double* G_ov = G_kpq + a * LDG + i * LDG2; diff --git a/include/macis/asci/pt2.hpp b/include/macis/asci/pt2.hpp new file mode 100644 index 00000000..76a48132 --- /dev/null +++ b/include/macis/asci/pt2.hpp @@ -0,0 +1,231 @@ +/* + * MACIS Copyright (c) 2023, The Regents of the University of California, + * through Lawrence Berkeley National Laboratory (subject to receipt of + * any required approvals from the U.S. Dept. of Energy). All rights reserved. + * + * See LICENSE.txt for details + */ + +#pragma once +#include +#include + +namespace macis { + + +template +double asci_pt2_constraint( + wavefunction_iterator_t cdets_begin, wavefunction_iterator_t cdets_end, + const double E_ASCI, const std::vector& C, size_t norb, + const double* T_pq, const double* G_red, const double* V_red, + const double* G_pqrs, const double* V_pqrs, HamiltonianGenerator& ham_gen, + MPI_Comm comm) { + + using clock_type = std::chrono::high_resolution_clock; + using duration_type = std::chrono::duration; + + auto logger = spdlog::get("asci_search"); + const size_t ncdets = std::distance(cdets_begin, cdets_end); + std::cout << "NDETS PT = " << ncdets << " " << C.size() << std::endl; + std::cout << "PT E0 = " << E_ASCI << std::endl; + + std::vector occ_alpha, vir_alpha; + std::vector occ_beta, vir_beta; + + // Get unique alpha strings + std::vector> uniq_alpha_wfn(cdets_begin, cdets_end); + std::transform(uniq_alpha_wfn.begin(), uniq_alpha_wfn.end(), + uniq_alpha_wfn.begin(), + [=](const auto& w) { return w & full_mask(); }); + std::sort(uniq_alpha_wfn.begin(), uniq_alpha_wfn.end(), + bitset_less_comparator{}); + { + auto it = std::unique(uniq_alpha_wfn.begin(), uniq_alpha_wfn.end()); + uniq_alpha_wfn.erase(it, uniq_alpha_wfn.end()); + } + const size_t nuniq_alpha = uniq_alpha_wfn.size(); + + // For each unique alpha, create a list of beta string and store metadata + struct beta_coeff_data { + wfn_t beta_string; + std::vector occ_beta; + std::vector vir_beta; + std::vector orb_ens_alpha; + std::vector orb_ens_beta; + double coeff; + double h_diag; + + beta_coeff_data(double c, size_t norb, + const std::vector& occ_alpha, wfn_t w, + const HamiltonianGenerator& ham_gen) { + coeff = c; + + // Compute Beta string + const auto beta_shift = w >> N / 2; + // Reduce the number of times things shift in inner loop + beta_string = beta_shift << N / 2; + + // Compute diagonal matrix element + h_diag = ham_gen.matrix_element(w, w); + + // Compute occ/vir for beta string + bitset_to_occ_vir(norb, beta_shift, occ_beta, vir_beta); + + // Precompute orbital energies + orb_ens_alpha = ham_gen.single_orbital_ens(norb, occ_alpha, occ_beta); + orb_ens_beta = ham_gen.single_orbital_ens(norb, occ_beta, occ_alpha); + } + }; + + struct unique_alpha_data { + std::vector bcd; + }; + + std::vector uad(nuniq_alpha); + for(auto i = 0; i < nuniq_alpha; ++i) { + const auto wfn_a = uniq_alpha_wfn[i]; + std::vector occ_alpha, vir_alpha; + bitset_to_occ_vir(norb, wfn_a, occ_alpha, vir_alpha); + for(auto j = 0; j < ncdets; ++j) { + const auto w = *(cdets_begin + j); + if((w & full_mask()) == wfn_a) { + uad[i].bcd.emplace_back(C[j], norb, occ_alpha, w, ham_gen); + } + } + } + + auto world_rank = comm_rank(comm); + auto world_size = comm_size(comm); + + const auto n_occ_alpha = uniq_alpha_wfn[0].count(); + const auto n_vir_alpha = norb - n_occ_alpha; + const auto n_sing_alpha = n_occ_alpha * n_vir_alpha; + const auto n_doub_alpha = (n_sing_alpha * (n_sing_alpha - norb + 1)) / 4; + + logger->info(" * NS = {} ND = {}", n_sing_alpha, n_doub_alpha); + + auto gen_c_st = clock_type::now(); + auto constraints = + dist_constraint_general(0, norb, + n_sing_alpha, n_doub_alpha, uniq_alpha_wfn, comm); + auto gen_c_en = clock_type::now(); + duration_type gen_c_dur = gen_c_en - gen_c_st; + logger->info(" * GEN_DUR = {:.2e} ms", gen_c_dur.count()); + + size_t max_size = std::min(100000000ul, + ncdets * (2 * n_sing_alpha + // AA + BB + 2 * n_doub_alpha + // AAAA + BBBB + n_sing_alpha * n_sing_alpha // AABB + )); + double EPT2 = 0.0; + + // Process ASCI pair contributions for each constraint + #pragma omp parallel + { + asci_contrib_container> asci_pairs; + asci_pairs.reserve(max_size); + #pragma omp for reduction(+:EPT2) + for(size_t ic = 0; ic < constraints.size(); ++ic) { + const auto& con = constraints[ic]; + //std::cout << std::distance(&constraints[0], &con) << "/" << constraints.size() << std::endl; + const double h_el_tol = 1e-16; + const auto& [C, B, C_min] = con; + wfn_t O = full_mask(norb); + + // Loop over unique alpha strings + for(size_t i_alpha = 0; i_alpha < nuniq_alpha; ++i_alpha) { + const auto& det = uniq_alpha_wfn[i_alpha]; + const auto occ_alpha = bits_to_indices(det); + + // AA excitations + for(const auto& bcd : uad[i_alpha].bcd) { + const auto& beta = bcd.beta_string; + const auto& coeff = bcd.coeff; + const auto& h_diag = bcd.h_diag; + const auto& occ_beta = bcd.occ_beta; + const auto& orb_ens_alpha = bcd.orb_ens_alpha; + generate_constraint_singles_contributions_ss( + coeff, det, C, O, B, beta, occ_alpha, occ_beta, + orb_ens_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, + h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); + } + + // AAAA excitations + for(const auto& bcd : uad[i_alpha].bcd) { + const auto& beta = bcd.beta_string; + const auto& coeff = bcd.coeff; + const auto& h_diag = bcd.h_diag; + const auto& occ_beta = bcd.occ_beta; + const auto& orb_ens_alpha = bcd.orb_ens_alpha; + generate_constraint_doubles_contributions_ss( + coeff, det, C, O, B, beta, occ_alpha, occ_beta, + orb_ens_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, + ham_gen, asci_pairs); + } + + // AABB excitations + for(const auto& bcd : uad[i_alpha].bcd) { + const auto& beta = bcd.beta_string; + const auto& coeff = bcd.coeff; + const auto& h_diag = bcd.h_diag; + const auto& occ_beta = bcd.occ_beta; + const auto& vir_beta = bcd.vir_beta; + const auto& orb_ens_alpha = bcd.orb_ens_alpha; + const auto& orb_ens_beta = bcd.orb_ens_beta; + generate_constraint_doubles_contributions_os( + coeff, det, C, O, B, beta, occ_alpha, occ_beta, vir_beta, + orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, + h_diag, E_ASCI, ham_gen, asci_pairs); + } + + // If the alpha determinant satisfies the constraint, + // append BB and BBBB excitations + if(satisfies_constraint(det, C, C_min)) { + for(const auto& bcd : uad[i_alpha].bcd) { + const auto& beta = bcd.beta_string; + const auto& coeff = bcd.coeff; + const auto& h_diag = bcd.h_diag; + const auto& occ_beta = bcd.occ_beta; + const auto& vir_beta = bcd.vir_beta; + const auto& eps_beta = bcd.orb_ens_beta; + + const auto state = det | beta; + const auto state_beta = bitset_hi_word(beta); + // BB Excitations + append_singles_asci_contributions<(N / 2), (N / 2)>( + coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, + eps_beta.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, + h_diag, E_ASCI, ham_gen, asci_pairs); + + // BBBB Excitations + append_ss_doubles_asci_contributions( + coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, + eps_beta.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, + asci_pairs); + + // No excition - to remove for PT2 + asci_pairs.push_back({state, std::numeric_limits::infinity(), 1.0}); + } // Beta Loop + } // Triplet Check + + } // Unique Alpha Loop + + double EPT2_local = 0.0; + // Local S&A for each quad + update EPT2 + { + auto uit = sort_and_accumulate_asci_pairs(asci_pairs.begin(), asci_pairs.end()); + for(auto it = asci_pairs.begin(); it != uit; ++it) { + //if(std::find(cdets_begin, cdets_end, it->state) == cdets_end) + if(!std::isinf(it->c_times_matel)) + EPT2_local += (it->c_times_matel * it->c_times_matel) / it->h_diag; + } + asci_pairs.clear(); + } + + EPT2 += EPT2_local; + } // Constraint Loop + } + + return EPT2; +} +} diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index 44794230..8ce5cfe8 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -16,6 +16,7 @@ #include #include #include +#include #include #include #include @@ -277,7 +278,9 @@ int main(int argc, char** argv) { std::vector active_ordm(n_active * n_active); std::vector active_trdm(active_ordm.size() * active_ordm.size()); + bool pt2 = true; double E0 = 0; + double EPT2 = 0; // CI if(job == Job::CI) { @@ -378,9 +381,22 @@ int main(int argc, char** argv) { sparsexx::write_dist_mm("ham.mtx", H, 1); } #endif + if(pt2) { + EPT2 = macis::asci_pt2_constraint( dets.begin(), dets.end(), E0 -(E_inactive + E_core), C, n_active, + ham_gen.T(), ham_gen.G_red(), ham_gen.V_red(),ham_gen.G(), ham_gen.V(), + ham_gen MACIS_MPI_CODE(, MPI_COMM_WORLD)); + } + } + + console->info("E(CI) = {:.12f} Eh", E0); + + if(pt2) { + console->info("E(PT2) = {:.12f} Eh", EPT2); + console->info("E(CI+PT2) = {:.12f} Eh", E0 + EPT2); } - // MCSCF + + // MCSCF } else if(job == Job::MCSCF) { // Possibly read active RDMs if(rdm_fname.size()) { @@ -410,9 +426,9 @@ int main(int argc, char** argv) { NumVirtual(n_virtual), E_core, T.data(), norb, V.data(), norb, active_ordm.data(), n_active, active_trdm.data(), n_active MACIS_MPI_CODE(, MPI_COMM_WORLD)); - } - console->info("E(CI) = {:.12f} Eh", E0); + console->info("E(CASSCF) = {:.12f} Eh", E0); + } // Write FCIDUMP file if requested if(fci_out_fname.size()) From 5e9f7fe503d4826b6af9ae68701d12cc9dc28ab7 Mon Sep 17 00:00:00 2001 From: Clang Robot Date: Thu, 17 Aug 2023 00:43:03 +0000 Subject: [PATCH 09/73] Committing clang-format changes --- .../macis/asci/determinant_contributions.hpp | 8 +- include/macis/asci/determinant_search.hpp | 2 +- include/macis/asci/determinant_sort.hpp | 3 +- include/macis/asci/mask_constraints.hpp | 10 +- include/macis/asci/pt2.hpp | 219 +++++++++--------- tests/standalone_driver.cxx | 12 +- 6 files changed, 128 insertions(+), 126 deletions(-) diff --git a/include/macis/asci/determinant_contributions.hpp b/include/macis/asci/determinant_contributions.hpp index 041979bb..759fea05 100644 --- a/include/macis/asci/determinant_contributions.hpp +++ b/include/macis/asci/determinant_contributions.hpp @@ -18,7 +18,7 @@ struct asci_contrib { WfnT state; double c_times_matel; double h_diag; - + auto rv() const { return c_times_matel / h_diag; } }; @@ -60,7 +60,7 @@ void append_singles_asci_contributions( // Calculate fast diagonal matrix element auto h_diag = ham_gen.fast_diag_single(eps_same[i], eps_same[a], i, a, root_diag); - //h_el /= (E0 - h_diag); + // h_el /= (E0 - h_diag); // Append to return values asci_contributions.push_back({ex_det, coeff * h_el, E0 - h_diag}); @@ -113,7 +113,7 @@ void append_ss_doubles_asci_contributions( auto h_diag = ham_gen.fast_diag_ss_double(eps_same[i], eps_same[j], eps_same[a], eps_same[b], i, j, a, b, root_diag); - //h_el /= (E0 - h_diag); + // h_el /= (E0 - h_diag); // Append {det, c*h_el} asci_contributions.push_back({ex_det, coeff * h_el, E0 - h_diag}); @@ -155,7 +155,7 @@ void append_os_doubles_asci_contributions( auto h_diag = ham_gen.fast_diag_os_double(eps_alpha[i], eps_beta[j], eps_alpha[a], eps_beta[b], i, j, a, b, root_diag); - //h_el /= (E0 - h_diag); + // h_el /= (E0 - h_diag); asci_contributions.push_back({ex_det, coeff * h_el, E0 - h_diag}); } // BJ loop diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index 03cc9b9d..c3c4fec2 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -529,7 +529,7 @@ std::vector> asci_search( // Finalize scores for(auto& x : asci_pairs) { x.c_times_matel = -std::abs(x.c_times_matel); - x.h_diag = std::abs(x.h_diag); + x.h_diag = std::abs(x.h_diag); } // Insert all dets with their coefficients as seeds diff --git a/include/macis/asci/determinant_sort.hpp b/include/macis/asci/determinant_sort.hpp index 9d37ce18..25de9878 100644 --- a/include/macis/asci/determinant_sort.hpp +++ b/include/macis/asci/determinant_sort.hpp @@ -108,7 +108,8 @@ void keep_only_largest_copy_asci_pairs( // Keep only max value else { - cur_it->c_times_matel = std::max(cur_it->c_times_matel, it->c_times_matel); + cur_it->c_times_matel = + std::max(cur_it->c_times_matel, it->c_times_matel); } } diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index 5430b00b..bf522f26 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -258,11 +258,11 @@ void generate_constraint_singles_contributions_ss( const size_t LDV2 = LDV * LDV; for(int ii = 0; ii < no; ++ii) { const auto i = fls(o); - o.flip(i); // Disable "i"-bit so it's not used in FLS next iteration + o.flip(i); // Disable "i"-bit so it's not used in FLS next iteration auto v_cpy = v; for(int aa = 0; aa < nv; ++aa) { const auto a = fls(v_cpy); - v_cpy.flip(a); // Disable "a"-bit so it's not used in FLS next iteration + v_cpy.flip(a); // Disable "a"-bit so it's not used in FLS next iteration double h_el = T_pq[a + i * LDT]; const double* G_ov = G_kpq + a * LDG + i * LDG2; @@ -283,7 +283,7 @@ void generate_constraint_singles_contributions_ss( // Compute Fast Diagonal Matrix Element auto h_diag = ham_gen.fast_diag_single(eps[i], eps[a], i, a, root_diag); - //h_el /= (E0 - h_diag); + // h_el /= (E0 - h_diag); asci_contributions.push_back({ex_det, coeff * h_el, E0 - h_diag}); } @@ -336,7 +336,7 @@ void generate_constraint_doubles_contributions_ss( // Evaluate fast diagonal matrix element auto h_diag = ham_gen.fast_diag_ss_double(eps[i], eps[j], eps[a], eps[b], i, j, a, b, root_diag); - //h_el /= (E0 - h_diag); + // h_el /= (E0 - h_diag); asci_contributions.push_back({full_ex, coeff * h_el, E0 - h_diag}); } @@ -394,7 +394,7 @@ void generate_constraint_doubles_contributions_os( auto h_diag = ham_gen.fast_diag_os_double(eps_same[i], eps_othr[j], eps_same[a], eps_othr[b], i, j, a, b, root_diag); - //h_el /= (E0 - h_diag); + // h_el /= (E0 - h_diag); asci_contributions.push_back({ex_det, coeff * h_el, E0 - h_diag}); } // BJ diff --git a/include/macis/asci/pt2.hpp b/include/macis/asci/pt2.hpp index 76a48132..8ef19245 100644 --- a/include/macis/asci/pt2.hpp +++ b/include/macis/asci/pt2.hpp @@ -12,21 +12,20 @@ namespace macis { - template -double asci_pt2_constraint( - wavefunction_iterator_t cdets_begin, wavefunction_iterator_t cdets_end, - const double E_ASCI, const std::vector& C, size_t norb, - const double* T_pq, const double* G_red, const double* V_red, - const double* G_pqrs, const double* V_pqrs, HamiltonianGenerator& ham_gen, - MPI_Comm comm) { - +double asci_pt2_constraint(wavefunction_iterator_t cdets_begin, + wavefunction_iterator_t cdets_end, + const double E_ASCI, const std::vector& C, + size_t norb, const double* T_pq, const double* G_red, + const double* V_red, const double* G_pqrs, + const double* V_pqrs, + HamiltonianGenerator& ham_gen, MPI_Comm comm) { using clock_type = std::chrono::high_resolution_clock; using duration_type = std::chrono::duration; auto logger = spdlog::get("asci_search"); const size_t ncdets = std::distance(cdets_begin, cdets_end); - std::cout << "NDETS PT = " << ncdets << " " << C.size() << std::endl; + std::cout << "NDETS PT = " << ncdets << " " << C.size() << std::endl; std::cout << "PT E0 = " << E_ASCI << std::endl; std::vector occ_alpha, vir_alpha; @@ -105,9 +104,8 @@ double asci_pt2_constraint( logger->info(" * NS = {} ND = {}", n_sing_alpha, n_doub_alpha); auto gen_c_st = clock_type::now(); - auto constraints = - dist_constraint_general(0, norb, - n_sing_alpha, n_doub_alpha, uniq_alpha_wfn, comm); + auto constraints = dist_constraint_general( + 0, norb, n_sing_alpha, n_doub_alpha, uniq_alpha_wfn, comm); auto gen_c_en = clock_type::now(); duration_type gen_c_dur = gen_c_en - gen_c_st; logger->info(" * GEN_DUR = {:.2e} ms", gen_c_dur.count()); @@ -119,113 +117,116 @@ double asci_pt2_constraint( )); double EPT2 = 0.0; - // Process ASCI pair contributions for each constraint - #pragma omp parallel +// Process ASCI pair contributions for each constraint +#pragma omp parallel { - asci_contrib_container> asci_pairs; - asci_pairs.reserve(max_size); - #pragma omp for reduction(+:EPT2) - for(size_t ic = 0; ic < constraints.size(); ++ic) { - const auto& con = constraints[ic]; - //std::cout << std::distance(&constraints[0], &con) << "/" << constraints.size() << std::endl; - const double h_el_tol = 1e-16; - const auto& [C, B, C_min] = con; - wfn_t O = full_mask(norb); - - // Loop over unique alpha strings - for(size_t i_alpha = 0; i_alpha < nuniq_alpha; ++i_alpha) { - const auto& det = uniq_alpha_wfn[i_alpha]; - const auto occ_alpha = bits_to_indices(det); - - // AA excitations - for(const auto& bcd : uad[i_alpha].bcd) { - const auto& beta = bcd.beta_string; - const auto& coeff = bcd.coeff; - const auto& h_diag = bcd.h_diag; - const auto& occ_beta = bcd.occ_beta; - const auto& orb_ens_alpha = bcd.orb_ens_alpha; - generate_constraint_singles_contributions_ss( - coeff, det, C, O, B, beta, occ_alpha, occ_beta, - orb_ens_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, - h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); - } - - // AAAA excitations - for(const auto& bcd : uad[i_alpha].bcd) { - const auto& beta = bcd.beta_string; - const auto& coeff = bcd.coeff; - const auto& h_diag = bcd.h_diag; - const auto& occ_beta = bcd.occ_beta; - const auto& orb_ens_alpha = bcd.orb_ens_alpha; - generate_constraint_doubles_contributions_ss( - coeff, det, C, O, B, beta, occ_alpha, occ_beta, - orb_ens_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, - ham_gen, asci_pairs); - } - - // AABB excitations - for(const auto& bcd : uad[i_alpha].bcd) { - const auto& beta = bcd.beta_string; - const auto& coeff = bcd.coeff; - const auto& h_diag = bcd.h_diag; - const auto& occ_beta = bcd.occ_beta; - const auto& vir_beta = bcd.vir_beta; - const auto& orb_ens_alpha = bcd.orb_ens_alpha; - const auto& orb_ens_beta = bcd.orb_ens_beta; - generate_constraint_doubles_contributions_os( - coeff, det, C, O, B, beta, occ_alpha, occ_beta, vir_beta, - orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, - h_diag, E_ASCI, ham_gen, asci_pairs); - } - - // If the alpha determinant satisfies the constraint, - // append BB and BBBB excitations - if(satisfies_constraint(det, C, C_min)) { + asci_contrib_container> asci_pairs; + asci_pairs.reserve(max_size); +#pragma omp for reduction(+ : EPT2) + for(size_t ic = 0; ic < constraints.size(); ++ic) { + const auto& con = constraints[ic]; + // std::cout << std::distance(&constraints[0], &con) << "/" << + // constraints.size() << std::endl; + const double h_el_tol = 1e-16; + const auto& [C, B, C_min] = con; + wfn_t O = full_mask(norb); + + // Loop over unique alpha strings + for(size_t i_alpha = 0; i_alpha < nuniq_alpha; ++i_alpha) { + const auto& det = uniq_alpha_wfn[i_alpha]; + const auto occ_alpha = bits_to_indices(det); + + // AA excitations + for(const auto& bcd : uad[i_alpha].bcd) { + const auto& beta = bcd.beta_string; + const auto& coeff = bcd.coeff; + const auto& h_diag = bcd.h_diag; + const auto& occ_beta = bcd.occ_beta; + const auto& orb_ens_alpha = bcd.orb_ens_alpha; + generate_constraint_singles_contributions_ss( + coeff, det, C, O, B, beta, occ_alpha, occ_beta, + orb_ens_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, + h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); + } + + // AAAA excitations + for(const auto& bcd : uad[i_alpha].bcd) { + const auto& beta = bcd.beta_string; + const auto& coeff = bcd.coeff; + const auto& h_diag = bcd.h_diag; + const auto& occ_beta = bcd.occ_beta; + const auto& orb_ens_alpha = bcd.orb_ens_alpha; + generate_constraint_doubles_contributions_ss( + coeff, det, C, O, B, beta, occ_alpha, occ_beta, + orb_ens_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, + ham_gen, asci_pairs); + } + + // AABB excitations for(const auto& bcd : uad[i_alpha].bcd) { const auto& beta = bcd.beta_string; const auto& coeff = bcd.coeff; const auto& h_diag = bcd.h_diag; const auto& occ_beta = bcd.occ_beta; const auto& vir_beta = bcd.vir_beta; - const auto& eps_beta = bcd.orb_ens_beta; - - const auto state = det | beta; - const auto state_beta = bitset_hi_word(beta); - // BB Excitations - append_singles_asci_contributions<(N / 2), (N / 2)>( - coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, - eps_beta.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, + const auto& orb_ens_alpha = bcd.orb_ens_alpha; + const auto& orb_ens_beta = bcd.orb_ens_beta; + generate_constraint_doubles_contributions_os( + coeff, det, C, O, B, beta, occ_alpha, occ_beta, vir_beta, + orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); + } + + // If the alpha determinant satisfies the constraint, + // append BB and BBBB excitations + if(satisfies_constraint(det, C, C_min)) { + for(const auto& bcd : uad[i_alpha].bcd) { + const auto& beta = bcd.beta_string; + const auto& coeff = bcd.coeff; + const auto& h_diag = bcd.h_diag; + const auto& occ_beta = bcd.occ_beta; + const auto& vir_beta = bcd.vir_beta; + const auto& eps_beta = bcd.orb_ens_beta; + + const auto state = det | beta; + const auto state_beta = bitset_hi_word(beta); + // BB Excitations + append_singles_asci_contributions<(N / 2), (N / 2)>( + coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, + eps_beta.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, + h_diag, E_ASCI, ham_gen, asci_pairs); + + // BBBB Excitations + append_ss_doubles_asci_contributions( + coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, + eps_beta.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, + ham_gen, asci_pairs); + + // No excition - to remove for PT2 + asci_pairs.push_back( + {state, std::numeric_limits::infinity(), 1.0}); + } // Beta Loop + } // Triplet Check + + } // Unique Alpha Loop + + double EPT2_local = 0.0; + // Local S&A for each quad + update EPT2 + { + auto uit = sort_and_accumulate_asci_pairs(asci_pairs.begin(), + asci_pairs.end()); + for(auto it = asci_pairs.begin(); it != uit; ++it) { + // if(std::find(cdets_begin, cdets_end, it->state) == cdets_end) + if(!std::isinf(it->c_times_matel)) + EPT2_local += (it->c_times_matel * it->c_times_matel) / it->h_diag; + } + asci_pairs.clear(); + } - // BBBB Excitations - append_ss_doubles_asci_contributions( - coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, - eps_beta.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, - asci_pairs); - - // No excition - to remove for PT2 - asci_pairs.push_back({state, std::numeric_limits::infinity(), 1.0}); - } // Beta Loop - } // Triplet Check - - } // Unique Alpha Loop - - double EPT2_local = 0.0; - // Local S&A for each quad + update EPT2 - { - auto uit = sort_and_accumulate_asci_pairs(asci_pairs.begin(), asci_pairs.end()); - for(auto it = asci_pairs.begin(); it != uit; ++it) { - //if(std::find(cdets_begin, cdets_end, it->state) == cdets_end) - if(!std::isinf(it->c_times_matel)) - EPT2_local += (it->c_times_matel * it->c_times_matel) / it->h_diag; - } - asci_pairs.clear(); - } - - EPT2 += EPT2_local; - } // Constraint Loop + EPT2 += EPT2_local; + } // Constraint Loop } return EPT2; } -} +} // namespace macis diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index 8ce5cfe8..c00f497d 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -15,8 +15,8 @@ #include #include #include -#include #include +#include #include #include #include @@ -382,9 +382,10 @@ int main(int argc, char** argv) { } #endif if(pt2) { - EPT2 = macis::asci_pt2_constraint( dets.begin(), dets.end(), E0 -(E_inactive + E_core), C, n_active, - ham_gen.T(), ham_gen.G_red(), ham_gen.V_red(),ham_gen.G(), ham_gen.V(), - ham_gen MACIS_MPI_CODE(, MPI_COMM_WORLD)); + EPT2 = macis::asci_pt2_constraint( + dets.begin(), dets.end(), E0 - (E_inactive + E_core), C, n_active, + ham_gen.T(), ham_gen.G_red(), ham_gen.V_red(), ham_gen.G(), + ham_gen.V(), ham_gen MACIS_MPI_CODE(, MPI_COMM_WORLD)); } } @@ -395,8 +396,7 @@ int main(int argc, char** argv) { console->info("E(CI+PT2) = {:.12f} Eh", E0 + EPT2); } - - // MCSCF + // MCSCF } else if(job == Job::MCSCF) { // Possibly read active RDMs if(rdm_fname.size()) { From b17a8238da5ea4e55c0ab533f6a735b9a6258b3e Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Thu, 31 Aug 2023 10:03:51 -0700 Subject: [PATCH 10/73] PT2 works with MPI --- include/macis/asci/pt2.hpp | 6 ++++-- 1 file changed, 4 insertions(+), 2 deletions(-) diff --git a/include/macis/asci/pt2.hpp b/include/macis/asci/pt2.hpp index 76a48132..07560ed0 100644 --- a/include/macis/asci/pt2.hpp +++ b/include/macis/asci/pt2.hpp @@ -26,8 +26,8 @@ double asci_pt2_constraint( auto logger = spdlog::get("asci_search"); const size_t ncdets = std::distance(cdets_begin, cdets_end); - std::cout << "NDETS PT = " << ncdets << " " << C.size() << std::endl; - std::cout << "PT E0 = " << E_ASCI << std::endl; + //std::cout << "NDETS PT = " << ncdets << " " << C.size() << std::endl; + //std::cout << "PT E0 = " << E_ASCI << std::endl; std::vector occ_alpha, vir_alpha; std::vector occ_beta, vir_beta; @@ -226,6 +226,8 @@ double asci_pt2_constraint( } // Constraint Loop } + EPT2 = allreduce(EPT2, MPI_SUM, comm); + return EPT2; } } From 7a4097ed21c2ca92c91fc9ba4d3c8803f5b4a952 Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Wed, 6 Sep 2023 16:48:06 -0700 Subject: [PATCH 11/73] Start generic wfn implementations --- include/macis/sd_operations.hpp | 458 ++++++++----------------- include/macis/util/cas.hpp | 2 +- include/macis/util/unused_untested.hpp | 194 +++++++++++ include/macis/wavefunction_io.hpp | 2 +- tests/sd_operations.cxx | 36 +- tests/standalone_driver.cxx | 5 +- 6 files changed, 356 insertions(+), 341 deletions(-) create mode 100644 include/macis/util/unused_untested.hpp diff --git a/include/macis/sd_operations.hpp b/include/macis/sd_operations.hpp index c04267f8..77150990 100644 --- a/include/macis/sd_operations.hpp +++ b/include/macis/sd_operations.hpp @@ -35,39 +35,6 @@ std::bitset canonical_hf_determinant(uint32_t nalpha, uint32_t nbeta) { return alpha | beta; } -/** - * @brief Generate canonical HF determinant. - * - * Generates a string representation of the canonical HF determinant - * consisting of a specifed number of alpha and beta orbitals. This variant - * does not assume energetic ordering of the HF orbitals. - * - * TODO: This assumes restricted orbitals - * - * @tparam N Number of bits for the total bit string of the state - * @param[in] nalpha Number of occupied alpha orbitals in the HF state - * @param[in] nbeta Number of occupied beta orbitals in the HF state - * @param[in] orb_ens Orbital eigenenergies. - * - * @returns The bitstring HF state consisting of the specified number of - * occupied orbitals populated according to the ordering of `orb_ens`. - */ -template -std::bitset canonical_hf_determinant(uint32_t nalpha, uint32_t nbeta, - const std::vector& orb_ens) { - static_assert((N % 2) == 0, "N Must Be Even"); - // First, find the sorted indices for the orbital energies - std::vector idx(orb_ens.size()); - std::iota(idx.begin(), idx.end(), 0); - std::stable_sort(idx.begin(), idx.end(), [&orb_ens](size_t i1, size_t i2) { - return orb_ens[i1] < orb_ens[i2]; - }); - // Next, fill the electrons by energy - std::bitset alpha(0), beta(0); - for(uint32_t i = 0; i < nalpha; i++) alpha.flip(idx[i]); - for(uint32_t i = 0; i < nbeta; i++) beta.flip(idx[i] + N / 2); - return alpha | beta; -} /** * @brief Generate the list of (un)occupied orbitals for a paricular state. @@ -95,40 +62,65 @@ void bitset_to_occ_vir(size_t norb, std::bitset state, } } -/** - * @brief Generate the list of (un)occupied orbitals for a paricular state. - * - * TODO: Test this function - * - * @tparam N Number of bits for the total bit string of the state - * @param[in] norb Number of orbitals used to describe the state (<= `N`) - * @param[in] state The state from which to determine orbital occupations. - * @param[out] occ List of occupied orbitals in `state` - * @param[out] vir List of unoccupied orbitals in `state` - * @param[in] as_orbs TODO:???? - */ +template +struct spin_wavefunction_type; template -void bitset_to_occ_vir_as(size_t norb, std::bitset state, - std::vector& occ, - std::vector& vir, - const std::vector& as_orbs) { - occ.clear(); - for(const auto i : as_orbs) - if(state[i]) occ.emplace_back(i); - const auto nocc = occ.size(); - assert(nocc <= norb); +struct spin_wavefunction_type> { + using type = std::bitset; +}; +template +using spin_wfn_t = typename spin_wavefunction_type::type; - const auto nvir = as_orbs.size() - nocc; - vir.resize(nvir); - auto it = vir.begin(); - for(const auto i : as_orbs) - if(!state[i]) *(it++) = i; +template +auto create_no_check(std::bitset state, unsigned p) { + return state.flip(p); +} + +template +auto single_excitation(std::bitset state, unsigned p, unsigned q) { + return state.flip(p).flip(q); +} + +template +auto double_excitation(std::bitset state, unsigned p, unsigned q, unsigned r, unsigned s) { + return state.flip(p).flip(q).flip(r).flip(s); } template -void append_singles(std::bitset state, const std::vector& occ, +auto alpha_string(std::bitset state) { return bitset_lo_word(state); } +template +auto beta_string(std::bitset state) { return bitset_hi_word(state); } +template +std::bitset<2*N> from_spin(std::bitset alpha, std::bitset beta) { + auto alpha_expand = expand_bitset<2*N>(alpha); + auto beta_expand = expand_bitset<2*N>(beta) << N; + return alpha_expand | beta_expand; +} + + +// TODO: Test this function +template +uint32_t first_occupied_flipped(std::bitset state, std::bitset ex) { + return ffs(state & ex) - 1u; +} + +// TODO: Test this function +template +double single_excitation_sign(std::bitset state, unsigned p, unsigned q) { + std::bitset mask = 0ul; + + if(p > q) { + mask = state & (full_mask(p) ^ full_mask(q + 1)); + } else { + mask = state & (full_mask(q) ^ full_mask(p + 1)); + } + return (mask.count() % 2) ? -1. : 1.; +} + +template +void append_singles(WfnType state, const std::vector& occ, const std::vector& vir, - std::vector>& singles) { + WfnContainer& singles) { const size_t nocc = occ.size(); const size_t nvir = vir.size(); @@ -137,15 +129,14 @@ void append_singles(std::bitset state, const std::vector& occ, for(size_t a = 0; a < nvir; ++a) for(size_t i = 0; i < nocc; ++i) { - auto ex = std::bitset(0).flip(occ[i]).flip(vir[a]); - singles.emplace_back(state ^ ex); + singles.emplace_back(single_excitation(state, occ[i], vir[a])); } } -template -void append_doubles(std::bitset state, const std::vector& occ, +template +void append_doubles(WfnType state, const std::vector& occ, const std::vector& vir, - std::vector>& doubles) { + WfnContainer& doubles) { const size_t nocc = occ.size(); const size_t nvir = vir.size(); @@ -158,16 +149,12 @@ void append_doubles(std::bitset state, const std::vector& occ, for(size_t i = 0; i < nocc; ++i) for(size_t b = a + 1; b < nvir; ++b) for(size_t j = i + 1; j < nocc; ++j) { - auto ex = - std::bitset(0).flip(occ[i]).flip(vir[a]).flip(occ[j]).flip( - vir[b]); - doubles.emplace_back(state ^ ex); + doubles.emplace_back(double_excitation(state, occ[i], occ[j], vir[a], vir[b])); } } -template -void generate_singles(size_t norb, std::bitset state, - std::vector>& singles) { +template +void generate_singles(size_t norb, WfnType state, WfnContainer& singles) { std::vector occ_orbs, vir_orbs; bitset_to_occ_vir(norb, state, occ_orbs, vir_orbs); @@ -175,9 +162,8 @@ void generate_singles(size_t norb, std::bitset state, append_singles(state, occ_orbs, vir_orbs, singles); } -template -void generate_doubles(size_t norb, std::bitset state, - std::vector>& doubles) { +template +void generate_doubles(size_t norb, WfnType state, WfnContainer& doubles) { std::vector occ_orbs, vir_orbs; bitset_to_occ_vir(norb, state, occ_orbs, vir_orbs); @@ -185,10 +171,9 @@ void generate_doubles(size_t norb, std::bitset state, append_doubles(state, occ_orbs, vir_orbs, doubles); } -template -void generate_singles_doubles(size_t norb, std::bitset state, - std::vector>& singles, - std::vector>& doubles) { +template +void generate_singles_doubles(size_t norb, WfnType state, + WfnContainer& singles, WfnContainer& doubles) { std::vector occ_orbs, vir_orbs; bitset_to_occ_vir(norb, state, occ_orbs, vir_orbs); @@ -198,197 +183,61 @@ void generate_singles_doubles(size_t norb, std::bitset state, append_doubles(state, occ_orbs, vir_orbs, doubles); } -// TODO: Test this function -template -void generate_singles_as(size_t norb, std::bitset state, - std::vector>& singles, - const std::vector& as_orbs) { - std::vector occ_orbs, vir_orbs; - bitset_to_occ_vir_as(norb, state, occ_orbs, vir_orbs, as_orbs); - - singles.clear(); - append_singles(state, occ_orbs, vir_orbs, singles); -} - -// TODO: Test this function -template -void generate_singles_doubles_as(size_t norb, std::bitset state, - std::vector>& singles, - std::vector>& doubles, - const std::vector& as_orbs) { - std::vector occ_orbs, vir_orbs; - bitset_to_occ_vir_as(norb, state, occ_orbs, vir_orbs, as_orbs); - - singles.clear(); - doubles.clear(); - append_singles(state, occ_orbs, vir_orbs, singles); - append_doubles(state, occ_orbs, vir_orbs, doubles); -} - -// TODO: Test this function -template -void generate_singles_spin_as(size_t norb, std::bitset state, - std::vector>& singles, - const std::vector as_orbs) { - auto state_alpha = bitset_lo_word(state); - auto state_beta = bitset_hi_word(state); - - std::vector> singles_alpha, singles_beta; - - // Generate Spin-Specific singles - generate_singles_as(norb, state_alpha, singles_alpha, as_orbs); - generate_singles_as(norb, state_beta, singles_beta, as_orbs); - - auto state_alpha_expand = expand_bitset(state_alpha); - auto state_beta_expand = expand_bitset(state_beta) << (N / 2); - - // Generate Singles in full space - singles.clear(); - - // Single Alpha + No Beta - for(auto s_alpha : singles_alpha) { - auto s_state = expand_bitset(s_alpha); - s_state = s_state | state_beta_expand; - singles.emplace_back(s_state); - } - - // No Alpha + Single Beta - for(auto s_beta : singles_beta) { - auto s_state = expand_bitset(s_beta) << (N / 2); - s_state = s_state | state_alpha_expand; - singles.emplace_back(s_state); - } -} - -// TODO: Test this function -template -void generate_singles_doubles_spin_as(size_t norb, std::bitset state, - std::vector>& singles, - std::vector>& doubles, - const std::vector& as_orbs) { - auto state_alpha = bitset_lo_word(state); - auto state_beta = bitset_hi_word(state); - - std::vector> singles_alpha, singles_beta; - std::vector> doubles_alpha, doubles_beta; - - // Generate Spin-Specific singles / doubles - generate_singles_doubles_as(norb, state_alpha, singles_alpha, doubles_alpha, - as_orbs); - generate_singles_doubles_as(norb, state_beta, singles_beta, doubles_beta, - as_orbs); - - auto state_alpha_expand = expand_bitset(state_alpha); - auto state_beta_expand = expand_bitset(state_beta) << (N / 2); - - // Generate Singles in full space - singles.clear(); - - // Single Alpha + No Beta - for(auto s_alpha : singles_alpha) { - auto s_state = expand_bitset(s_alpha); - s_state = s_state | state_beta_expand; - singles.emplace_back(s_state); - } - // No Alpha + Single Beta - for(auto s_beta : singles_beta) { - auto s_state = expand_bitset(s_beta) << (N / 2); - s_state = s_state | state_alpha_expand; - singles.emplace_back(s_state); - } - - // Generate Doubles in full space - doubles.clear(); +template +void generate_singles_spin(size_t norb, WfnType state, WfnContainer& singles) { - // Double Alpha + No Beta - for(auto d_alpha : doubles_alpha) { - auto d_state = expand_bitset(d_alpha); - d_state = d_state | state_beta_expand; - doubles.emplace_back(d_state); - } + auto state_alpha = alpha_string(state); + auto state_beta = beta_string (state); - // No Alpha + Double Beta - for(auto d_beta : doubles_beta) { - auto d_state = expand_bitset(d_beta) << (N / 2); - d_state = d_state | state_alpha_expand; - doubles.emplace_back(d_state); - } - - // Single Alpha + Single Beta - for(auto s_alpha : singles_alpha) - for(auto s_beta : singles_beta) { - auto d_state_alpha = expand_bitset(s_alpha); - auto d_state_beta = expand_bitset(s_beta) << (N / 2); - doubles.emplace_back(d_state_alpha | d_state_beta); - } -} - -template -void generate_singles_spin(size_t norb, std::bitset state, - std::vector>& singles) { - auto state_alpha = bitset_lo_word(state); - auto state_beta = bitset_hi_word(state); - - std::vector> singles_alpha, singles_beta; + using spin_wfn_type = spin_wfn_t; + std::vector singles_alpha, singles_beta; // Generate Spin-Specific singles / doubles generate_singles(norb, state_alpha, singles_alpha); generate_singles(norb, state_beta, singles_beta); - auto state_alpha_expand = expand_bitset(state_alpha); - auto state_beta_expand = expand_bitset(state_beta) << (N / 2); - // Generate Singles in full space singles.clear(); // Single Alpha + No Beta for(auto s_alpha : singles_alpha) { - auto s_state = expand_bitset(s_alpha); - s_state = s_state | state_beta_expand; - singles.emplace_back(s_state); + singles.emplace_back(from_spin(s_alpha, state_beta)); } // No Alpha + Single Beta for(auto s_beta : singles_beta) { - auto s_state = expand_bitset(s_beta) << (N / 2); - s_state = s_state | state_alpha_expand; - singles.emplace_back(s_state); + singles.emplace_back(from_spin(state_alpha, s_beta)); } } -template -void generate_singles_doubles_spin(size_t norb, std::bitset state, - std::vector>& singles, - std::vector>& doubles) { - auto state_alpha = bitset_lo_word(state); - auto state_beta = bitset_hi_word(state); +template +void generate_singles_doubles_spin(size_t norb, WfnType state, + WfnContainer& singles, WfnContainer& doubles) { + + auto state_alpha = alpha_string(state); + auto state_beta = beta_string (state); - std::vector> singles_alpha, singles_beta; - std::vector> doubles_alpha, doubles_beta; + using spin_wfn_type = spin_wfn_t; + std::vector singles_alpha, singles_beta; + std::vector doubles_alpha, doubles_beta; // Generate Spin-Specific singles / doubles generate_singles_doubles(norb, state_alpha, singles_alpha, doubles_alpha); generate_singles_doubles(norb, state_beta, singles_beta, doubles_beta); - auto state_alpha_expand = expand_bitset(state_alpha); - auto state_beta_expand = expand_bitset(state_beta) << (N / 2); // Generate Singles in full space singles.clear(); // Single Alpha + No Beta for(auto s_alpha : singles_alpha) { - auto s_state = expand_bitset(s_alpha); - s_state = s_state | state_beta_expand; - singles.emplace_back(s_state); + singles.emplace_back(from_spin(s_alpha, state_beta)); } // No Alpha + Single Beta for(auto s_beta : singles_beta) { - auto s_state = expand_bitset(s_beta) << (N / 2); - s_state = s_state | state_alpha_expand; - singles.emplace_back(s_state); + singles.emplace_back(from_spin(state_alpha, s_beta)); } // Generate Doubles in full space @@ -396,58 +245,49 @@ void generate_singles_doubles_spin(size_t norb, std::bitset state, // Double Alpha + No Beta for(auto d_alpha : doubles_alpha) { - auto d_state = expand_bitset(d_alpha); - d_state = d_state | state_beta_expand; - doubles.emplace_back(d_state); + doubles.emplace_back(from_spin(d_alpha, state_beta)); } // No Alpha + Double Beta for(auto d_beta : doubles_beta) { - auto d_state = expand_bitset(d_beta) << (N / 2); - d_state = d_state | state_alpha_expand; - doubles.emplace_back(d_state); + doubles.emplace_back(from_spin(state_alpha, d_beta)); } // Single Alpha + Single Beta for(auto s_alpha : singles_alpha) for(auto s_beta : singles_beta) { - auto d_state_alpha = expand_bitset(s_alpha); - auto d_state_beta = expand_bitset(s_beta) << (N / 2); - doubles.emplace_back(d_state_alpha | d_state_beta); + doubles.emplace_back(from_spin(s_alpha, s_beta)); } } -template -void generate_cisd_hilbert_space(size_t norb, std::bitset state, - std::vector>& dets) { +template +void generate_cisd_hilbert_space(size_t norb, WfnType state, WfnContainer& dets) { dets.clear(); dets.emplace_back(state); - std::vector> singles, doubles; + std::vector singles, doubles; generate_singles_doubles_spin(norb, state, singles, doubles); dets.insert(dets.end(), singles.begin(), singles.end()); dets.insert(dets.end(), doubles.begin(), doubles.end()); } -template -std::vector> generate_cisd_hilbert_space(size_t norb, - std::bitset state) { - std::vector> dets; +template +auto generate_cisd_hilbert_space(size_t norb, WfnType state) { + std::vector dets; generate_cisd_hilbert_space(norb, state, dets); return dets; } -template -std::vector> generate_combs(uint64_t nbits, uint64_t nset) { +template +std::vector generate_combs(uint64_t nbits, uint64_t nset) { std::vector v(nbits, false); std::fill_n(v.begin(), nset, true); - std::vector> store; + std::vector store; do { - std::bitset temp = 0ul; - std::bitset one = 1ul; + WfnType temp(0ul); for(uint64_t i = 0; i < nbits; ++i) if(v[i]) { - temp = temp | (one << i); + temp = create_no_check(temp, i); } store.emplace_back(temp); @@ -456,66 +296,44 @@ std::vector> generate_combs(uint64_t nbits, uint64_t nset) { return store; } -template -std::vector> generate_hilbert_space(size_t norbs, size_t nalpha, - size_t nbeta) { +template +std::vector generate_hilbert_space(size_t norbs, size_t nalpha, + size_t nbeta) { // Get all alpha and beta combs - auto alpha_dets = generate_combs(norbs, nalpha); - auto beta_dets = generate_combs(norbs, nbeta); + using spin_wfn_type = spin_wfn_t; + auto alpha_dets = generate_combs(norbs, nalpha); + auto beta_dets = generate_combs(norbs, nbeta); - std::vector> states; + std::vector states; states.reserve(alpha_dets.size() * beta_dets.size()); for(auto alpha_det : alpha_dets) for(auto beta_det : beta_dets) { - std::bitset state = alpha_det | (beta_det << (N / 2)); - states.emplace_back(state); + states.emplace_back(from_spin(alpha_det, beta_det)); } return states; } -template -void generate_cis_hilbert_space(size_t norb, std::bitset state, - std::vector>& dets) { +template +void generate_cis_hilbert_space(size_t norb, WfnType state, + WfnContainer& dets) { dets.clear(); dets.emplace_back(state); - std::vector> singles; + std::vector singles; generate_singles_spin(norb, state, singles); dets.insert(dets.end(), singles.begin(), singles.end()); } -template -std::vector> generate_cis_hilbert_space(size_t norb, - std::bitset state) { - std::vector> dets; +template +std::vector generate_cis_hilbert_space(size_t norb, WfnType state) { + std::vector dets; generate_cis_hilbert_space(norb, state, dets); return dets; } // TODO: Test this function -template -uint32_t first_occupied_flipped(std::bitset state, std::bitset ex) { - return ffs(state & ex) - 1u; -} - -// TODO: Test this function -template -double single_excitation_sign(std::bitset state, unsigned p, unsigned q) { - std::bitset mask = 0ul; - - if(p > q) { - mask = state & (full_mask(p) ^ full_mask(q + 1)); - } else { - mask = state & (full_mask(q) ^ full_mask(p + 1)); - } - return (mask.count() % 2) ? -1. : 1.; -} - -// TODO: Test this function -template -inline auto single_excitation_sign_indices(std::bitset bra, - std::bitset ket, - std::bitset ex) { +template +inline auto single_excitation_sign_indices(WfnType bra, WfnType ket, WfnType ex) { auto o1 = first_occupied_flipped(ket, ex); auto v1 = first_occupied_flipped(bra, ex); auto sign = single_excitation_sign(ket, v1, o1); @@ -524,15 +342,14 @@ inline auto single_excitation_sign_indices(std::bitset bra, } // TODO: Test this function -template -inline auto doubles_sign_indices(std::bitset bra, std::bitset ket, - std::bitset ex) { +template +inline auto doubles_sign_indices(WfnType bra, WfnType ket, WfnType ex) { const auto o1 = first_occupied_flipped(ket, ex); const auto v1 = first_occupied_flipped(bra, ex); auto sign = single_excitation_sign(ket, v1, o1); - ket.flip(o1).flip(v1); - ex.flip(o1).flip(v1); + ket = single_excitation(ket, o1, v1); + ex = single_excitation(ex, o1, v1); const auto o2 = first_occupied_flipped(ket, ex); const auto v2 = first_occupied_flipped(bra, ex); @@ -542,13 +359,13 @@ inline auto doubles_sign_indices(std::bitset bra, std::bitset ket, } // TODO: Test this function -template -inline auto doubles_sign(std::bitset bra, std::bitset ket, - std::bitset ex) { +template +inline auto doubles_sign(WfnType bra, WfnType ket, WfnType ex) { auto [p, q, r, s, sign] = doubles_sign_indices(bra, ket, ex); return sign; } +#if 0 // TODO: Test this function template void generate_residues(std::bitset state, std::vector>& res) { @@ -591,14 +408,14 @@ void generate_residues(std::bitset state, std::vector>& res) { res.emplace_back(state & ~mask); } } +#endif -template -std::string to_canonical_string(std::bitset state) { - static_assert((N % 2) == 0, "N Odd"); - auto state_alpha = bitset_lo_word(state); - auto state_beta = bitset_hi_word(state); +template +std::string to_canonical_string(WfnType state) { + auto state_alpha = alpha_string(state); + auto state_beta = beta_string (state); std::string str; - for(size_t i = 0; i < N / 2; ++i) { + for(size_t i = 0; i < state_alpha.size(); ++i) { if(state_alpha[i] and state_beta[i]) str.push_back('2'); else if(state_alpha[i]) @@ -611,20 +428,21 @@ std::string to_canonical_string(std::bitset state) { return str; } -template -std::bitset from_canonical_string(std::string str) { - std::bitset state_alpha(0), state_beta(0); - for(auto i = 0ul; i < str.length(); ++i) { +template +WfnType from_canonical_string(std::string str) { + using spin_wfn_type = spin_wfn_t; + spin_wfn_type state_alpha(0), state_beta(0); + for(auto i = 0ul; i < std::min(str.length(),state_alpha.size()); ++i) { if(str[i] == '2') { - state_alpha.set(i); - state_beta.set(i); + state_alpha = create_no_check(state_alpha, i); + state_beta = create_no_check(state_beta , i); } else if(str[i] == 'u') { - state_alpha.set(i); + state_alpha = create_no_check(state_alpha, i); } else if(str[i] == 'd') { - state_beta.set(i); + state_beta = create_no_check(state_beta, i); } } - auto state = state_alpha | (state_beta << (N / 2)); + auto state = from_spin(state_alpha, state_beta); return state; } diff --git a/include/macis/util/cas.hpp b/include/macis/util/cas.hpp index 63c8f4a2..34b85b19 100644 --- a/include/macis/util/cas.hpp +++ b/include/macis/util/cas.hpp @@ -49,7 +49,7 @@ double compute_casci_rdms( rank4_span(V, no, no, no, no)); // Compute Lowest Energy Eigenvalue (ED) - auto dets = generate_hilbert_space(norb.get(), nalpha, nbeta); + auto dets = generate_hilbert_space>(norb.get(), nalpha, nbeta); double E0 = selected_ci_diag(dets.begin(), dets.end(), ham_gen, settings.ci_matel_tol, settings.ci_max_subspace, settings.ci_res_tol, C, diff --git a/include/macis/util/unused_untested.hpp b/include/macis/util/unused_untested.hpp new file mode 100644 index 00000000..491ee17e --- /dev/null +++ b/include/macis/util/unused_untested.hpp @@ -0,0 +1,194 @@ + +#if 0 +/** + * @brief Generate canonical HF determinant. + * + * Generates a string representation of the canonical HF determinant + * consisting of a specifed number of alpha and beta orbitals. This variant + * does not assume energetic ordering of the HF orbitals. + * + * TODO: This assumes restricted orbitals + * + * @tparam N Number of bits for the total bit string of the state + * @param[in] nalpha Number of occupied alpha orbitals in the HF state + * @param[in] nbeta Number of occupied beta orbitals in the HF state + * @param[in] orb_ens Orbital eigenenergies. + * + * @returns The bitstring HF state consisting of the specified number of + * occupied orbitals populated according to the ordering of `orb_ens`. + */ +template +std::bitset canonical_hf_determinant(uint32_t nalpha, uint32_t nbeta, + const std::vector& orb_ens) { + static_assert((N % 2) == 0, "N Must Be Even"); + // First, find the sorted indices for the orbital energies + std::vector idx(orb_ens.size()); + std::iota(idx.begin(), idx.end(), 0); + std::stable_sort(idx.begin(), idx.end(), [&orb_ens](size_t i1, size_t i2) { + return orb_ens[i1] < orb_ens[i2]; + }); + // Next, fill the electrons by energy + std::bitset alpha(0), beta(0); + for(uint32_t i = 0; i < nalpha; i++) alpha.flip(idx[i]); + for(uint32_t i = 0; i < nbeta; i++) beta.flip(idx[i] + N / 2); + return alpha | beta; +} + +/** + * @brief Generate the list of (un)occupied orbitals for a paricular state. + * + * TODO: Test this function + * + * @tparam N Number of bits for the total bit string of the state + * @param[in] norb Number of orbitals used to describe the state (<= `N`) + * @param[in] state The state from which to determine orbital occupations. + * @param[out] occ List of occupied orbitals in `state` + * @param[out] vir List of unoccupied orbitals in `state` + * @param[in] as_orbs TODO:???? + */ +template +void bitset_to_occ_vir_as(size_t norb, std::bitset state, + std::vector& occ, + std::vector& vir, + const std::vector& as_orbs) { + occ.clear(); + for(const auto i : as_orbs) + if(state[i]) occ.emplace_back(i); + const auto nocc = occ.size(); + assert(nocc <= norb); + + const auto nvir = as_orbs.size() - nocc; + vir.resize(nvir); + auto it = vir.begin(); + for(const auto i : as_orbs) + if(!state[i]) *(it++) = i; +} + + + +// TODO: Test this function +template +void generate_singles_as(size_t norb, std::bitset state, + std::vector>& singles, + const std::vector& as_orbs) { + std::vector occ_orbs, vir_orbs; + bitset_to_occ_vir_as(norb, state, occ_orbs, vir_orbs, as_orbs); + + singles.clear(); + append_singles(state, occ_orbs, vir_orbs, singles); +} + +// TODO: Test this function +template +void generate_singles_doubles_as(size_t norb, std::bitset state, + std::vector>& singles, + std::vector>& doubles, + const std::vector& as_orbs) { + std::vector occ_orbs, vir_orbs; + bitset_to_occ_vir_as(norb, state, occ_orbs, vir_orbs, as_orbs); + + singles.clear(); + doubles.clear(); + append_singles(state, occ_orbs, vir_orbs, singles); + append_doubles(state, occ_orbs, vir_orbs, doubles); +} + +// TODO: Test this function +template +void generate_singles_spin_as(size_t norb, std::bitset state, + std::vector>& singles, + const std::vector as_orbs) { + auto state_alpha = bitset_lo_word(state); + auto state_beta = bitset_hi_word(state); + + std::vector> singles_alpha, singles_beta; + + // Generate Spin-Specific singles + generate_singles_as(norb, state_alpha, singles_alpha, as_orbs); + generate_singles_as(norb, state_beta, singles_beta, as_orbs); + + auto state_alpha_expand = expand_bitset(state_alpha); + auto state_beta_expand = expand_bitset(state_beta) << (N / 2); + + // Generate Singles in full space + singles.clear(); + + // Single Alpha + No Beta + for(auto s_alpha : singles_alpha) { + auto s_state = expand_bitset(s_alpha); + s_state = s_state | state_beta_expand; + singles.emplace_back(s_state); + } + + // No Alpha + Single Beta + for(auto s_beta : singles_beta) { + auto s_state = expand_bitset(s_beta) << (N / 2); + s_state = s_state | state_alpha_expand; + singles.emplace_back(s_state); + } +} + +// TODO: Test this function +template +void generate_singles_doubles_spin_as(size_t norb, std::bitset state, + std::vector>& singles, + std::vector>& doubles, + const std::vector& as_orbs) { + auto state_alpha = bitset_lo_word(state); + auto state_beta = bitset_hi_word(state); + + std::vector> singles_alpha, singles_beta; + std::vector> doubles_alpha, doubles_beta; + + // Generate Spin-Specific singles / doubles + generate_singles_doubles_as(norb, state_alpha, singles_alpha, doubles_alpha, + as_orbs); + generate_singles_doubles_as(norb, state_beta, singles_beta, doubles_beta, + as_orbs); + + auto state_alpha_expand = expand_bitset(state_alpha); + auto state_beta_expand = expand_bitset(state_beta) << (N / 2); + + // Generate Singles in full space + singles.clear(); + + // Single Alpha + No Beta + for(auto s_alpha : singles_alpha) { + auto s_state = expand_bitset(s_alpha); + s_state = s_state | state_beta_expand; + singles.emplace_back(s_state); + } + + // No Alpha + Single Beta + for(auto s_beta : singles_beta) { + auto s_state = expand_bitset(s_beta) << (N / 2); + s_state = s_state | state_alpha_expand; + singles.emplace_back(s_state); + } + + // Generate Doubles in full space + doubles.clear(); + + // Double Alpha + No Beta + for(auto d_alpha : doubles_alpha) { + auto d_state = expand_bitset(d_alpha); + d_state = d_state | state_beta_expand; + doubles.emplace_back(d_state); + } + + // No Alpha + Double Beta + for(auto d_beta : doubles_beta) { + auto d_state = expand_bitset(d_beta) << (N / 2); + d_state = d_state | state_alpha_expand; + doubles.emplace_back(d_state); + } + + // Single Alpha + Single Beta + for(auto s_alpha : singles_alpha) + for(auto s_beta : singles_beta) { + auto d_state_alpha = expand_bitset(s_alpha); + auto d_state_beta = expand_bitset(s_beta) << (N / 2); + doubles.emplace_back(d_state_alpha | d_state_beta); + } +} +#endif diff --git a/include/macis/wavefunction_io.hpp b/include/macis/wavefunction_io.hpp index bc38f7ee..1483d864 100644 --- a/include/macis/wavefunction_io.hpp +++ b/include/macis/wavefunction_io.hpp @@ -67,7 +67,7 @@ void read_wavefunction(std::string fname, std::vector>& states, std::stringstream ss{line}; std::string c, d; ss >> c >> d; - states.emplace_back(from_canonical_string(d)); + states.emplace_back(from_canonical_string>(d)); coeffs.emplace_back(std::stod(c)); } } diff --git a/tests/sd_operations.cxx b/tests/sd_operations.cxx index dd4612a6..3635eff2 100644 --- a/tests/sd_operations.cxx +++ b/tests/sd_operations.cxx @@ -20,16 +20,18 @@ TEST_CASE("Slater Det Operations") { REQUIRE(hf == 0x0003000F); } +#if 0 SECTION("Unordered") { std::vector orb_energies = {3, 2, 7, 8, 5}; auto hf = macis::canonical_hf_determinant<32>(3, 2, orb_energies); REQUIRE(hf == 0x00030013); } +#endif } SECTION("Occupied / Unoccupied Conversion") { SECTION("Default") { - std::bitset<64> state = 0x00000000000000AF; + macis::wfn_t<64> state = 0x00000000000000AF; std::vector ref_occ = {0, 1, 2, 3, 5, 7}; std::vector ref_vir = {4, 6, 8, 9, 10, 11}; @@ -45,13 +47,13 @@ TEST_CASE("Slater Det Operations") { SECTION("Singles") { SECTION("Single Spin") { - std::vector> ref_singles = { + std::vector> ref_singles = { 0b00011110, 0b00101110, 0b01001110, 0b10001110, 0b00011101, 0b00101101, 0b01001101, 0b10001101, 0b00011011, 0b00101011, 0b01001011, 0b10001011, 0b00010111, 0b00100111, 0b01000111, 0b10000111}; - std::vector> singles; + std::vector> singles; auto state = macis::canonical_hf_determinant<64>(4, 0); // all alpha macis::generate_singles(8, state, singles); @@ -63,7 +65,7 @@ TEST_CASE("Slater Det Operations") { } SECTION("Both Spin") { - std::vector> ref_singles = { + std::vector> ref_singles = { 0x0F0000001E, 0x0F0000001D, 0x0F0000001B, 0x0F00000017, 0x0F0000002E, 0x0F0000002D, 0x0F0000002B, 0x0F00000027, 0x0F0000004E, 0x0F0000004D, 0x0F0000004B, 0x0F00000047, 0x0F0000008E, 0x0F0000008D, 0x0F0000008B, @@ -73,7 +75,7 @@ TEST_CASE("Slater Det Operations") { 0x8B0000000f, 0x870000000f}; auto state = macis::canonical_hf_determinant<64>(4, 4); - std::vector> singles; + std::vector> singles; macis::generate_singles_spin(8, state, singles); auto cmp = macis::bitset_less_comparator<64>{}; @@ -86,7 +88,7 @@ TEST_CASE("Slater Det Operations") { SECTION("Doubles") { SECTION("Single Spin") { - std::vector> ref_doubles = { + std::vector> ref_doubles = { 0b00111100, 0b01011100, 0b10011100, 0b01101100, 0b10101100, 0b11001100, 0b00111010, 0b01011010, 0b10011010, 0b01101010, 0b10101010, 0b11001010, 0b00111001, 0b01011001, 0b10011001, @@ -96,7 +98,7 @@ TEST_CASE("Slater Det Operations") { 0b00110011, 0b01010011, 0b10010011, 0b01100011, 0b10100011, 0b11000011}; - std::vector> doubles; + std::vector> doubles; auto state = macis::canonical_hf_determinant<64>(4, 0); // all alpha macis::generate_doubles(8, state, doubles); @@ -108,7 +110,7 @@ TEST_CASE("Slater Det Operations") { } SECTION("Both Spins") { - std::vector> ref_doubles = { + std::vector> ref_doubles = { 0x0F0000003C, 0x0F0000003A, 0x0F00000036, 0x0F0000005C, 0x0F0000005A, 0x0F00000056, 0x0F0000009C, 0x0F0000009A, 0x0F00000096, 0x0F00000039, 0x0F00000035, 0x0F00000059, 0x0F00000055, 0x0F00000099, 0x0F00000095, @@ -176,7 +178,7 @@ TEST_CASE("Slater Det Operations") { 0x4E00000087, 0x4D00000087, 0x4B00000087, 0x4700000087, 0x8E00000087, 0x8D00000087, 0x8B00000087, 0x8700000087}; auto state = macis::canonical_hf_determinant<64>(4, 4); - std::vector> singles, doubles; + std::vector> singles, doubles; macis::generate_singles_doubles_spin(8, state, singles, doubles); auto cmp = macis::bitset_less_comparator<64>{}; @@ -189,7 +191,7 @@ TEST_CASE("Slater Det Operations") { SECTION("CIS") { auto state = macis::canonical_hf_determinant<64>(4, 4); - std::vector> singles; + std::vector> singles; macis::generate_singles_spin(8, state, singles); singles.push_back(state); auto cis = macis::generate_cis_hilbert_space(8, state); @@ -202,7 +204,7 @@ TEST_CASE("Slater Det Operations") { SECTION("CISD") { auto state = macis::canonical_hf_determinant<64>(4, 4); - std::vector> singles, doubles; + std::vector> singles, doubles; macis::generate_singles_doubles_spin(8, state, singles, doubles); singles.insert(singles.end(), doubles.begin(), doubles.end()); singles.push_back(state); @@ -216,13 +218,13 @@ TEST_CASE("Slater Det Operations") { SECTION("FCI") { SECTION("Single Spin") { - std::vector> ref_combs = {0x3, 0x5, 0x9, 0x6, 0xA, 0xC}; - auto combs = macis::generate_combs<64>(4, 2); + std::vector> ref_combs = {0x3, 0x5, 0x9, 0x6, 0xA, 0xC}; + auto combs = macis::generate_combs>(4, 2); REQUIRE(combs == ref_combs); } SECTION("Both Spins") { - std::vector> ref_dets = { + std::vector> ref_dets = { 0x300000003, 0x500000003, 0x900000003, 0x600000003, 0xA00000003, 0xC00000003, 0x300000005, 0x500000005, 0x900000005, 0x600000005, 0xA00000005, 0xC00000005, 0x300000009, 0x500000009, 0x900000009, @@ -232,7 +234,7 @@ TEST_CASE("Slater Det Operations") { 0x30000000C, 0x50000000C, 0x90000000C, 0x60000000C, 0xA0000000C, 0xC0000000C}; - auto dets = macis::generate_hilbert_space<64>(4, 2, 2); + auto dets = macis::generate_hilbert_space>(4, 2, 2); REQUIRE(dets == ref_dets); } } @@ -248,13 +250,13 @@ TEST_CASE("Slater Det Operations") { SECTION("From String") { SECTION("Full String") { std::string str = "220ud000000000000000000000000000"; - auto det = macis::from_canonical_string<64>(str); + auto det = macis::from_canonical_string>(str); REQUIRE(det == state); } SECTION("Short String") { std::string str = "220ud"; - auto det = macis::from_canonical_string<64>(str); + auto det = macis::from_canonical_string>(str); REQUIRE(det == state); } } diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index 8ce5cfe8..495e726d 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -63,6 +63,7 @@ int main(int argc, char** argv) { spdlog::set_pattern("[%n] %v"); constexpr size_t nwfn_bits = 64; + using wfn_type = macis::wfn_t; MACIS_MPI_CODE(MPI_Init(&argc, &argv);) @@ -300,7 +301,7 @@ int main(int argc, char** argv) { : spdlog::stdout_color_mt("determinants"); det_logger->info("Print leading determinants > {:.12f}", determinants_threshold); - auto dets = macis::generate_hilbert_space( + auto dets = macis::generate_hilbert_space( n_active, nalpha, nbeta); for(size_t i = 0; i < dets.size(); ++i) { if(std::abs(C_local[i]) > determinants_threshold) { @@ -317,7 +318,7 @@ int main(int argc, char** argv) { macis::rank4_span(V_active.data(), n_active, n_active, n_active, n_active)); - std::vector> dets; + std::vector dets; std::vector C; if(asci_wfn_fname.size()) { // Read wave function from standard file From 5e0ab33d6c79ad678f472406890674a0941e059c Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Thu, 7 Sep 2023 11:17:38 -0700 Subject: [PATCH 12/73] Generic Hamiltonian Generator --- .../macis/asci/determinant_contributions.hpp | 6 ++-- include/macis/asci/determinant_search.hpp | 8 ++--- include/macis/asci/grow.hpp | 4 +-- include/macis/asci/iteration.hpp | 4 +-- include/macis/asci/mask_constraints.hpp | 6 ++-- include/macis/asci/pt2.hpp | 4 +-- include/macis/asci/refine.hpp | 2 +- include/macis/csr_hamiltonian.hpp | 25 +++++++-------- include/macis/hamiltonian_generator.hpp | 16 ++++------ .../hamiltonian_generator/double_loop.hpp | 32 +++++++++---------- .../hamiltonian_generator/fast_diagonals.hpp | 32 +++++++++---------- include/macis/hamiltonian_generator/impl.hpp | 8 ++--- .../hamiltonian_generator/matrix_elements.hpp | 32 +++++++++---------- include/macis/hamiltonian_generator/rdms.hpp | 4 +-- include/macis/solvers/selected_ci_diag.hpp | 7 ++-- include/macis/util/cas.hpp | 6 ++-- src/macis/casscf.cxx | 2 +- tests/asci.cxx | 2 +- tests/csr_hamiltonian.cxx | 4 +-- tests/davidson.cxx | 4 +-- tests/double_loop.cxx | 4 +-- tests/standalone_driver.cxx | 2 +- 22 files changed, 104 insertions(+), 110 deletions(-) diff --git a/include/macis/asci/determinant_contributions.hpp b/include/macis/asci/determinant_contributions.hpp index 041979bb..1db2b827 100644 --- a/include/macis/asci/determinant_contributions.hpp +++ b/include/macis/asci/determinant_contributions.hpp @@ -33,7 +33,7 @@ void append_singles_asci_contributions( const std::vector& occ_othr, const double* eps_same, const double* T_pq, const size_t LDT, const double* G_kpq, const size_t LDG, const double* V_kpq, const size_t LDV, double h_el_tol, double root_diag, - double E0, HamiltonianGenerator<2 * N>& ham_gen, + double E0, HamiltonianGenerator>& ham_gen, asci_contrib_container>& asci_contributions) { const auto LDG2 = LDG * LDG; const auto LDV2 = LDV * LDV; @@ -74,7 +74,7 @@ void append_ss_doubles_asci_contributions( const std::vector& ss_occ, const std::vector& vir, const std::vector& os_occ, const double* eps_same, const double* G, size_t LDG, double h_el_tol, double root_diag, double E0, - HamiltonianGenerator<2 * N>& ham_gen, + HamiltonianGenerator>& ham_gen, asci_contrib_container>& asci_contributions) { const size_t nocc = ss_occ.size(); const size_t nvir = vir.size(); @@ -130,7 +130,7 @@ void append_os_doubles_asci_contributions( const std::vector& vir_alpha, const std::vector& vir_beta, const double* eps_alpha, const double* eps_beta, const double* V, size_t LDV, double h_el_tol, - double root_diag, double E0, HamiltonianGenerator<2 * N>& ham_gen, + double root_diag, double E0, HamiltonianGenerator>& ham_gen, asci_contrib_container>& asci_contributions) { const size_t LDV2 = LDV * LDV; for(auto i : occ_alpha) diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index 03cc9b9d..8582b832 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -56,7 +56,7 @@ asci_contrib_container> asci_contributions_standard( wavefunction_iterator_t cdets_end, const double E_ASCI, const std::vector& C, size_t norb, const double* T_pq, const double* G_red, const double* V_red, const double* G_pqrs, - const double* V_pqrs, HamiltonianGenerator& ham_gen) { + const double* V_pqrs, HamiltonianGenerator>& ham_gen) { auto logger = spdlog::get("asci_search"); const size_t ncdets = std::distance(cdets_begin, cdets_end); @@ -147,7 +147,7 @@ asci_contrib_container> asci_contributions_constraint( wavefunction_iterator_t cdets_end, const double E_ASCI, const std::vector& C, size_t norb, const double* T_pq, const double* G_red, const double* V_red, const double* G_pqrs, - const double* V_pqrs, HamiltonianGenerator& ham_gen, MPI_Comm comm) { + const double* V_pqrs, HamiltonianGenerator>& ham_gen, MPI_Comm comm) { using clock_type = std::chrono::high_resolution_clock; using duration_type = std::chrono::duration; @@ -183,7 +183,7 @@ asci_contrib_container> asci_contributions_constraint( beta_coeff_data(double c, size_t norb, const std::vector& occ_alpha, wfn_t w, - const HamiltonianGenerator& ham_gen) { + const HamiltonianGenerator>& ham_gen) { coeff = c; // Compute Beta string @@ -399,7 +399,7 @@ std::vector> asci_search( const std::vector& C, size_t norb, const double* T_pq, const double* G_red, const double* V_red, const double* G_pqrs, const double* V_pqrs, - HamiltonianGenerator& ham_gen MACIS_MPI_CODE(, MPI_Comm comm)) { + HamiltonianGenerator>& ham_gen MACIS_MPI_CODE(, MPI_Comm comm)) { using clock_type = std::chrono::high_resolution_clock; using duration_type = std::chrono::duration; diff --git a/include/macis/asci/grow.hpp b/include/macis/asci/grow.hpp index f3f4260e..bf6dd471 100644 --- a/include/macis/asci/grow.hpp +++ b/include/macis/asci/grow.hpp @@ -16,7 +16,7 @@ namespace macis { template auto asci_grow(ASCISettings asci_settings, MCSCFSettings mcscf_settings, double E0, std::vector> wfn, std::vector X, - HamiltonianGenerator& ham_gen, + HamiltonianGenerator>& ham_gen, size_t norb MACIS_MPI_CODE(, MPI_Comm comm)) { #ifdef MACIS_ENABLE_MPI auto world_rank = comm_rank(comm); @@ -124,7 +124,7 @@ auto asci_grow(ASCISettings asci_settings, MCSCFSettings mcscf_settings, logger->trace(" * Rediagonalizing"); auto rdg_st = hrt_t::now(); std::vector X_local; - selected_ci_diag( + selected_ci_diag( wfn.begin(), wfn.end(), ham_gen, mcscf_settings.ci_matel_tol, mcscf_settings.ci_max_subspace, mcscf_settings.ci_res_tol, X_local MACIS_MPI_CODE(, comm)); diff --git a/include/macis/asci/iteration.hpp b/include/macis/asci/iteration.hpp index aa6e271c..8db17efc 100644 --- a/include/macis/asci/iteration.hpp +++ b/include/macis/asci/iteration.hpp @@ -16,7 +16,7 @@ namespace macis { template auto asci_iter(ASCISettings asci_settings, MCSCFSettings mcscf_settings, size_t ndets_max, double E0, std::vector> wfn, - std::vector X, HamiltonianGenerator& ham_gen, + std::vector X, HamiltonianGenerator>& ham_gen, size_t norb MACIS_MPI_CODE(, MPI_Comm comm)) { // Sort wfn on coefficient weights if(wfn.size() > 1) reorder_ci_on_coeff(wfn, X); @@ -31,7 +31,7 @@ auto asci_iter(ASCISettings asci_settings, MCSCFSettings mcscf_settings, // Rediagonalize std::vector X_local; // Precludes guess reuse - auto E = selected_ci_diag( + auto E = selected_ci_diag( wfn.begin(), wfn.end(), ham_gen, mcscf_settings.ci_matel_tol, mcscf_settings.ci_max_subspace, mcscf_settings.ci_res_tol, X_local MACIS_MPI_CODE(, comm)); diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index 5430b00b..50472f62 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -247,7 +247,7 @@ void generate_constraint_singles_contributions_ss( const std::vector& occ_othr, const double* eps, const double* T_pq, const size_t LDT, const double* G_kpq, const size_t LDG, const double* V_kpq, const size_t LDV, double h_el_tol, double root_diag, - double E0, HamiltonianGenerator& ham_gen, + double E0, HamiltonianGenerator>& ham_gen, asci_contrib_container>& asci_contributions) { auto [o, v] = generate_constraint_single_excitations(det, T, O, B); const auto no = o.count(); @@ -296,7 +296,7 @@ void generate_constraint_doubles_contributions_ss( wfn_t os_det, const std::vector& occ_same, const std::vector& occ_othr, const double* eps, const double* G, const size_t LDG, double h_el_tol, double root_diag, double E0, - HamiltonianGenerator& ham_gen, + HamiltonianGenerator>& ham_gen, asci_contrib_container>& asci_contributions) { auto [O, V] = generate_constraint_double_excitations(det, T, O_mask, B); const auto no_pairs = O.size(); @@ -350,7 +350,7 @@ void generate_constraint_doubles_contributions_os( const std::vector& occ_othr, const std::vector& vir_othr, const double* eps_same, const double* eps_othr, const double* V, const size_t LDV, double h_el_tol, - double root_diag, double E0, HamiltonianGenerator& ham_gen, + double root_diag, double E0, HamiltonianGenerator>& ham_gen, asci_contrib_container>& asci_contributions) { // Generate Single Excitations that Satisfy the Constraint auto [o, v] = generate_constraint_single_excitations(det, T, O, B); diff --git a/include/macis/asci/pt2.hpp b/include/macis/asci/pt2.hpp index 07560ed0..2ddd927a 100644 --- a/include/macis/asci/pt2.hpp +++ b/include/macis/asci/pt2.hpp @@ -18,7 +18,7 @@ double asci_pt2_constraint( wavefunction_iterator_t cdets_begin, wavefunction_iterator_t cdets_end, const double E_ASCI, const std::vector& C, size_t norb, const double* T_pq, const double* G_red, const double* V_red, - const double* G_pqrs, const double* V_pqrs, HamiltonianGenerator& ham_gen, + const double* G_pqrs, const double* V_pqrs, HamiltonianGenerator>& ham_gen, MPI_Comm comm) { using clock_type = std::chrono::high_resolution_clock; @@ -57,7 +57,7 @@ double asci_pt2_constraint( beta_coeff_data(double c, size_t norb, const std::vector& occ_alpha, wfn_t w, - const HamiltonianGenerator& ham_gen) { + const HamiltonianGenerator>& ham_gen) { coeff = c; // Compute Beta string diff --git a/include/macis/asci/refine.hpp b/include/macis/asci/refine.hpp index 4a1f53e6..34701c5b 100644 --- a/include/macis/asci/refine.hpp +++ b/include/macis/asci/refine.hpp @@ -14,7 +14,7 @@ namespace macis { template auto asci_refine(ASCISettings asci_settings, MCSCFSettings mcscf_settings, double E0, std::vector> wfn, std::vector X, - HamiltonianGenerator& ham_gen, + HamiltonianGenerator>& ham_gen, size_t norb MACIS_MPI_CODE(, MPI_Comm comm)) { auto logger = spdlog::get("asci_refine"); #ifdef MACIS_ENABLE_MPI diff --git a/include/macis/csr_hamiltonian.hpp b/include/macis/csr_hamiltonian.hpp index 2a9dc24b..903ed1ac 100644 --- a/include/macis/csr_hamiltonian.hpp +++ b/include/macis/csr_hamiltonian.hpp @@ -18,12 +18,12 @@ #include namespace macis { -// Base implementation of bitset CSR generation -template +// Base implementation of CSR hamiltonian generation +template sparsexx::csr_matrix make_csr_hamiltonian_block( - wavefunction_iterator_t bra_begin, wavefunction_iterator_t bra_end, - wavefunction_iterator_t ket_begin, wavefunction_iterator_t ket_end, - HamiltonianGenerator& ham_gen, double H_thresh) { + WfnIterator bra_begin, WfnIterator bra_end, + WfnIterator ket_begin, WfnIterator ket_end, + HamiltonianGenerator& ham_gen, double H_thresh) { size_t nbra = std::distance(bra_begin, bra_end); size_t nket = std::distance(ket_begin, ket_end); @@ -35,21 +35,20 @@ sparsexx::csr_matrix make_csr_hamiltonian_block( } } -template +template sparsexx::csr_matrix make_csr_hamiltonian( - wavefunction_iterator_t sd_begin, wavefunction_iterator_t sd_end, - HamiltonianGenerator& ham_gen, double H_thresh) { + WfnIterator sd_begin, WfnIterator sd_end, + HamiltonianGenerator& ham_gen, double H_thresh) { return make_csr_hamiltonian_block(sd_begin, sd_end, sd_begin, sd_end, ham_gen, H_thresh); } #ifdef MACIS_ENABLE_MPI // Base implementation of dist-CSR H construction for bitsets -template +template sparsexx::dist_sparse_matrix> -make_dist_csr_hamiltonian(MPI_Comm comm, wavefunction_iterator_t sd_begin, - wavefunction_iterator_t sd_end, - HamiltonianGenerator& ham_gen, +make_dist_csr_hamiltonian(MPI_Comm comm, WfnIterator sd_begin, WfnIterator sd_end, + HamiltonianGenerator& ham_gen, const double H_thresh) { using namespace sparsexx; using namespace sparsexx::detail; @@ -69,7 +68,7 @@ make_dist_csr_hamiltonian(MPI_Comm comm, wavefunction_iterator_t sd_begin, if(world_size > 1) { // Create a copy of SD's with local bra dets zero'd out - std::vector> sds_offdiag(sd_begin, sd_end); + std::vector sds_offdiag(sd_begin, sd_end); for(auto i = bra_st; i < bra_en; ++i) sds_offdiag[i] = 0ul; // Build off-diagonal part diff --git a/include/macis/hamiltonian_generator.hpp b/include/macis/hamiltonian_generator.hpp index 9ef9583b..ea4c9758 100644 --- a/include/macis/hamiltonian_generator.hpp +++ b/include/macis/hamiltonian_generator.hpp @@ -7,35 +7,31 @@ */ #pragma once -#include #include #include #include namespace macis { -template +template class HamiltonianGenerator { - static_assert(N % 2 == 0, "N Must Be Even"); public: - constexpr static size_t nbits = N; - using full_det_t = std::bitset; - using spin_det_t = std::bitset; + using full_det_t = WfnType; + using spin_det_t = spin_wfn_t; template using sparse_matrix_type = sparsexx::csr_matrix; - using full_det_iterator = wavefunction_iterator_t; + using full_det_container = std::vector; + using full_det_iterator = typename full_det_container::iterator; using matrix_span_t = matrix_span; using rank3_span_t = rank3_span; using rank4_span_t = rank4_span; public: - inline spin_det_t alpha_string(full_det_t str) { return bitset_lo_word(str); } - inline spin_det_t beta_string(full_det_t str) { return bitset_hi_word(str); } size_t norb_; size_t norb2_; @@ -184,7 +180,7 @@ class HamiltonianGenerator { virtual void SetJustSingles(bool /*_js*/) {} virtual bool GetJustSingles() { return false; } - virtual size_t GetNimp() const { return N / 2; } + //virtual size_t GetNimp() const { return N / 2; } }; } // namespace macis diff --git a/include/macis/hamiltonian_generator/double_loop.hpp b/include/macis/hamiltonian_generator/double_loop.hpp index 5628a5e6..7f00f053 100644 --- a/include/macis/hamiltonian_generator/double_loop.hpp +++ b/include/macis/hamiltonian_generator/double_loop.hpp @@ -13,10 +13,10 @@ namespace macis { -template -class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { +template +class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { public: - using base_type = HamiltonianGenerator; + using base_type = HamiltonianGenerator; using full_det_t = typename base_type::full_det_t; using spin_det_t = typename base_type::spin_det_t; using full_det_iterator = typename base_type::full_det_iterator; @@ -49,8 +49,8 @@ class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { size_t nrow = 0; if(bra.count()) { // Separate out into alpha/beta components - spin_det_t bra_alpha = bitset_lo_word(bra); - spin_det_t bra_beta = bitset_hi_word(bra); + spin_det_t bra_alpha = alpha_string(bra); + spin_det_t bra_beta = beta_string(bra); // Get occupied indices bits_to_indices(bra_alpha, bra_occ_alpha); @@ -60,13 +60,13 @@ class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { for(size_t j = 0; j < nket_dets; ++j) { const auto ket = *(ket_begin + j); if(ket.count()) { - spin_det_t ket_alpha = bitset_lo_word(ket); - spin_det_t ket_beta = bitset_hi_word(ket); + spin_det_t ket_alpha = alpha_string(ket); + spin_det_t ket_beta = beta_string(ket); full_det_t ex_total = bra ^ ket; if(ex_total.count() <= 4) { - spin_det_t ex_alpha = bitset_lo_word(ex_total); - spin_det_t ex_beta = bitset_hi_word(ex_total); + spin_det_t ex_alpha = alpha_string(ex_total); + spin_det_t ex_beta = beta_string(ex_total); // Compute Matrix Element const auto h_el = this->matrix_element( @@ -128,8 +128,8 @@ class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { // if( (i%1000) == 0 ) std::cout << i << std::endl; if(bra.count()) { // Separate out into alpha/beta components - spin_det_t bra_alpha = bitset_lo_word(bra); - spin_det_t bra_beta = bitset_hi_word(bra); + spin_det_t bra_alpha = alpha_string(bra); + spin_det_t bra_beta = beta_string(bra); // Get occupied indices bits_to_indices(bra_alpha, bra_occ_alpha); @@ -139,13 +139,13 @@ class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { for(size_t j = 0; j < nket_dets; ++j) { const auto ket = *(ket_begin + j); if(ket.count()) { - spin_det_t ket_alpha = bitset_lo_word(ket); - spin_det_t ket_beta = bitset_hi_word(ket); + spin_det_t ket_alpha = alpha_string(ket); + spin_det_t ket_beta = beta_string(ket); full_det_t ex_total = bra ^ ket; if(ex_total.count() <= 4) { - spin_det_t ex_alpha = bitset_lo_word(ex_total); - spin_det_t ex_beta = bitset_hi_word(ex_total); + spin_det_t ex_alpha = alpha_string(ex_total); + spin_det_t ex_beta = beta_string(ex_total); const double val = C[i] * C[j]; @@ -167,7 +167,7 @@ class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { public: template DoubleLoopHamiltonianGenerator(Args &&...args) - : HamiltonianGenerator(std::forward(args)...) {} + : HamiltonianGenerator(std::forward(args)...) {} }; } // namespace macis diff --git a/include/macis/hamiltonian_generator/fast_diagonals.hpp b/include/macis/hamiltonian_generator/fast_diagonals.hpp index 52cab806..e561ea7c 100644 --- a/include/macis/hamiltonian_generator/fast_diagonals.hpp +++ b/include/macis/hamiltonian_generator/fast_diagonals.hpp @@ -11,8 +11,8 @@ namespace macis { -template -double HamiltonianGenerator::single_orbital_en( +template +double HamiltonianGenerator::single_orbital_en( uint32_t orb, const std::vector& ss_occ, const std::vector& os_occ) const { // One electron component @@ -28,8 +28,8 @@ double HamiltonianGenerator::single_orbital_en( return orb_en; } -template -std::vector HamiltonianGenerator::single_orbital_ens( +template +std::vector HamiltonianGenerator::single_orbital_ens( size_t norb, const std::vector& ss_occ, const std::vector& os_occ) const { std::vector ens(norb); @@ -50,8 +50,8 @@ std::vector HamiltonianGenerator::single_orbital_ens( return ens; } -template -double HamiltonianGenerator::fast_diag_single( +template +double HamiltonianGenerator::fast_diag_single( // These refer to original determinant double hol_en, double par_en, uint32_t orb_hol, uint32_t orb_par, double orig_det_Hii) const { @@ -59,8 +59,8 @@ double HamiltonianGenerator::fast_diag_single( G2_red_(orb_hol, orb_par); } -template -double HamiltonianGenerator::fast_diag_single( +template +double HamiltonianGenerator::fast_diag_single( // These refer to original determinant const std::vector& ss_occ, const std::vector& os_occ, uint32_t orb_hol, uint32_t orb_par, double orig_det_Hii) const { @@ -69,8 +69,8 @@ double HamiltonianGenerator::fast_diag_single( return fast_diag_single(hol_en, par_en, orb_hol, orb_par, orig_det_Hii); } -template -double HamiltonianGenerator::fast_diag_ss_double( +template +double HamiltonianGenerator::fast_diag_ss_double( // These refer to original determinant double hol1_en, double hol2_en, double par1_en, double par2_en, uint32_t orb_hol1, uint32_t orb_hol2, uint32_t orb_par1, uint32_t orb_par2, @@ -84,8 +84,8 @@ double HamiltonianGenerator::fast_diag_ss_double( G2_red_(orb_par2, orb_hol2) - G2_red_(orb_hol2, orb_par2); } -template -double HamiltonianGenerator::fast_diag_ss_double( +template +double HamiltonianGenerator::fast_diag_ss_double( // These refer to original determinant const std::vector& ss_occ, const std::vector& os_occ, uint32_t orb_hol1, uint32_t orb_hol2, uint32_t orb_par1, uint32_t orb_par2, @@ -98,8 +98,8 @@ double HamiltonianGenerator::fast_diag_ss_double( orb_hol2, orb_par1, orb_par2, orig_det_Hii); } -template -double HamiltonianGenerator::fast_diag_os_double( +template +double HamiltonianGenerator::fast_diag_os_double( // These refer to original determinant double en_holu, double en_hold, double en_paru, double en_pard, uint32_t orb_holu, uint32_t orb_hold, uint32_t orb_paru, uint32_t orb_pard, @@ -111,8 +111,8 @@ double HamiltonianGenerator::fast_diag_os_double( V2_red_(orb_paru, orb_hold) - V2_red_(orb_holu, orb_pard); } -template -double HamiltonianGenerator::fast_diag_os_double( +template +double HamiltonianGenerator::fast_diag_os_double( // These refer to original determinant const std::vector& ss_occ, const std::vector& os_occ, uint32_t orb_holu, uint32_t orb_hold, uint32_t orb_paru, uint32_t orb_pard, diff --git a/include/macis/hamiltonian_generator/impl.hpp b/include/macis/hamiltonian_generator/impl.hpp index 2ead987b..3cbead5b 100644 --- a/include/macis/hamiltonian_generator/impl.hpp +++ b/include/macis/hamiltonian_generator/impl.hpp @@ -11,8 +11,8 @@ namespace macis { -template -HamiltonianGenerator::HamiltonianGenerator(matrix_span T, +template +HamiltonianGenerator::HamiltonianGenerator(matrix_span T, rank4_span_t V) : norb_(T.extent(0)), norb2_(norb_ * norb_), @@ -22,8 +22,8 @@ HamiltonianGenerator::HamiltonianGenerator(matrix_span T, generate_integral_intermediates(V_pqrs_); } -template -void HamiltonianGenerator::generate_integral_intermediates(rank4_span_t V) { +template +void HamiltonianGenerator::generate_integral_intermediates(rank4_span_t V) { if(V.extent(0) != norb_ or V.extent(1) != norb_ or V.extent(2) != norb_ or V.extent(3) != norb_) throw std::runtime_error("V has incorrect dimensions"); diff --git a/include/macis/hamiltonian_generator/matrix_elements.hpp b/include/macis/hamiltonian_generator/matrix_elements.hpp index 7c232a3f..b3be534d 100644 --- a/include/macis/hamiltonian_generator/matrix_elements.hpp +++ b/include/macis/hamiltonian_generator/matrix_elements.hpp @@ -11,13 +11,13 @@ namespace macis { -template -double HamiltonianGenerator::matrix_element(full_det_t bra, +template +double HamiltonianGenerator::matrix_element(full_det_t bra, full_det_t ket) const { - auto bra_alpha = bitset_lo_word(bra); - auto ket_alpha = bitset_lo_word(ket); - auto bra_beta = bitset_hi_word(bra); - auto ket_beta = bitset_hi_word(ket); + auto bra_alpha = alpha_string(bra); + auto ket_alpha = alpha_string(ket); + auto bra_beta = beta_string(bra); + auto ket_beta = beta_string(ket); auto ex_alpha = bra_alpha ^ ket_alpha; auto ex_beta = bra_beta ^ ket_beta; @@ -29,8 +29,8 @@ double HamiltonianGenerator::matrix_element(full_det_t bra, ex_beta, bra_occ_alpha, bra_occ_beta); } -template -double HamiltonianGenerator::matrix_element( +template +double HamiltonianGenerator::matrix_element( spin_det_t bra_alpha, spin_det_t ket_alpha, spin_det_t ex_alpha, spin_det_t bra_beta, spin_det_t ket_beta, spin_det_t ex_beta, const std::vector& bra_occ_alpha, @@ -62,16 +62,16 @@ double HamiltonianGenerator::matrix_element( return matrix_element_diag(bra_occ_alpha, bra_occ_beta); } -template -double HamiltonianGenerator::matrix_element_4(spin_det_t bra, spin_det_t ket, +template +double HamiltonianGenerator::matrix_element_4(spin_det_t bra, spin_det_t ket, spin_det_t ex) const { auto [o1, v1, o2, v2, sign] = doubles_sign_indices(bra, ket, ex); return sign * G_pqrs_(v1, o1, v2, o2); } -template -double HamiltonianGenerator::matrix_element_22( +template +double HamiltonianGenerator::matrix_element_22( spin_det_t bra_alpha, spin_det_t ket_alpha, spin_det_t ex_alpha, spin_det_t bra_beta, spin_det_t ket_beta, spin_det_t ex_beta) const { auto [o1, v1, sign_a] = @@ -83,8 +83,8 @@ double HamiltonianGenerator::matrix_element_22( return sign * V_pqrs_(v1, o1, v2, o2); } -template -double HamiltonianGenerator::matrix_element_2( +template +double HamiltonianGenerator::matrix_element_2( spin_det_t bra, spin_det_t ket, spin_det_t ex, const std::vector& bra_occ_alpha, const std::vector& bra_occ_beta) const { @@ -105,8 +105,8 @@ double HamiltonianGenerator::matrix_element_2( return sign * h_el; } -template -double HamiltonianGenerator::matrix_element_diag( +template +double HamiltonianGenerator::matrix_element_diag( const std::vector& occ_alpha, const std::vector& occ_beta) const { double h_el = 0; diff --git a/include/macis/hamiltonian_generator/rdms.hpp b/include/macis/hamiltonian_generator/rdms.hpp index ba4cc0f9..00dea8e9 100644 --- a/include/macis/hamiltonian_generator/rdms.hpp +++ b/include/macis/hamiltonian_generator/rdms.hpp @@ -16,8 +16,8 @@ namespace macis { -template -void HamiltonianGenerator::rotate_hamiltonian_ordm(const double* ordm) { +template +void HamiltonianGenerator::rotate_hamiltonian_ordm(const double* ordm) { // SVD on ordm to get natural orbitals std::vector natural_orbitals(ordm, ordm + norb2_); std::vector S(norb_); diff --git a/include/macis/solvers/selected_ci_diag.hpp b/include/macis/solvers/selected_ci_diag.hpp index 0a1e293f..6c1e73ca 100644 --- a/include/macis/solvers/selected_ci_diag.hpp +++ b/include/macis/solvers/selected_ci_diag.hpp @@ -121,10 +121,9 @@ double serial_selected_ci_diag(const SpMatType& H, size_t davidson_max_m, return E; } -template -double selected_ci_diag(wavefunction_iterator_t dets_begin, - wavefunction_iterator_t dets_end, - HamiltonianGenerator& ham_gen, double h_el_tol, +template +double selected_ci_diag(WfnIterator dets_begin, WfnIterator dets_end, + HamiltonianGenerator& ham_gen, double h_el_tol, size_t davidson_max_m, double davidson_res_tol, std::vector& C_local, MACIS_MPI_CODE(MPI_Comm comm, ) diff --git a/include/macis/util/cas.hpp b/include/macis/util/cas.hpp index 34b85b19..faf7c115 100644 --- a/include/macis/util/cas.hpp +++ b/include/macis/util/cas.hpp @@ -34,8 +34,8 @@ double compute_casci_rdms( MCSCFSettings settings, NumOrbital norb, size_t nalpha, size_t nbeta, double* T, double* V, double* ORDM, double* TRDM, std::vector& C MACIS_MPI_CODE(, MPI_Comm comm)) { - constexpr auto nbits = HamGen::nbits; + using wfn_type = typename HamGen::full_det_t; #ifdef MACIS_ENABLE_MPI int rank; MPI_Comm_rank(comm, &rank); @@ -49,9 +49,9 @@ double compute_casci_rdms( rank4_span(V, no, no, no, no)); // Compute Lowest Energy Eigenvalue (ED) - auto dets = generate_hilbert_space>(norb.get(), nalpha, nbeta); + auto dets = generate_hilbert_space(norb.get(), nalpha, nbeta); double E0 = - selected_ci_diag(dets.begin(), dets.end(), ham_gen, settings.ci_matel_tol, + selected_ci_diag(dets.begin(), dets.end(), ham_gen, settings.ci_matel_tol, settings.ci_max_subspace, settings.ci_res_tol, C, MACIS_MPI_CODE(comm, ) true); diff --git a/src/macis/casscf.cxx b/src/macis/casscf.cxx index d58ae4df..049ebf30 100644 --- a/src/macis/casscf.cxx +++ b/src/macis/casscf.cxx @@ -19,7 +19,7 @@ double casscf_diis(MCSCFSettings settings, NumElectron nalpha, size_t LDT, double* V, size_t LDV, double* A1RDM, size_t LDD1, double* A2RDM, size_t LDD2 MACIS_MPI_CODE(, MPI_Comm comm)) { - using generator_t = DoubleLoopHamiltonianGenerator<64>; + using generator_t = DoubleLoopHamiltonianGenerator>; using functor_t = CASRDMFunctor; functor_t op; return mcscf_impl(op, settings, nalpha, nbeta, norb, ninact, nact, diff --git a/tests/asci.cxx b/tests/asci.cxx index 03358cb5..560bc149 100644 --- a/tests/asci.cxx +++ b/tests/asci.cxx @@ -231,7 +231,7 @@ TEST_CASE("ASCI") { macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); // Hamiltonian Genereator - using generator_t = macis::DoubleLoopHamiltonianGenerator<64>; + using generator_t = macis::DoubleLoopHamiltonianGenerator>; generator_t ham_gen( macis::matrix_span(T.data(), norb, norb), macis::rank4_span(V.data(), norb, norb, norb, norb)); diff --git a/tests/csr_hamiltonian.cxx b/tests/csr_hamiltonian.cxx index ba3e3a87..fc0a41be 100644 --- a/tests/csr_hamiltonian.cxx +++ b/tests/csr_hamiltonian.cxx @@ -27,7 +27,7 @@ TEST_CASE("CSR Hamiltonian") { macis::read_fcidump_1body(water_ccpvdz_fcidump, T.data(), norb); macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator<64>; + using generator_type = macis::DoubleLoopHamiltonianGenerator>; #if 0 generator_type ham_gen(norb, V.data(), T.data()); @@ -82,7 +82,7 @@ TEST_CASE("Distributed CSR Hamiltonian") { macis::read_fcidump_1body(water_ccpvdz_fcidump, T.data(), norb); macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator<64>; + using generator_type = macis::DoubleLoopHamiltonianGenerator>; #if 0 generator_type ham_gen(norb, V.data(), T.data()); diff --git a/tests/davidson.cxx b/tests/davidson.cxx index 64a9394e..88105c31 100644 --- a/tests/davidson.cxx +++ b/tests/davidson.cxx @@ -32,7 +32,7 @@ TEST_CASE("Davidson") { macis::read_fcidump_1body(water_ccpvdz_fcidump, T.data(), norb); macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator<64>; + using generator_type = macis::DoubleLoopHamiltonianGenerator>; #if 0 generator_type ham_gen(norb, V.data(), T.data()); @@ -85,7 +85,7 @@ TEST_CASE("Parallel Davidson") { macis::read_fcidump_1body(water_ccpvdz_fcidump, T.data(), norb); macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator<64>; + using generator_type = macis::DoubleLoopHamiltonianGenerator>; #if 0 generator_type ham_gen(norb, V.data(), T.data()); diff --git a/tests/double_loop.cxx b/tests/double_loop.cxx index 5f326b3b..7822f368 100644 --- a/tests/double_loop.cxx +++ b/tests/double_loop.cxx @@ -28,7 +28,7 @@ TEST_CASE("Double Loop") { macis::read_fcidump_1body(water_ccpvdz_fcidump, T.data(), norb); macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator<64>; + using generator_type = macis::DoubleLoopHamiltonianGenerator>; #if 0 generator_type ham_gen(norb, V.data(), T.data()); @@ -194,7 +194,7 @@ TEST_CASE("RDMS") { macis::rank4_span V_span(V.data(), norb, norb, norb, norb); macis::rank4_span trdm_span(trdm.data(), norb, norb, norb, norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator<128>; + using generator_type = macis::DoubleLoopHamiltonianGenerator>; generator_type ham_gen(T_span, V_span); auto abs_sum = [](auto a, auto b) { return a + std::abs(b); }; diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index 495e726d..8849e116 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -285,7 +285,7 @@ int main(int argc, char** argv) { // CI if(job == Job::CI) { - using generator_t = macis::DoubleLoopHamiltonianGenerator; + using generator_t = macis::DoubleLoopHamiltonianGenerator; if(ci_exp == CIExpansion::CAS) { std::vector C_local; // TODO: VERIFY MPI + CAS From c9579ebea4d430c027268b56f74857a6b26c17fb Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Thu, 7 Sep 2023 12:23:04 -0700 Subject: [PATCH 13/73] Refactor HamiltonianGenerator into Base + implementation to encapsulate wfn-independent code --- include/macis/asci/grow.hpp | 2 +- include/macis/hamiltonian_generator.hpp | 89 +------------- include/macis/hamiltonian_generator/base.hpp | 113 ++++++++++++++++++ include/macis/hamiltonian_generator/impl.hpp | 65 ---------- src/macis/CMakeLists.txt | 2 + src/macis/hamiltonian_generator/base.cxx | 8 ++ .../macis/hamiltonian_generator/base.ipp | 80 +++++++++++-- .../hamiltonian_generator/fast_diagonals.ipp | 32 ++--- tests/double_loop.cxx | 2 + 9 files changed, 218 insertions(+), 175 deletions(-) create mode 100644 include/macis/hamiltonian_generator/base.hpp create mode 100644 src/macis/hamiltonian_generator/base.cxx rename include/macis/hamiltonian_generator/rdms.hpp => src/macis/hamiltonian_generator/base.ipp (57%) rename include/macis/hamiltonian_generator/fast_diagonals.hpp => src/macis/hamiltonian_generator/fast_diagonals.ipp (86%) diff --git a/include/macis/asci/grow.hpp b/include/macis/asci/grow.hpp index bf6dd471..2b661401 100644 --- a/include/macis/asci/grow.hpp +++ b/include/macis/asci/grow.hpp @@ -119,7 +119,7 @@ auto asci_grow(ASCISettings asci_settings, MCSCFSettings mcscf_settings, #endif // Regenerate intermediates - ham_gen.generate_integral_intermediates(ham_gen.V_pqrs_); + ham_gen.generate_integral_intermediates(); logger->trace(" * Rediagonalizing"); auto rdg_st = hrt_t::now(); diff --git a/include/macis/hamiltonian_generator.hpp b/include/macis/hamiltonian_generator.hpp index ea4c9758..f34b2fb8 100644 --- a/include/macis/hamiltonian_generator.hpp +++ b/include/macis/hamiltonian_generator.hpp @@ -8,57 +8,21 @@ #pragma once #include -#include -#include +#include namespace macis { template -class HamiltonianGenerator { +class HamiltonianGenerator : public HamiltonianGeneratorBase { public: using full_det_t = WfnType; using spin_det_t = spin_wfn_t; - template - using sparse_matrix_type = sparsexx::csr_matrix; - using full_det_container = std::vector; using full_det_iterator = typename full_det_container::iterator; - using matrix_span_t = matrix_span; - using rank3_span_t = rank3_span; - using rank4_span_t = rank4_span; - - public: - - size_t norb_; - size_t norb2_; - size_t norb3_; - matrix_span_t T_pq_; - rank4_span_t V_pqrs_; - - // G(i,j,k,l) = (ij|kl) - (il|kj) - std::vector G_pqrs_data_; - rank4_span_t G_pqrs_; - - // G_red(i,j,k) = G(i,j,k,k) - std::vector G_red_data_; - rank3_span_t G_red_; - - // V_red(i,j,k) = (ij|kk) - std::vector V_red_data_; - rank3_span_t V_red_; - - // G2_red(i,j) = 0.5 * G(i,i,j,j) - std::vector G2_red_data_; - matrix_span_t G2_red_; - - // V2_red(i,j) = (ii|jj) - std::vector V2_red_data_; - matrix_span_t V2_red_; - virtual sparse_matrix_type make_csr_hamiltonian_block_32bit_( full_det_iterator, full_det_iterator, full_det_iterator, full_det_iterator, double) = 0; @@ -68,16 +32,11 @@ class HamiltonianGenerator { full_det_iterator, double) = 0; public: - HamiltonianGenerator(matrix_span_t T, rank4_span_t V); - virtual ~HamiltonianGenerator() noexcept = default; - void generate_integral_intermediates(rank4_span_t V); + HamiltonianGenerator(matrix_span_t T, rank4_span_t V) : + HamiltonianGeneratorBase(T,V) {}; - inline auto* T() const { return T_pq_.data_handle(); } - inline auto* G_red() const { return G_red_data_.data(); } - inline auto* V_red() const { return V_red_data_.data(); } - inline auto* G() const { return G_pqrs_data_.data(); } - inline auto* V() const { return V_pqrs_.data_handle(); } + virtual ~HamiltonianGenerator() noexcept = default; double matrix_element_4(spin_det_t bra, spin_det_t ket, spin_det_t ex) const; double matrix_element_22(spin_det_t bra_alpha, spin_det_t ket_alpha, @@ -97,42 +56,6 @@ class HamiltonianGenerator { const std::vector& bra_occ_alpha, const std::vector& bra_occ_beta) const; - double single_orbital_en(uint32_t orb, const std::vector& ss_occ, - const std::vector& os_occ) const; - - std::vector single_orbital_ens( - size_t norb, const std::vector& ss_occ, - const std::vector& os_occ) const; - - double fast_diag_single(const std::vector& ss_occ, - const std::vector& os_occ, uint32_t orb_hol, - uint32_t orb_par, double orig_det_Hii) const; - - double fast_diag_single(double hol_en, double par_en, uint32_t orb_hol, - uint32_t orb_par, double orig_det_Hii) const; - - double fast_diag_ss_double(double en_hol1, double en_hol2, double en_par1, - double en_par2, uint32_t orb_hol1, - uint32_t orb_hol2, uint32_t orb_par1, - uint32_t orb_par2, double orig_det_Hii) const; - - double fast_diag_ss_double(const std::vector& ss_occ, - const std::vector& os_occ, - uint32_t orb_hol1, uint32_t orb_hol2, - uint32_t orb_par1, uint32_t orb_par2, - double orig_det_Hii) const; - - double fast_diag_os_double(double en_holu, double en_hold, double en_paru, - double en_pard, uint32_t orb_holu, - uint32_t orb_hold, uint32_t orb_paru, - uint32_t orb_pard, double orig_det_Hii) const; - - double fast_diag_os_double(const std::vector& up_occ, - const std::vector& do_occ, - uint32_t orb_holu, uint32_t orb_hold, - uint32_t orb_paru, uint32_t orb_pard, - double orig_det_Hii) const; - double matrix_element(full_det_t bra, full_det_t ket) const; template @@ -176,8 +99,6 @@ class HamiltonianGenerator { full_det_iterator, full_det_iterator, double* C, matrix_span_t ordm, rank4_span_t trdm) = 0; - void rotate_hamiltonian_ordm(const double* ordm); - virtual void SetJustSingles(bool /*_js*/) {} virtual bool GetJustSingles() { return false; } //virtual size_t GetNimp() const { return N / 2; } diff --git a/include/macis/hamiltonian_generator/base.hpp b/include/macis/hamiltonian_generator/base.hpp new file mode 100644 index 00000000..e96cf9e8 --- /dev/null +++ b/include/macis/hamiltonian_generator/base.hpp @@ -0,0 +1,113 @@ +/* + * MACIS Copyright (c) 2023, The Regents of the University of California, + * through Lawrence Berkeley National Laboratory (subject to receipt of + * any required approvals from the U.S. Dept. of Energy). All rights reserved. + * + * See LICENSE.txt for details + */ + +#pragma once +#include +#include + +namespace macis { + +template +class HamiltonianGeneratorBase { + + protected: + + template + using sparse_matrix_type = sparsexx::csr_matrix; + + using matrix_span_t = matrix_span; + using rank3_span_t = rank3_span; + using rank4_span_t = rank4_span; + + size_t norb_; + size_t norb2_; + size_t norb3_; + matrix_span_t T_pq_; + rank4_span_t V_pqrs_; + + // G(i,j,k,l) = (ij|kl) - (il|kj) + std::vector G_pqrs_data_; + rank4_span_t G_pqrs_; + + // G_red(i,j,k) = G(i,j,k,k) + std::vector G_red_data_; + rank3_span_t G_red_; + + // V_red(i,j,k) = (ij|kk) + std::vector V_red_data_; + rank3_span_t V_red_; + + // G2_red(i,j) = 0.5 * G(i,i,j,j) + std::vector G2_red_data_; + matrix_span_t G2_red_; + + // V2_red(i,j) = (ii|jj) + std::vector V2_red_data_; + matrix_span_t V2_red_; + + void generate_integral_intermediates_(rank4_span_t V); + + public: + + HamiltonianGeneratorBase(matrix_span_t T, rank4_span_t V); + virtual ~HamiltonianGeneratorBase() noexcept = default; + + inline auto* T() const { return T_pq_.data_handle(); } + inline auto* G_red() const { return G_red_data_.data(); } + inline auto* V_red() const { return V_red_data_.data(); } + inline auto* G() const { return G_pqrs_data_.data(); } + inline auto* V() const { return V_pqrs_.data_handle(); } + + inline void generate_integral_intermediates() { + generate_integral_intermediates_(V_pqrs_); + } + + + double single_orbital_en(uint32_t orb, const std::vector& ss_occ, + const std::vector& os_occ) const; + + std::vector single_orbital_ens( + size_t norb, const std::vector& ss_occ, + const std::vector& os_occ) const; + + double fast_diag_single(const std::vector& ss_occ, + const std::vector& os_occ, uint32_t orb_hol, + uint32_t orb_par, double orig_det_Hii) const; + + double fast_diag_single(double hol_en, double par_en, uint32_t orb_hol, + uint32_t orb_par, double orig_det_Hii) const; + + double fast_diag_ss_double(double en_hol1, double en_hol2, double en_par1, + double en_par2, uint32_t orb_hol1, + uint32_t orb_hol2, uint32_t orb_par1, + uint32_t orb_par2, double orig_det_Hii) const; + + double fast_diag_ss_double(const std::vector& ss_occ, + const std::vector& os_occ, + uint32_t orb_hol1, uint32_t orb_hol2, + uint32_t orb_par1, uint32_t orb_par2, + double orig_det_Hii) const; + + double fast_diag_os_double(double en_holu, double en_hold, double en_paru, + double en_pard, uint32_t orb_holu, + uint32_t orb_hold, uint32_t orb_paru, + uint32_t orb_pard, double orig_det_Hii) const; + + double fast_diag_os_double(const std::vector& up_occ, + const std::vector& do_occ, + uint32_t orb_holu, uint32_t orb_hold, + uint32_t orb_paru, uint32_t orb_pard, + double orig_det_Hii) const; + + + + void rotate_hamiltonian_ordm(const Scalar* ordm); + +}; + +} diff --git a/include/macis/hamiltonian_generator/impl.hpp b/include/macis/hamiltonian_generator/impl.hpp index 3cbead5b..d4d8e964 100644 --- a/include/macis/hamiltonian_generator/impl.hpp +++ b/include/macis/hamiltonian_generator/impl.hpp @@ -7,70 +7,5 @@ */ #pragma once -#include -namespace macis { - -template -HamiltonianGenerator::HamiltonianGenerator(matrix_span T, - rank4_span_t V) - : norb_(T.extent(0)), - norb2_(norb_ * norb_), - norb3_(norb2_ * norb_), - T_pq_(T), - V_pqrs_(V) { - generate_integral_intermediates(V_pqrs_); -} - -template -void HamiltonianGenerator::generate_integral_intermediates(rank4_span_t V) { - if(V.extent(0) != norb_ or V.extent(1) != norb_ or V.extent(2) != norb_ or - V.extent(3) != norb_) - throw std::runtime_error("V has incorrect dimensions"); - - size_t no = norb_; - size_t no2 = no * no; - size_t no3 = no2 * no; - size_t no4 = no3 * no; - - // G(i,j,k,l) = V(i,j,k,l) - V(i,l,k,j) - G_pqrs_data_ = std::vector(begin(V), end(V)); - G_pqrs_ = rank4_span_t(G_pqrs_data_.data(), no, no, no, no); - for(auto i = 0ul; i < no; ++i) - for(auto j = 0ul; j < no; ++j) - for(auto k = 0ul; k < no; ++k) - for(auto l = 0ul; l < no; ++l) { - G_pqrs_(i, j, k, l) -= V(i, l, k, j); - } - - // G_red(i,j,k) = G(i,j,k,k) = G(k,k,i,j) - // V_red(i,j,k) = V(i,j,k,k) = V(k,k,i,j) - G_red_data_.resize(no3); - V_red_data_.resize(no3); - G_red_ = rank3_span_t(G_red_data_.data(), no, no, no); - V_red_ = rank3_span_t(V_red_data_.data(), no, no, no); - for(auto j = 0ul; j < no; ++j) - for(auto i = 0ul; i < no; ++i) - for(auto k = 0ul; k < no; ++k) { - G_red_(k, i, j) = G_pqrs_(k, k, i, j); - V_red_(k, i, j) = V(k, k, i, j); - } - - // G2_red(i,j) = 0.5 * G(i,i,j,j) - // V2_red(i,j) = V(i,i,j,j) - G2_red_data_.resize(no2); - V2_red_data_.resize(no2); - G2_red_ = matrix_span(G2_red_data_.data(), no, no); - V2_red_ = matrix_span(V2_red_data_.data(), no, no); - for(auto j = 0ul; j < no; ++j) - for(auto i = 0ul; i < no; ++i) { - G2_red_(i, j) = 0.5 * G_pqrs_(i, i, j, j); - V2_red_(i, j) = V(i, i, j, j); - } -} - -} // namespace macis - -#include #include -#include diff --git a/src/macis/CMakeLists.txt b/src/macis/CMakeLists.txt index 26155ac6..57d9ed6a 100644 --- a/src/macis/CMakeLists.txt +++ b/src/macis/CMakeLists.txt @@ -15,6 +15,8 @@ add_library( macis orbital_rotation_utilities.cxx orbital_hessian.cxx orbital_steps.cxx + + hamiltonian_generator/base.cxx ) target_include_directories( macis PUBLIC diff --git a/src/macis/hamiltonian_generator/base.cxx b/src/macis/hamiltonian_generator/base.cxx new file mode 100644 index 00000000..e96ce11a --- /dev/null +++ b/src/macis/hamiltonian_generator/base.cxx @@ -0,0 +1,8 @@ +#include "base.ipp" +#include "fast_diagonals.ipp" + +namespace macis { + +template class HamiltonianGeneratorBase; + +} diff --git a/include/macis/hamiltonian_generator/rdms.hpp b/src/macis/hamiltonian_generator/base.ipp similarity index 57% rename from include/macis/hamiltonian_generator/rdms.hpp rename to src/macis/hamiltonian_generator/base.ipp index 00dea8e9..a39ea749 100644 --- a/include/macis/hamiltonian_generator/rdms.hpp +++ b/src/macis/hamiltonian_generator/base.ipp @@ -7,7 +7,8 @@ */ #pragma once -#include +#include + #pragma GCC diagnostic push #pragma GCC diagnostic ignored "-Wunused-parameter" #include @@ -16,17 +17,77 @@ namespace macis { -template -void HamiltonianGenerator::rotate_hamiltonian_ordm(const double* ordm) { +template +HamiltonianGeneratorBase::HamiltonianGeneratorBase(matrix_span_t T, + rank4_span_t V) + : norb_(T.extent(0)), + norb2_(norb_ * norb_), + norb3_(norb2_ * norb_), + T_pq_(T), + V_pqrs_(V) { + generate_integral_intermediates_(V_pqrs_); +} + +template +void HamiltonianGeneratorBase::generate_integral_intermediates_(rank4_span_t V) { + if(V.extent(0) != norb_ or V.extent(1) != norb_ or V.extent(2) != norb_ or + V.extent(3) != norb_) + throw std::runtime_error("V has incorrect dimensions"); + + size_t no = norb_; + size_t no2 = no * no; + size_t no3 = no2 * no; + size_t no4 = no3 * no; + + // G(i,j,k,l) = V(i,j,k,l) - V(i,l,k,j) + G_pqrs_data_ = std::vector(begin(V), end(V)); + G_pqrs_ = rank4_span_t(G_pqrs_data_.data(), no, no, no, no); + for(auto i = 0ul; i < no; ++i) + for(auto j = 0ul; j < no; ++j) + for(auto k = 0ul; k < no; ++k) + for(auto l = 0ul; l < no; ++l) { + G_pqrs_(i, j, k, l) -= V(i, l, k, j); + } + + // G_red(i,j,k) = G(i,j,k,k) = G(k,k,i,j) + // V_red(i,j,k) = V(i,j,k,k) = V(k,k,i,j) + G_red_data_.resize(no3); + V_red_data_.resize(no3); + G_red_ = rank3_span_t(G_red_data_.data(), no, no, no); + V_red_ = rank3_span_t(V_red_data_.data(), no, no, no); + for(auto j = 0ul; j < no; ++j) + for(auto i = 0ul; i < no; ++i) + for(auto k = 0ul; k < no; ++k) { + G_red_(k, i, j) = G_pqrs_(k, k, i, j); + V_red_(k, i, j) = V(k, k, i, j); + } + + // G2_red(i,j) = 0.5 * G(i,i,j,j) + // V2_red(i,j) = V(i,i,j,j) + G2_red_data_.resize(no2); + V2_red_data_.resize(no2); + G2_red_ = matrix_span(G2_red_data_.data(), no, no); + V2_red_ = matrix_span(V2_red_data_.data(), no, no); + for(auto j = 0ul; j < no; ++j) + for(auto i = 0ul; i < no; ++i) { + G2_red_(i, j) = 0.5 * G_pqrs_(i, i, j, j); + V2_red_(i, j) = V(i, i, j, j); + } +} + + + +template +void HamiltonianGeneratorBase::rotate_hamiltonian_ordm(const Scalar* ordm) { // SVD on ordm to get natural orbitals - std::vector natural_orbitals(ordm, ordm + norb2_); - std::vector S(norb_); + std::vector natural_orbitals(ordm, ordm + norb2_); + std::vector S(norb_); lapack::gesvd(lapack::Job::OverwriteVec, lapack::Job::NoVec, norb_, norb_, natural_orbitals.data(), norb_, S.data(), NULL, 1, NULL, 1); #if 0 { - std::vector tmp(norb2_); + std::vector tmp(norb2_); blas::gemm(blas::Layout::ColMajor, blas::Op::Trans, blas::Op::NoTrans, norb_, norb_, norb_, 1., natural_orbitals.data(), norb_, natural_orbitals.data(), norb_, 0., tmp.data(), norb_ ); @@ -34,7 +95,7 @@ void HamiltonianGenerator::rotate_hamiltonian_ordm(const double* ordm) std::cout << "MAX = " << *std::max_element(tmp.begin(),tmp.end(), []( auto x, auto y ){ return std::abs(x) < std::abs(y); } ) << std::endl; - double max_diff = 0.; + Scalar max_diff = 0.; for( auto i = 0; i < norb_; ++i ) for( auto j = i+1; j < norb_; ++j ) { max_diff = std::max( max_diff, @@ -44,7 +105,7 @@ void HamiltonianGenerator::rotate_hamiltonian_ordm(const double* ordm) } #endif - std::vector tmp(norb3_ * norb_), tmp2(norb3_ * norb_); + std::vector tmp(norb3_ * norb_), tmp2(norb3_ * norb_); // Transform T // T <- N**H * T * N @@ -95,7 +156,8 @@ void HamiltonianGenerator::rotate_hamiltonian_ordm(const double* ordm) natural_orbitals.data(), norb_, 0., V_pqrs_.data_handle(), norb3_); // Regenerate intermediates - generate_integral_intermediates(V_pqrs_); + generate_integral_intermediates_(V_pqrs_); } } // namespace macis + diff --git a/include/macis/hamiltonian_generator/fast_diagonals.hpp b/src/macis/hamiltonian_generator/fast_diagonals.ipp similarity index 86% rename from include/macis/hamiltonian_generator/fast_diagonals.hpp rename to src/macis/hamiltonian_generator/fast_diagonals.ipp index e561ea7c..a76292b7 100644 --- a/include/macis/hamiltonian_generator/fast_diagonals.hpp +++ b/src/macis/hamiltonian_generator/fast_diagonals.ipp @@ -11,8 +11,8 @@ namespace macis { -template -double HamiltonianGenerator::single_orbital_en( +template +double HamiltonianGeneratorBase::single_orbital_en( uint32_t orb, const std::vector& ss_occ, const std::vector& os_occ) const { // One electron component @@ -28,8 +28,8 @@ double HamiltonianGenerator::single_orbital_en( return orb_en; } -template -std::vector HamiltonianGenerator::single_orbital_ens( +template +std::vector HamiltonianGeneratorBase::single_orbital_ens( size_t norb, const std::vector& ss_occ, const std::vector& os_occ) const { std::vector ens(norb); @@ -50,8 +50,8 @@ std::vector HamiltonianGenerator::single_orbital_ens( return ens; } -template -double HamiltonianGenerator::fast_diag_single( +template +double HamiltonianGeneratorBase::fast_diag_single( // These refer to original determinant double hol_en, double par_en, uint32_t orb_hol, uint32_t orb_par, double orig_det_Hii) const { @@ -59,8 +59,8 @@ double HamiltonianGenerator::fast_diag_single( G2_red_(orb_hol, orb_par); } -template -double HamiltonianGenerator::fast_diag_single( +template +double HamiltonianGeneratorBase::fast_diag_single( // These refer to original determinant const std::vector& ss_occ, const std::vector& os_occ, uint32_t orb_hol, uint32_t orb_par, double orig_det_Hii) const { @@ -69,8 +69,8 @@ double HamiltonianGenerator::fast_diag_single( return fast_diag_single(hol_en, par_en, orb_hol, orb_par, orig_det_Hii); } -template -double HamiltonianGenerator::fast_diag_ss_double( +template +double HamiltonianGeneratorBase::fast_diag_ss_double( // These refer to original determinant double hol1_en, double hol2_en, double par1_en, double par2_en, uint32_t orb_hol1, uint32_t orb_hol2, uint32_t orb_par1, uint32_t orb_par2, @@ -84,8 +84,8 @@ double HamiltonianGenerator::fast_diag_ss_double( G2_red_(orb_par2, orb_hol2) - G2_red_(orb_hol2, orb_par2); } -template -double HamiltonianGenerator::fast_diag_ss_double( +template +double HamiltonianGeneratorBase::fast_diag_ss_double( // These refer to original determinant const std::vector& ss_occ, const std::vector& os_occ, uint32_t orb_hol1, uint32_t orb_hol2, uint32_t orb_par1, uint32_t orb_par2, @@ -98,8 +98,8 @@ double HamiltonianGenerator::fast_diag_ss_double( orb_hol2, orb_par1, orb_par2, orig_det_Hii); } -template -double HamiltonianGenerator::fast_diag_os_double( +template +double HamiltonianGeneratorBase::fast_diag_os_double( // These refer to original determinant double en_holu, double en_hold, double en_paru, double en_pard, uint32_t orb_holu, uint32_t orb_hold, uint32_t orb_paru, uint32_t orb_pard, @@ -111,8 +111,8 @@ double HamiltonianGenerator::fast_diag_os_double( V2_red_(orb_paru, orb_hold) - V2_red_(orb_holu, orb_pard); } -template -double HamiltonianGenerator::fast_diag_os_double( +template +double HamiltonianGeneratorBase::fast_diag_os_double( // These refer to original determinant const std::vector& ss_occ, const std::vector& os_occ, uint32_t orb_holu, uint32_t orb_hold, uint32_t orb_paru, uint32_t orb_pard, diff --git a/tests/double_loop.cxx b/tests/double_loop.cxx index 7822f368..fa4ab232 100644 --- a/tests/double_loop.cxx +++ b/tests/double_loop.cxx @@ -12,6 +12,8 @@ #include #include +#include + #include "ut_common.hpp" TEST_CASE("Double Loop") { From 979b1b0e0b234962b61fb1b412894debeb4cfa02 Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Fri, 8 Sep 2023 08:24:09 -0700 Subject: [PATCH 14/73] Refactor source locations for CAS(SCF) utilities --- include/macis/asci/iteration.hpp | 2 +- include/macis/{util => mcscf}/cas.hpp | 2 +- include/macis/{util => mcscf}/diis.hpp | 0 include/macis/{util => mcscf}/fock_matrices.hpp | 0 include/macis/{util => mcscf}/mcscf.hpp | 0 include/macis/{util => mcscf}/mcscf_impl.hpp | 15 ++++++++------- .../macis/{util => mcscf}/orbital_energies.hpp | 0 .../macis/{util => mcscf}/orbital_gradient.hpp | 0 include/macis/{util => mcscf}/orbital_hessian.hpp | 4 ++-- .../orbital_rotation_utilities.hpp | 0 include/macis/{util => mcscf}/orbital_steps.hpp | 0 src/macis/CMakeLists.txt | 15 ++++++++------- src/macis/{ => mcscf}/casscf.cxx | 6 +++--- src/macis/{ => mcscf}/fock_matrices.cxx | 2 +- src/macis/{ => mcscf}/orbital_energies.cxx | 2 +- src/macis/{ => mcscf}/orbital_gradient.cxx | 4 ++-- src/macis/{ => mcscf}/orbital_hessian.cxx | 2 +- .../{ => mcscf}/orbital_rotation_utilities.cxx | 2 +- src/macis/{ => mcscf}/orbital_steps.cxx | 4 ++-- src/macis/moller_plesset.cxx | 2 +- tests/fcidump.cxx | 2 +- tests/fock_matrices.cxx | 2 +- tests/mcscf.cxx | 2 +- tests/standalone_driver.cxx | 4 ++-- 24 files changed, 37 insertions(+), 35 deletions(-) rename include/macis/{util => mcscf}/cas.hpp (98%) rename include/macis/{util => mcscf}/diis.hpp (100%) rename include/macis/{util => mcscf}/fock_matrices.hpp (100%) rename include/macis/{util => mcscf}/mcscf.hpp (100%) rename include/macis/{util => mcscf}/mcscf_impl.hpp (98%) rename include/macis/{util => mcscf}/orbital_energies.hpp (100%) rename include/macis/{util => mcscf}/orbital_gradient.hpp (100%) rename include/macis/{util => mcscf}/orbital_hessian.hpp (96%) rename include/macis/{util => mcscf}/orbital_rotation_utilities.hpp (100%) rename include/macis/{util => mcscf}/orbital_steps.hpp (100%) rename src/macis/{ => mcscf}/casscf.cxx (91%) rename src/macis/{ => mcscf}/fock_matrices.cxx (99%) rename src/macis/{ => mcscf}/orbital_energies.cxx (95%) rename src/macis/{ => mcscf}/orbital_gradient.cxx (99%) rename src/macis/{ => mcscf}/orbital_hessian.cxx (99%) rename src/macis/{ => mcscf}/orbital_rotation_utilities.cxx (98%) rename src/macis/{ => mcscf}/orbital_steps.cxx (99%) diff --git a/include/macis/asci/iteration.hpp b/include/macis/asci/iteration.hpp index 8db17efc..dd913c43 100644 --- a/include/macis/asci/iteration.hpp +++ b/include/macis/asci/iteration.hpp @@ -9,7 +9,7 @@ #pragma once #include #include -#include +#include namespace macis { diff --git a/include/macis/util/cas.hpp b/include/macis/mcscf/cas.hpp similarity index 98% rename from include/macis/util/cas.hpp rename to include/macis/mcscf/cas.hpp index faf7c115..2ca1962b 100644 --- a/include/macis/util/cas.hpp +++ b/include/macis/mcscf/cas.hpp @@ -9,7 +9,7 @@ #pragma once #include #include -#include +#include namespace macis { diff --git a/include/macis/util/diis.hpp b/include/macis/mcscf/diis.hpp similarity index 100% rename from include/macis/util/diis.hpp rename to include/macis/mcscf/diis.hpp diff --git a/include/macis/util/fock_matrices.hpp b/include/macis/mcscf/fock_matrices.hpp similarity index 100% rename from include/macis/util/fock_matrices.hpp rename to include/macis/mcscf/fock_matrices.hpp diff --git a/include/macis/util/mcscf.hpp b/include/macis/mcscf/mcscf.hpp similarity index 100% rename from include/macis/util/mcscf.hpp rename to include/macis/mcscf/mcscf.hpp diff --git a/include/macis/util/mcscf_impl.hpp b/include/macis/mcscf/mcscf_impl.hpp similarity index 98% rename from include/macis/util/mcscf_impl.hpp rename to include/macis/mcscf/mcscf_impl.hpp index 48d1f850..746c9cce 100644 --- a/include/macis/util/mcscf_impl.hpp +++ b/include/macis/mcscf/mcscf_impl.hpp @@ -7,16 +7,17 @@ */ #pragma once -#include #include -#include -#include -#include -#include -#include -#include #include +#include +#include +#include +#include +#include +#include +#include + // #include namespace macis { diff --git a/include/macis/util/orbital_energies.hpp b/include/macis/mcscf/orbital_energies.hpp similarity index 100% rename from include/macis/util/orbital_energies.hpp rename to include/macis/mcscf/orbital_energies.hpp diff --git a/include/macis/util/orbital_gradient.hpp b/include/macis/mcscf/orbital_gradient.hpp similarity index 100% rename from include/macis/util/orbital_gradient.hpp rename to include/macis/mcscf/orbital_gradient.hpp diff --git a/include/macis/util/orbital_hessian.hpp b/include/macis/mcscf/orbital_hessian.hpp similarity index 96% rename from include/macis/util/orbital_hessian.hpp rename to include/macis/mcscf/orbital_hessian.hpp index 53f59c18..88b05935 100644 --- a/include/macis/util/orbital_hessian.hpp +++ b/include/macis/mcscf/orbital_hessian.hpp @@ -8,8 +8,8 @@ #pragma once #include -#include -#include +#include +#include namespace macis { diff --git a/include/macis/util/orbital_rotation_utilities.hpp b/include/macis/mcscf/orbital_rotation_utilities.hpp similarity index 100% rename from include/macis/util/orbital_rotation_utilities.hpp rename to include/macis/mcscf/orbital_rotation_utilities.hpp diff --git a/include/macis/util/orbital_steps.hpp b/include/macis/mcscf/orbital_steps.hpp similarity index 100% rename from include/macis/util/orbital_steps.hpp rename to include/macis/mcscf/orbital_steps.hpp diff --git a/src/macis/CMakeLists.txt b/src/macis/CMakeLists.txt index 57d9ed6a..b50aafbe 100644 --- a/src/macis/CMakeLists.txt +++ b/src/macis/CMakeLists.txt @@ -6,15 +6,16 @@ add_library( macis fcidump.cxx - fock_matrices.cxx transform.cxx - orbital_gradient.cxx - casscf.cxx moller_plesset.cxx - orbital_energies.cxx - orbital_rotation_utilities.cxx - orbital_hessian.cxx - orbital_steps.cxx + + mcscf/fock_matrices.cxx + mcscf/casscf.cxx + mcscf/orbital_gradient.cxx + mcscf/orbital_energies.cxx + mcscf/orbital_rotation_utilities.cxx + mcscf/orbital_hessian.cxx + mcscf/orbital_steps.cxx hamiltonian_generator/base.cxx ) diff --git a/src/macis/casscf.cxx b/src/macis/mcscf/casscf.cxx similarity index 91% rename from src/macis/casscf.cxx rename to src/macis/mcscf/casscf.cxx index 049ebf30..075f3777 100644 --- a/src/macis/casscf.cxx +++ b/src/macis/mcscf/casscf.cxx @@ -7,9 +7,9 @@ */ #include -#include -#include -#include +#include +#include +#include namespace macis { diff --git a/src/macis/fock_matrices.cxx b/src/macis/mcscf/fock_matrices.cxx similarity index 99% rename from src/macis/fock_matrices.cxx rename to src/macis/mcscf/fock_matrices.cxx index a2708f14..40bd82b8 100644 --- a/src/macis/fock_matrices.cxx +++ b/src/macis/mcscf/fock_matrices.cxx @@ -7,7 +7,7 @@ */ #include -#include +#include #include namespace macis { diff --git a/src/macis/orbital_energies.cxx b/src/macis/mcscf/orbital_energies.cxx similarity index 95% rename from src/macis/orbital_energies.cxx rename to src/macis/mcscf/orbital_energies.cxx index 97395b59..ef34c632 100644 --- a/src/macis/orbital_energies.cxx +++ b/src/macis/mcscf/orbital_energies.cxx @@ -6,7 +6,7 @@ * See LICENSE.txt for details */ -#include +#include namespace macis { diff --git a/src/macis/orbital_gradient.cxx b/src/macis/mcscf/orbital_gradient.cxx similarity index 99% rename from src/macis/orbital_gradient.cxx rename to src/macis/mcscf/orbital_gradient.cxx index 918bfbae..3abedee9 100644 --- a/src/macis/orbital_gradient.cxx +++ b/src/macis/mcscf/orbital_gradient.cxx @@ -7,8 +7,8 @@ */ #include -#include -#include +#include +#include #include #include diff --git a/src/macis/orbital_hessian.cxx b/src/macis/mcscf/orbital_hessian.cxx similarity index 99% rename from src/macis/orbital_hessian.cxx rename to src/macis/mcscf/orbital_hessian.cxx index fcddd407..e5734bfa 100644 --- a/src/macis/orbital_hessian.cxx +++ b/src/macis/mcscf/orbital_hessian.cxx @@ -9,7 +9,7 @@ #include #include #include -#include +#include #include namespace macis { diff --git a/src/macis/orbital_rotation_utilities.cxx b/src/macis/mcscf/orbital_rotation_utilities.cxx similarity index 98% rename from src/macis/orbital_rotation_utilities.cxx rename to src/macis/mcscf/orbital_rotation_utilities.cxx index 8912902b..8ffdfe35 100644 --- a/src/macis/orbital_rotation_utilities.cxx +++ b/src/macis/mcscf/orbital_rotation_utilities.cxx @@ -6,7 +6,7 @@ * See LICENSE.txt for details */ -#include +#include namespace macis { diff --git a/src/macis/orbital_steps.cxx b/src/macis/mcscf/orbital_steps.cxx similarity index 99% rename from src/macis/orbital_steps.cxx rename to src/macis/mcscf/orbital_steps.cxx index 95fd4f43..d50a4a5c 100644 --- a/src/macis/orbital_steps.cxx +++ b/src/macis/mcscf/orbital_steps.cxx @@ -6,8 +6,8 @@ * See LICENSE.txt for details */ -#include -#include +#include +#include namespace macis { diff --git a/src/macis/moller_plesset.cxx b/src/macis/moller_plesset.cxx index 5e00d85c..902d8b19 100644 --- a/src/macis/moller_plesset.cxx +++ b/src/macis/moller_plesset.cxx @@ -9,7 +9,7 @@ #include #include #include -#include +#include namespace macis { diff --git a/tests/fcidump.cxx b/tests/fcidump.cxx index 7f39c11c..9d0d08fe 100644 --- a/tests/fcidump.cxx +++ b/tests/fcidump.cxx @@ -9,7 +9,7 @@ #include #include #include -#include +#include #include "ut_common.hpp" diff --git a/tests/fock_matrices.cxx b/tests/fock_matrices.cxx index 75a84a05..042a0e05 100644 --- a/tests/fock_matrices.cxx +++ b/tests/fock_matrices.cxx @@ -9,7 +9,7 @@ #include #include #include -#include +#include #include "ut_common.hpp" diff --git a/tests/mcscf.cxx b/tests/mcscf.cxx index 7bdd1b80..c1a372da 100644 --- a/tests/mcscf.cxx +++ b/tests/mcscf.cxx @@ -12,7 +12,7 @@ #include #include #include -#include +#include #include "ut_common.hpp" diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index 8849e116..e8926d69 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -18,10 +18,10 @@ #include #include #include -#include #include #include -#include +#include +#include #include #include #include From bc4ed605f8aac63fda86ec32b4b9df6dcd4fdeb2 Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Fri, 8 Sep 2023 09:50:17 -0700 Subject: [PATCH 15/73] Generic ASCI contributions w/o constraints --- .../macis/asci/determinant_contributions.hpp | 51 ++++++++++++------- include/macis/asci/determinant_search.hpp | 21 ++++---- include/macis/asci/pt2.hpp | 9 ++-- include/macis/sd_operations.hpp | 32 ++++++++++++ tests/asci.cxx | 16 ++++-- 5 files changed, 95 insertions(+), 34 deletions(-) diff --git a/include/macis/asci/determinant_contributions.hpp b/include/macis/asci/determinant_contributions.hpp index 1db2b827..9853ff74 100644 --- a/include/macis/asci/determinant_contributions.hpp +++ b/include/macis/asci/determinant_contributions.hpp @@ -25,16 +25,17 @@ struct asci_contrib { template using asci_contrib_container = std::vector>; -template + +template void append_singles_asci_contributions( - double coeff, wfn_t<2 * N> state_full, wfn_t state_same, + double coeff, WfnType state_full, SpinWfnType state_same, const std::vector& occ_same, const std::vector& vir_same, const std::vector& occ_othr, const double* eps_same, const double* T_pq, const size_t LDT, const double* G_kpq, const size_t LDG, const double* V_kpq, const size_t LDV, double h_el_tol, double root_diag, - double E0, HamiltonianGenerator>& ham_gen, - asci_contrib_container>& asci_contributions) { + double E0, const HamiltonianGeneratorBase& ham_gen, + asci_contrib_container& asci_contributions) { const auto LDG2 = LDG * LDG; const auto LDV2 = LDV * LDV; for(auto i : occ_same) @@ -50,8 +51,7 @@ void append_singles_asci_contributions( if(std::abs(h_el) < h_el_tol) continue; // Calculate Excited Determinant - auto ex_det = state_full; - ex_det.flip(i + NShift).flip(a + NShift); + auto ex_det = single_excitation_spin(state_full, i, a); // Calculate Excitation Sign in a Canonical Way auto sign = single_excitation_sign(state_same, a, i); @@ -68,14 +68,15 @@ void append_singles_asci_contributions( } // Loop over single extitations } -template +template void append_ss_doubles_asci_contributions( - double coeff, wfn_t<2 * N> state_full, wfn_t state_spin, + double coeff, WfnType state_full, SpinWfnType state_same, + SpinWfnType state_other, const std::vector& ss_occ, const std::vector& vir, const std::vector& os_occ, const double* eps_same, const double* G, size_t LDG, double h_el_tol, double root_diag, double E0, - HamiltonianGenerator>& ham_gen, - asci_contrib_container>& asci_contributions) { + const HamiltonianGeneratorBase& ham_gen, + asci_contrib_container& asci_contributions) { const size_t nocc = ss_occ.size(); const size_t nvir = vir.size(); @@ -95,6 +96,7 @@ void append_ss_doubles_asci_contributions( if(std::abs(G_aibj) < h_el_tol) continue; +#if 0 // Calculate excited determinant string (spin) const auto full_ex_spin = wfn_t(0).flip(i).flip(j).flip(a).flip(b); auto ex_det_spin = state_spin ^ full_ex_spin; @@ -105,6 +107,19 @@ void append_ss_doubles_asci_contributions( // Calculate full excited determinant const auto full_ex = expand_bitset<2 * N>(full_ex_spin) << NShift; auto ex_det = state_full ^ full_ex; +#else + // TODO: Can this be made faster since the orbital indices are known + // in advance? + // Compute excited determinant (spin) + const auto full_ex_spin = double_excitation(SpinWfnType(0), i,j,a,b); + const auto ex_det_spin = state_same ^ full_ex_spin; + + // Calculate the sign in a canonical way + double sign = doubles_sign(state_same, ex_det_spin, full_ex_spin); + + // Calculate full excited determinant + auto ex_det = from_spin_safe(ex_det_spin, state_other); +#endif // Update sign of matrix element auto h_el = sign * G_aibj; @@ -122,16 +137,16 @@ void append_ss_doubles_asci_contributions( } // AI Loop } -template +template void append_os_doubles_asci_contributions( - double coeff, wfn_t<2 * N> state_full, wfn_t state_alpha, - wfn_t state_beta, const std::vector& occ_alpha, + double coeff, WfnType state_full, SpinWfnType state_alpha, + SpinWfnType state_beta, const std::vector& occ_alpha, const std::vector& occ_beta, const std::vector& vir_alpha, const std::vector& vir_beta, const double* eps_alpha, const double* eps_beta, const double* V, size_t LDV, double h_el_tol, - double root_diag, double E0, HamiltonianGenerator>& ham_gen, - asci_contrib_container>& asci_contributions) { + double root_diag, double E0, const HamiltonianGeneratorBase& ham_gen, + asci_contrib_container& asci_contributions) { const size_t LDV2 = LDV * LDV; for(auto i : occ_alpha) for(auto a : vir_alpha) { @@ -147,8 +162,10 @@ void append_os_doubles_asci_contributions( double sign_beta = single_excitation_sign(state_beta, b, j); double sign = sign_alpha * sign_beta; - auto ex_det = state_full; - ex_det.flip(a).flip(i).flip(j + N).flip(b + N); + //auto ex_det = state_full; + //ex_det.flip(a).flip(i).flip(j + N).flip(b + N); + auto ex_det = single_excitation_spin(state_full, a, i); + ex_det = single_excitation_spin(ex_det, b, j); auto h_el = sign * V_aibj; // Evaluate fast diagonal element diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index 8582b832..7037dc39 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -86,27 +86,27 @@ asci_contrib_container> asci_contributions_standard( const double h_el_tol = asci_settings.h_el_tol; // Singles - AA - append_singles_asci_contributions<(N / 2), 0>( + append_singles_asci_contributions( coeff, state, state_alpha, occ_alpha, vir_alpha, occ_beta, eps_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); // Singles - BB - append_singles_asci_contributions<(N / 2), (N / 2)>( + append_singles_asci_contributions( coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, eps_beta.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); if(not asci_settings.just_singles) { // Doubles - AAAA - append_ss_doubles_asci_contributions( - coeff, state, state_alpha, occ_alpha, vir_alpha, occ_beta, + append_ss_doubles_asci_contributions( + coeff, state, state_alpha, state_beta, occ_alpha, vir_alpha, occ_beta, eps_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); // Doubles - BBBB - append_ss_doubles_asci_contributions( - coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, + append_ss_doubles_asci_contributions( + coeff, state, state_beta, state_alpha, occ_beta, vir_beta, occ_alpha, eps_beta.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); @@ -335,16 +335,17 @@ asci_contrib_container> asci_contributions_constraint( const auto& eps_beta = bcd.orb_ens_beta; const auto state = det | beta; - const auto state_beta = bitset_hi_word(beta); + const auto state_alpha = alpha_string(state); + const auto state_beta = beta_string(beta); // BB Excitations - append_singles_asci_contributions<(N / 2), (N / 2)>( + append_singles_asci_contributions( coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, eps_beta.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); // BBBB Excitations - append_ss_doubles_asci_contributions( - coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, + append_ss_doubles_asci_contributions( + coeff, state, state_beta, state_alpha, occ_beta, vir_beta, occ_alpha, eps_beta.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); diff --git a/include/macis/asci/pt2.hpp b/include/macis/asci/pt2.hpp index 2ddd927a..b4592d62 100644 --- a/include/macis/asci/pt2.hpp +++ b/include/macis/asci/pt2.hpp @@ -190,16 +190,17 @@ double asci_pt2_constraint( const auto& eps_beta = bcd.orb_ens_beta; const auto state = det | beta; - const auto state_beta = bitset_hi_word(beta); + const auto state_alpha = alpha_string(state); + const auto state_beta = beta_string(beta); // BB Excitations - append_singles_asci_contributions<(N / 2), (N / 2)>( + append_singles_asci_contributions( coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, eps_beta.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); // BBBB Excitations - append_ss_doubles_asci_contributions( - coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, + append_ss_doubles_asci_contributions( + coeff, state, state_beta, state_alpha, occ_beta, vir_beta, occ_alpha, eps_beta.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); diff --git a/include/macis/sd_operations.hpp b/include/macis/sd_operations.hpp index 77150990..26a12a28 100644 --- a/include/macis/sd_operations.hpp +++ b/include/macis/sd_operations.hpp @@ -64,6 +64,7 @@ void bitset_to_occ_vir(size_t norb, std::bitset state, template struct spin_wavefunction_type; + template struct spin_wavefunction_type> { using type = std::bitset; @@ -71,6 +72,11 @@ struct spin_wavefunction_type> { template using spin_wfn_t = typename spin_wavefunction_type::type; +enum class Spin { + Alpha, + Beta +}; + template auto create_no_check(std::bitset state, unsigned p) { return state.flip(p); @@ -81,11 +87,29 @@ auto single_excitation(std::bitset state, unsigned p, unsigned q) { return state.flip(p).flip(q); } +template +auto single_excitation_spin(std::bitset state, unsigned p, unsigned q) { + static_assert(N%2 == 0, "Num Bits Must Be Even"); + if constexpr (Sigma == Spin::Alpha) + return single_excitation(state,p,q); + else + return single_excitation(state,p+N/2,q+N/2); +} + template auto double_excitation(std::bitset state, unsigned p, unsigned q, unsigned r, unsigned s) { return state.flip(p).flip(q).flip(r).flip(s); } +template +auto double_excitation_spin(std::bitset state, unsigned p, unsigned q, unsigned r, unsigned s) { + static_assert(N%2 == 0, "Num Bits Must Be Even"); + if constexpr (Sigma == Spin::Alpha) + return double_excitation(state,p,q,r,s); + else + return double_excitation(state,p+N/2,q+N/2,r+N/2,s+N/2); +} + template auto alpha_string(std::bitset state) { return bitset_lo_word(state); } template @@ -97,6 +121,14 @@ std::bitset<2*N> from_spin(std::bitset alpha, std::bitset beta) { return alpha_expand | beta_expand; } +template +auto from_spin_safe(SpinWfnType s1, SpinWfnType s2) { + if constexpr (Sigma == Spin::Alpha) + return from_spin(s1,s2); + else + return from_spin(s2,s1); +} + // TODO: Test this function template diff --git a/tests/asci.cxx b/tests/asci.cxx index 560bc149..a6eb65b7 100644 --- a/tests/asci.cxx +++ b/tests/asci.cxx @@ -13,6 +13,7 @@ #include #include #include +#include #include #include #include @@ -254,8 +255,8 @@ TEST_CASE("ASCI") { asci_settings, mcscf_settings, E0, std::move(dets), std::move(C), ham_gen, norb MACIS_MPI_CODE(, MPI_COMM_WORLD)); - std::cout << E0 - -8.542926243842e+01 << std::endl; - REQUIRE(E0 == Approx(-8.542926243842e+01)); + //std::cout << E0 - -8.542926243842e+01 << std::endl; + REQUIRE(std::abs(E0 - -8.542926243842e+01) < 1e-11); REQUIRE(dets.size() == 10000); REQUIRE(C.size() == 10000); REQUIRE(std::inner_product(C.begin(), C.end(), C.begin(), 0.0) == @@ -266,12 +267,21 @@ TEST_CASE("ASCI") { asci_settings, mcscf_settings, E0, std::move(dets), std::move(C), ham_gen, norb MACIS_MPI_CODE(, MPI_COMM_WORLD)); - REQUIRE(E0 == Approx(-8.542925964708e+01)); + REQUIRE(std::abs(E0 - -8.542925964708e+01) < 1e-11); REQUIRE(dets.size() == 10000); REQUIRE(C.size() == 10000); REQUIRE(std::inner_product(C.begin(), C.end(), C.begin(), 0.0) == Approx(1.0)); + // ASCI-PT2 + auto EPT2 = macis::asci_pt2_constraint( dets.begin(), dets.end(), E0, C, norb, + ham_gen.T(), ham_gen.G_red(), ham_gen.V_red(),ham_gen.G(), ham_gen.V(), + ham_gen MACIS_MPI_CODE(, MPI_COMM_WORLD)); + + std::cout << std::scientific << std::setprecision(12); + std::cout << EPT2 << std::endl; + REQUIRE(std::abs(EPT2 - -5.701585096318e-03) < 1e-10); + MACIS_MPI_CODE(MPI_Barrier(MPI_COMM_WORLD);) spdlog::drop_all(); } From e17fc9db6c0fd30e1ec769534276206864bc676c Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Fri, 8 Sep 2023 12:21:10 -0700 Subject: [PATCH 16/73] First attempt at wfn-generic constraint code --- include/macis/asci/determinant_search.hpp | 6 +-- include/macis/asci/mask_constraints.hpp | 58 ++++++++++++----------- include/macis/asci/pt2.hpp | 6 +-- 3 files changed, 36 insertions(+), 34 deletions(-) diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index 7037dc39..83cf37ad 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -290,7 +290,7 @@ asci_contrib_container> asci_contributions_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_singles_contributions_ss( - coeff, det, C, O, B, beta, occ_alpha, occ_beta, + coeff, det|beta, C, O, B, occ_alpha, occ_beta, orb_ens_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -303,7 +303,7 @@ asci_contrib_container> asci_contributions_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_doubles_contributions_ss( - coeff, det, C, O, B, beta, occ_alpha, occ_beta, + coeff, det|beta, C, O, B, occ_alpha, occ_beta, orb_ens_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -318,7 +318,7 @@ asci_contrib_container> asci_contributions_constraint( const auto& orb_ens_alpha = bcd.orb_ens_alpha; const auto& orb_ens_beta = bcd.orb_ens_beta; generate_constraint_doubles_contributions_os( - coeff, det, C, O, B, beta, occ_alpha, occ_beta, vir_beta, + coeff, det|beta, C, O, B, occ_alpha, occ_beta, vir_beta, orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index 50472f62..b1a18f58 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -240,16 +240,16 @@ size_t constraint_histogram(wfn_t det, size_t n_os_singles, return ndet; } -template +template void generate_constraint_singles_contributions_ss( - double coeff, wfn_t det, wfn_t T, wfn_t O, wfn_t B, - wfn_t os_det, const std::vector& occ_same, + double coeff, WfnType det, WfnType T, WfnType O, WfnType B, + const std::vector& occ_same, const std::vector& occ_othr, const double* eps, const double* T_pq, const size_t LDT, const double* G_kpq, const size_t LDG, const double* V_kpq, const size_t LDV, double h_el_tol, double root_diag, - double E0, HamiltonianGenerator>& ham_gen, - asci_contrib_container>& asci_contributions) { - auto [o, v] = generate_constraint_single_excitations(det, T, O, B); + double E0, HamiltonianGeneratorBase& ham_gen, + asci_contrib_container& asci_contributions) { + auto [o, v] = generate_constraint_single_excitations(alpha_string(det), alpha_string(T), alpha_string(O), alpha_string(B)); const auto no = o.count(); const auto nv = v.count(); if(!no or !nv) return; @@ -274,8 +274,8 @@ void generate_constraint_singles_contributions_ss( if(std::abs(coeff * h_el) < h_el_tol) continue; // Calculate Excited Determinant - auto ex_det = det | os_det; - ex_det.flip(i).flip(a); + auto ex_det = single_excitation_spin(det, i, a ); + // Compute Sign in a Canonical Way auto sign = single_excitation_sign(det, a, i); @@ -290,15 +290,15 @@ void generate_constraint_singles_contributions_ss( } } -template +template void generate_constraint_doubles_contributions_ss( - double coeff, wfn_t det, wfn_t T, wfn_t O_mask, wfn_t B, - wfn_t os_det, const std::vector& occ_same, + double coeff, WfnType det, WfnType T, WfnType O_mask, WfnType B, + const std::vector& occ_same, const std::vector& occ_othr, const double* eps, const double* G, const size_t LDG, double h_el_tol, double root_diag, double E0, - HamiltonianGenerator>& ham_gen, - asci_contrib_container>& asci_contributions) { - auto [O, V] = generate_constraint_double_excitations(det, T, O_mask, B); + HamiltonianGeneratorBase& ham_gen, + asci_contrib_container& asci_contributions) { + auto [O, V] = generate_constraint_double_excitations(alpha_string(det), alpha_string(T), alpha_string(O_mask), alpha_string(B)); const auto no_pairs = O.size(); const auto nv_pairs = V.size(); if(!no_pairs or !nv_pairs) return; @@ -309,7 +309,7 @@ void generate_constraint_doubles_contributions_ss( const auto i = ffs(ij) - 1; const auto j = fls(ij); const auto G_ij = G + (j + i * LDG2) * LDG; - const auto ex_ij = det ^ ij; + const auto ex_ij = single_excitation_spin(det,i,j); // det ^ ij; for(int _ab = 0; _ab < nv_pairs; ++_ab) { const auto ab = V[_ab]; const auto a = ffs(ab) - 1; @@ -321,14 +321,14 @@ void generate_constraint_doubles_contributions_ss( if(std::abs(coeff * G_aibj) < h_el_tol) continue; // Calculate Excited Determinant (spin) - const auto full_ex_spin = ij | ab; - const auto ex_det_spin = ex_ij | ab; + const auto full_ex_spin = single_excitation_spin(ij,a,b); // ij | ab; + const auto ex_det_spin = single_excitation_spin(ex_ij,a,b); // ex_ij | ab; // Compute Sign in a Canonical Way - auto sign = doubles_sign(det, ex_det_spin, full_ex_spin); + auto sign = doubles_sign(alpha_string(det), alpha_string(ex_det_spin), full_ex_spin); // Calculate Full Excited Determinant - const auto full_ex = ex_det_spin | os_det; + const auto full_ex = ex_det_spin;// | os_det; // Update Sign of Matrix Element auto h_el = sign * G_aibj; @@ -343,17 +343,17 @@ void generate_constraint_doubles_contributions_ss( } } -template +template void generate_constraint_doubles_contributions_os( - double coeff, wfn_t det, wfn_t T, wfn_t O, wfn_t B, - wfn_t os_det, const std::vector& occ_same, + double coeff, WfnType det, WfnType T, WfnType O, WfnType B, + const std::vector& occ_same, const std::vector& occ_othr, const std::vector& vir_othr, const double* eps_same, const double* eps_othr, const double* V, const size_t LDV, double h_el_tol, - double root_diag, double E0, HamiltonianGenerator>& ham_gen, - asci_contrib_container>& asci_contributions) { + double root_diag, double E0, HamiltonianGeneratorBase& ham_gen, + asci_contrib_container& asci_contributions) { // Generate Single Excitations that Satisfy the Constraint - auto [o, v] = generate_constraint_single_excitations(det, T, O, B); + auto [o, v] = generate_constraint_single_excitations(alpha_string(det), alpha_string(T), alpha_string(O), alpha_string(B)); const auto no = o.count(); const auto nv = v.count(); if(!no or !nv) return; @@ -381,12 +381,14 @@ void generate_constraint_doubles_contributions_os( // double sign_othr = single_excitation_sign( os_det >> (N/2), b, j // ); double sign_othr = - single_excitation_sign(bitset_hi_word(os_det), b, j); + single_excitation_sign(beta_string(det), b, j); double sign = sign_same * sign_othr; // Compute Excited Determinant - auto ex_det = det | os_det; - ex_det.flip(i).flip(a).flip(j + N / 2).flip(b + N / 2); + //auto ex_det = det | os_det; + //ex_det.flip(i).flip(a).flip(j + N / 2).flip(b + N / 2); + auto ex_det = single_excitation_spin(det,i,a); + ex_det = single_excitation_spin(ex_det,j,b); // Finalize Matrix Element auto h_el = sign * V_aibj; diff --git a/include/macis/asci/pt2.hpp b/include/macis/asci/pt2.hpp index b4592d62..354a42e5 100644 --- a/include/macis/asci/pt2.hpp +++ b/include/macis/asci/pt2.hpp @@ -145,7 +145,7 @@ double asci_pt2_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_singles_contributions_ss( - coeff, det, C, O, B, beta, occ_alpha, occ_beta, + coeff, det|beta, C, O, B, occ_alpha, occ_beta, orb_ens_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -158,7 +158,7 @@ double asci_pt2_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_doubles_contributions_ss( - coeff, det, C, O, B, beta, occ_alpha, occ_beta, + coeff, det|beta, C, O, B, occ_alpha, occ_beta, orb_ens_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -173,7 +173,7 @@ double asci_pt2_constraint( const auto& orb_ens_alpha = bcd.orb_ens_alpha; const auto& orb_ens_beta = bcd.orb_ens_beta; generate_constraint_doubles_contributions_os( - coeff, det, C, O, B, beta, occ_alpha, occ_beta, vir_beta, + coeff, det|beta, C, O, B, occ_alpha, occ_beta, vir_beta, orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } From e80b9d2ca18ca6def7e7b7518a55352d054822f8 Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Mon, 11 Sep 2023 09:32:47 -0700 Subject: [PATCH 17/73] Introduce wavefunction_traits, move most bitset-specific logic into template specialization --- .../macis/asci/determinant_contributions.hpp | 14 +- include/macis/asci/determinant_search.hpp | 24 +- include/macis/asci/mask_constraints.hpp | 26 +- include/macis/asci/pt2.hpp | 11 +- .../hamiltonian_generator/double_loop.hpp | 38 +-- .../hamiltonian_generator/matrix_elements.hpp | 14 +- include/macis/sd_operations.hpp | 276 +++++++----------- include/macis/util/rdms.hpp | 5 +- include/macis/util/unused_untested.hpp | 44 +++ include/macis/wfn/raw_bitset.hpp | 127 ++++++++ tests/asci.cxx | 8 +- tests/csr_hamiltonian.cxx | 12 +- tests/davidson.cxx | 12 +- tests/double_loop.cxx | 24 +- tests/sd_operations.cxx | 62 ++-- tests/standalone_driver.cxx | 3 +- 16 files changed, 430 insertions(+), 270 deletions(-) create mode 100644 include/macis/wfn/raw_bitset.hpp diff --git a/include/macis/asci/determinant_contributions.hpp b/include/macis/asci/determinant_contributions.hpp index 9853ff74..89a76610 100644 --- a/include/macis/asci/determinant_contributions.hpp +++ b/include/macis/asci/determinant_contributions.hpp @@ -36,6 +36,7 @@ void append_singles_asci_contributions( const double* V_kpq, const size_t LDV, double h_el_tol, double root_diag, double E0, const HamiltonianGeneratorBase& ham_gen, asci_contrib_container& asci_contributions) { + using wfn_traits = wavefunction_traits; const auto LDG2 = LDG * LDG; const auto LDV2 = LDV * LDV; for(auto i : occ_same) @@ -51,7 +52,7 @@ void append_singles_asci_contributions( if(std::abs(h_el) < h_el_tol) continue; // Calculate Excited Determinant - auto ex_det = single_excitation_spin(state_full, i, a); + auto ex_det = wfn_traits::template single_excitation_no_check(state_full, i, a); // Calculate Excitation Sign in a Canonical Way auto sign = single_excitation_sign(state_same, a, i); @@ -77,6 +78,8 @@ void append_ss_doubles_asci_contributions( const double* G, size_t LDG, double h_el_tol, double root_diag, double E0, const HamiltonianGeneratorBase& ham_gen, asci_contrib_container& asci_contributions) { + using wfn_traits = wavefunction_traits; + using spin_wfn_traits = wavefunction_traits; const size_t nocc = ss_occ.size(); const size_t nvir = vir.size(); @@ -111,14 +114,14 @@ void append_ss_doubles_asci_contributions( // TODO: Can this be made faster since the orbital indices are known // in advance? // Compute excited determinant (spin) - const auto full_ex_spin = double_excitation(SpinWfnType(0), i,j,a,b); + const auto full_ex_spin = spin_wfn_traits::double_excitation_no_check(SpinWfnType(0), i,j,a,b); const auto ex_det_spin = state_same ^ full_ex_spin; // Calculate the sign in a canonical way double sign = doubles_sign(state_same, ex_det_spin, full_ex_spin); // Calculate full excited determinant - auto ex_det = from_spin_safe(ex_det_spin, state_other); + auto ex_det = wfn_traits::template from_spin(ex_det_spin, state_other); #endif // Update sign of matrix element @@ -147,6 +150,7 @@ void append_os_doubles_asci_contributions( const double* eps_beta, const double* V, size_t LDV, double h_el_tol, double root_diag, double E0, const HamiltonianGeneratorBase& ham_gen, asci_contrib_container& asci_contributions) { + using wfn_traits = wavefunction_traits; const size_t LDV2 = LDV * LDV; for(auto i : occ_alpha) for(auto a : vir_alpha) { @@ -164,8 +168,8 @@ void append_os_doubles_asci_contributions( double sign = sign_alpha * sign_beta; //auto ex_det = state_full; //ex_det.flip(a).flip(i).flip(j + N).flip(b + N); - auto ex_det = single_excitation_spin(state_full, a, i); - ex_det = single_excitation_spin(ex_det, b, j); + auto ex_det = wfn_traits::template single_excitation_no_check(state_full, a, i); + ex_det = wfn_traits::template single_excitation_no_check(ex_det, b, j); auto h_el = sign * V_aibj; // Evaluate fast diagonal element diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index 83cf37ad..8fd017fd 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -57,6 +57,9 @@ asci_contrib_container> asci_contributions_standard( const std::vector& C, size_t norb, const double* T_pq, const double* G_red, const double* V_red, const double* G_pqrs, const double* V_pqrs, HamiltonianGenerator>& ham_gen) { + using wfn_traits = wavefunction_traits>; + using spin_wfn_type = spin_wfn_t>; + using spin_wfn_traits = wavefunction_traits; auto logger = spdlog::get("asci_search"); const size_t ncdets = std::distance(cdets_begin, cdets_end); @@ -68,13 +71,13 @@ asci_contrib_container> asci_contributions_standard( for(size_t i = 0; i < ncdets; ++i) { // Alias state data auto state = *(cdets_begin + i); - auto state_alpha = bitset_lo_word(state); - auto state_beta = bitset_hi_word(state); + auto state_alpha = wfn_traits::alpha_string(state); + auto state_beta = wfn_traits::beta_string(state); auto coeff = C[i]; // Get occupied and virtual indices - bitset_to_occ_vir(norb, state_alpha, occ_alpha, vir_alpha); - bitset_to_occ_vir(norb, state_beta, occ_beta, vir_beta); + spin_wfn_traits::state_to_occ_vir(norb, state_alpha, occ_alpha, vir_alpha); + spin_wfn_traits::state_to_occ_vir(norb, state_beta, occ_beta, vir_beta); // Precompute orbital energies auto eps_alpha = ham_gen.single_orbital_ens(norb, occ_alpha, occ_beta); @@ -150,6 +153,9 @@ asci_contrib_container> asci_contributions_constraint( const double* V_pqrs, HamiltonianGenerator>& ham_gen, MPI_Comm comm) { using clock_type = std::chrono::high_resolution_clock; using duration_type = std::chrono::duration; + using wfn_traits = wavefunction_traits>; + using spin_wfn_type = spin_wfn_t>; + using spin_wfn_traits = wavefunction_traits; auto logger = spdlog::get("asci_search"); const size_t ncdets = std::distance(cdets_begin, cdets_end); @@ -195,7 +201,7 @@ asci_contrib_container> asci_contributions_constraint( h_diag = ham_gen.matrix_element(w, w); // Compute occ/vir for beta string - bitset_to_occ_vir(norb, beta_shift, occ_beta, vir_beta); + wfn_traits::state_to_occ_vir(norb, beta_shift, occ_beta, vir_beta); // Precompute orbital energies orb_ens_alpha = ham_gen.single_orbital_ens(norb, occ_alpha, occ_beta); @@ -211,7 +217,7 @@ asci_contrib_container> asci_contributions_constraint( for(auto i = 0; i < nuniq_alpha; ++i) { const auto wfn_a = uniq_alpha_wfn[i]; std::vector occ_alpha, vir_alpha; - bitset_to_occ_vir(norb, wfn_a, occ_alpha, vir_alpha); + wfn_traits::state_to_occ_vir(norb, wfn_a, occ_alpha, vir_alpha); for(auto j = 0; j < ncdets; ++j) { const auto w = *(cdets_begin + j); if((w & full_mask()) == wfn_a) { @@ -223,7 +229,7 @@ asci_contrib_container> asci_contributions_constraint( auto world_rank = comm_rank(comm); auto world_size = comm_size(comm); - const auto n_occ_alpha = uniq_alpha_wfn[0].count(); + const auto n_occ_alpha = wfn_traits::count(uniq_alpha_wfn[0]); const auto n_vir_alpha = norb - n_occ_alpha; const auto n_sing_alpha = n_occ_alpha * n_vir_alpha; const auto n_doub_alpha = (n_sing_alpha * (n_sing_alpha - norb + 1)) / 4; @@ -335,8 +341,8 @@ asci_contrib_container> asci_contributions_constraint( const auto& eps_beta = bcd.orb_ens_beta; const auto state = det | beta; - const auto state_alpha = alpha_string(state); - const auto state_beta = beta_string(beta); + const auto state_alpha = wfn_traits::alpha_string(state); + const auto state_beta = wfn_traits::beta_string(beta); // BB Excitations append_singles_asci_contributions( coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index b1a18f58..a02a3479 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -249,7 +249,8 @@ void generate_constraint_singles_contributions_ss( const double* V_kpq, const size_t LDV, double h_el_tol, double root_diag, double E0, HamiltonianGeneratorBase& ham_gen, asci_contrib_container& asci_contributions) { - auto [o, v] = generate_constraint_single_excitations(alpha_string(det), alpha_string(T), alpha_string(O), alpha_string(B)); + using wfn_traits = wavefunction_traits; + auto [o, v] = generate_constraint_single_excitations(wfn_traits::alpha_string(det), wfn_traits::alpha_string(T), wfn_traits::alpha_string(O), wfn_traits::alpha_string(B)); const auto no = o.count(); const auto nv = v.count(); if(!no or !nv) return; @@ -274,7 +275,7 @@ void generate_constraint_singles_contributions_ss( if(std::abs(coeff * h_el) < h_el_tol) continue; // Calculate Excited Determinant - auto ex_det = single_excitation_spin(det, i, a ); + auto ex_det = wfn_traits::template single_excitation_no_check(det, i, a ); // Compute Sign in a Canonical Way @@ -298,7 +299,9 @@ void generate_constraint_doubles_contributions_ss( const size_t LDG, double h_el_tol, double root_diag, double E0, HamiltonianGeneratorBase& ham_gen, asci_contrib_container& asci_contributions) { - auto [O, V] = generate_constraint_double_excitations(alpha_string(det), alpha_string(T), alpha_string(O_mask), alpha_string(B)); + using wfn_traits = wavefunction_traits; + using spin_wfn_traits = wavefunction_traits>; + auto [O, V] = generate_constraint_double_excitations(wfn_traits::alpha_string(det), wfn_traits::alpha_string(T), wfn_traits::alpha_string(O_mask), wfn_traits::alpha_string(B)); const auto no_pairs = O.size(); const auto nv_pairs = V.size(); if(!no_pairs or !nv_pairs) return; @@ -309,7 +312,7 @@ void generate_constraint_doubles_contributions_ss( const auto i = ffs(ij) - 1; const auto j = fls(ij); const auto G_ij = G + (j + i * LDG2) * LDG; - const auto ex_ij = single_excitation_spin(det,i,j); // det ^ ij; + const auto ex_ij = wfn_traits::template single_excitation_no_check(det,i,j); // det ^ ij; for(int _ab = 0; _ab < nv_pairs; ++_ab) { const auto ab = V[_ab]; const auto a = ffs(ab) - 1; @@ -321,11 +324,11 @@ void generate_constraint_doubles_contributions_ss( if(std::abs(coeff * G_aibj) < h_el_tol) continue; // Calculate Excited Determinant (spin) - const auto full_ex_spin = single_excitation_spin(ij,a,b); // ij | ab; - const auto ex_det_spin = single_excitation_spin(ex_ij,a,b); // ex_ij | ab; + const auto full_ex_spin = spin_wfn_traits::template single_excitation_no_check(ij,a,b); // ij | ab; + const auto ex_det_spin = wfn_traits::template single_excitation_no_check(ex_ij,a,b); // ex_ij | ab; // Compute Sign in a Canonical Way - auto sign = doubles_sign(alpha_string(det), alpha_string(ex_det_spin), full_ex_spin); + auto sign = doubles_sign(wfn_traits::alpha_string(det), wfn_traits::alpha_string(ex_det_spin), full_ex_spin); // Calculate Full Excited Determinant const auto full_ex = ex_det_spin;// | os_det; @@ -352,8 +355,9 @@ void generate_constraint_doubles_contributions_os( const double* eps_othr, const double* V, const size_t LDV, double h_el_tol, double root_diag, double E0, HamiltonianGeneratorBase& ham_gen, asci_contrib_container& asci_contributions) { + using wfn_traits = wavefunction_traits; // Generate Single Excitations that Satisfy the Constraint - auto [o, v] = generate_constraint_single_excitations(alpha_string(det), alpha_string(T), alpha_string(O), alpha_string(B)); + auto [o, v] = generate_constraint_single_excitations(wfn_traits::alpha_string(det), wfn_traits::alpha_string(T), wfn_traits::alpha_string(O), wfn_traits::alpha_string(B)); const auto no = o.count(); const auto nv = v.count(); if(!no or !nv) return; @@ -381,14 +385,14 @@ void generate_constraint_doubles_contributions_os( // double sign_othr = single_excitation_sign( os_det >> (N/2), b, j // ); double sign_othr = - single_excitation_sign(beta_string(det), b, j); + single_excitation_sign(wfn_traits::beta_string(det), b, j); double sign = sign_same * sign_othr; // Compute Excited Determinant //auto ex_det = det | os_det; //ex_det.flip(i).flip(a).flip(j + N / 2).flip(b + N / 2); - auto ex_det = single_excitation_spin(det,i,a); - ex_det = single_excitation_spin(ex_det,j,b); + auto ex_det = wfn_traits::template single_excitation_no_check(det,i,a); + ex_det = wfn_traits::template single_excitation_no_check(ex_det,j,b); // Finalize Matrix Element auto h_el = sign * V_aibj; diff --git a/include/macis/asci/pt2.hpp b/include/macis/asci/pt2.hpp index 354a42e5..0610a0af 100644 --- a/include/macis/asci/pt2.hpp +++ b/include/macis/asci/pt2.hpp @@ -23,6 +23,7 @@ double asci_pt2_constraint( using clock_type = std::chrono::high_resolution_clock; using duration_type = std::chrono::duration; + using wfn_traits = wavefunction_traits>; auto logger = spdlog::get("asci_search"); const size_t ncdets = std::distance(cdets_begin, cdets_end); @@ -69,7 +70,7 @@ double asci_pt2_constraint( h_diag = ham_gen.matrix_element(w, w); // Compute occ/vir for beta string - bitset_to_occ_vir(norb, beta_shift, occ_beta, vir_beta); + wfn_traits::state_to_occ_vir(norb, beta_shift, occ_beta, vir_beta); // Precompute orbital energies orb_ens_alpha = ham_gen.single_orbital_ens(norb, occ_alpha, occ_beta); @@ -85,7 +86,7 @@ double asci_pt2_constraint( for(auto i = 0; i < nuniq_alpha; ++i) { const auto wfn_a = uniq_alpha_wfn[i]; std::vector occ_alpha, vir_alpha; - bitset_to_occ_vir(norb, wfn_a, occ_alpha, vir_alpha); + wfn_traits::state_to_occ_vir(norb, wfn_a, occ_alpha, vir_alpha); for(auto j = 0; j < ncdets; ++j) { const auto w = *(cdets_begin + j); if((w & full_mask()) == wfn_a) { @@ -97,7 +98,7 @@ double asci_pt2_constraint( auto world_rank = comm_rank(comm); auto world_size = comm_size(comm); - const auto n_occ_alpha = uniq_alpha_wfn[0].count(); + const auto n_occ_alpha = wfn_traits::count(uniq_alpha_wfn[0]); const auto n_vir_alpha = norb - n_occ_alpha; const auto n_sing_alpha = n_occ_alpha * n_vir_alpha; const auto n_doub_alpha = (n_sing_alpha * (n_sing_alpha - norb + 1)) / 4; @@ -190,8 +191,8 @@ double asci_pt2_constraint( const auto& eps_beta = bcd.orb_ens_beta; const auto state = det | beta; - const auto state_alpha = alpha_string(state); - const auto state_beta = beta_string(beta); + const auto state_alpha = wfn_traits::alpha_string(state); + const auto state_beta = wfn_traits::beta_string(beta); // BB Excitations append_singles_asci_contributions( coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, diff --git a/include/macis/hamiltonian_generator/double_loop.hpp b/include/macis/hamiltonian_generator/double_loop.hpp index 7f00f053..fe2f85d0 100644 --- a/include/macis/hamiltonian_generator/double_loop.hpp +++ b/include/macis/hamiltonian_generator/double_loop.hpp @@ -31,6 +31,7 @@ class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { sparse_matrix_type make_csr_hamiltonian_block_( full_det_iterator bra_begin, full_det_iterator bra_end, full_det_iterator ket_begin, full_det_iterator ket_end, double H_thresh) { + using wfn_traits = wavefunction_traits; const size_t nbra_dets = std::distance(bra_begin, bra_end); const size_t nket_dets = std::distance(ket_begin, ket_end); @@ -47,10 +48,10 @@ class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { const auto bra = *(bra_begin + i); size_t nrow = 0; - if(bra.count()) { + if(wfn_traits::count(bra)) { // Separate out into alpha/beta components - spin_det_t bra_alpha = alpha_string(bra); - spin_det_t bra_beta = beta_string(bra); + spin_det_t bra_alpha = wfn_traits::alpha_string(bra); + spin_det_t bra_beta = wfn_traits::beta_string(bra); // Get occupied indices bits_to_indices(bra_alpha, bra_occ_alpha); @@ -59,14 +60,14 @@ class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { // Loop over ket determinants for(size_t j = 0; j < nket_dets; ++j) { const auto ket = *(ket_begin + j); - if(ket.count()) { - spin_det_t ket_alpha = alpha_string(ket); - spin_det_t ket_beta = beta_string(ket); + if(wfn_traits::count(ket)) { + spin_det_t ket_alpha = wfn_traits::alpha_string(ket); + spin_det_t ket_beta = wfn_traits::beta_string(ket); full_det_t ex_total = bra ^ ket; - if(ex_total.count() <= 4) { - spin_det_t ex_alpha = alpha_string(ex_total); - spin_det_t ex_beta = beta_string(ex_total); + if(wfn_traits::count(ex_total) <= 4) { + spin_det_t ex_alpha = wfn_traits::alpha_string(ex_total); + spin_det_t ex_beta = wfn_traits::beta_string(ex_total); // Compute Matrix Element const auto h_el = this->matrix_element( @@ -117,6 +118,7 @@ class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { void form_rdms(full_det_iterator bra_begin, full_det_iterator bra_end, full_det_iterator ket_begin, full_det_iterator ket_end, double *C, matrix_span_t ordm, rank4_span_t trdm) override { + using wfn_traits = wavefunction_traits; const size_t nbra_dets = std::distance(bra_begin, bra_end); const size_t nket_dets = std::distance(ket_begin, ket_end); @@ -126,10 +128,10 @@ class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { for(size_t i = 0; i < nbra_dets; ++i) { const auto bra = *(bra_begin + i); // if( (i%1000) == 0 ) std::cout << i << std::endl; - if(bra.count()) { + if(wfn_traits::count(bra)) { // Separate out into alpha/beta components - spin_det_t bra_alpha = alpha_string(bra); - spin_det_t bra_beta = beta_string(bra); + spin_det_t bra_alpha = wfn_traits::alpha_string(bra); + spin_det_t bra_beta = wfn_traits::beta_string(bra); // Get occupied indices bits_to_indices(bra_alpha, bra_occ_alpha); @@ -138,14 +140,14 @@ class DoubleLoopHamiltonianGenerator : public HamiltonianGenerator { // Loop over ket determinants for(size_t j = 0; j < nket_dets; ++j) { const auto ket = *(ket_begin + j); - if(ket.count()) { - spin_det_t ket_alpha = alpha_string(ket); - spin_det_t ket_beta = beta_string(ket); + if(wfn_traits::count(ket)) { + spin_det_t ket_alpha = wfn_traits::alpha_string(ket); + spin_det_t ket_beta = wfn_traits::beta_string(ket); full_det_t ex_total = bra ^ ket; - if(ex_total.count() <= 4) { - spin_det_t ex_alpha = alpha_string(ex_total); - spin_det_t ex_beta = beta_string(ex_total); + if(wfn_traits::count(ex_total) <= 4) { + spin_det_t ex_alpha = wfn_traits::alpha_string(ex_total); + spin_det_t ex_beta = wfn_traits::beta_string(ex_total); const double val = C[i] * C[j]; diff --git a/include/macis/hamiltonian_generator/matrix_elements.hpp b/include/macis/hamiltonian_generator/matrix_elements.hpp index b3be534d..f34637b6 100644 --- a/include/macis/hamiltonian_generator/matrix_elements.hpp +++ b/include/macis/hamiltonian_generator/matrix_elements.hpp @@ -14,10 +14,11 @@ namespace macis { template double HamiltonianGenerator::matrix_element(full_det_t bra, full_det_t ket) const { - auto bra_alpha = alpha_string(bra); - auto ket_alpha = alpha_string(ket); - auto bra_beta = beta_string(bra); - auto ket_beta = beta_string(ket); + using wfn_traits = wavefunction_traits; + auto bra_alpha = wfn_traits::alpha_string(bra); + auto ket_alpha = wfn_traits::alpha_string(ket); + auto bra_beta = wfn_traits::beta_string(bra); + auto ket_beta = wfn_traits::beta_string(ket); auto ex_alpha = bra_alpha ^ ket_alpha; auto ex_beta = bra_beta ^ ket_beta; @@ -35,8 +36,9 @@ double HamiltonianGenerator::matrix_element( spin_det_t bra_beta, spin_det_t ket_beta, spin_det_t ex_beta, const std::vector& bra_occ_alpha, const std::vector& bra_occ_beta) const { - const uint32_t ex_alpha_count = ex_alpha.count(); - const uint32_t ex_beta_count = ex_beta.count(); + using spin_wfn_traits = wavefunction_traits; + const uint32_t ex_alpha_count = spin_wfn_traits::count(ex_alpha); + const uint32_t ex_beta_count = spin_wfn_traits::count(ex_beta); if((ex_alpha_count + ex_beta_count) > 4) return 0.; diff --git a/include/macis/sd_operations.hpp b/include/macis/sd_operations.hpp index 26a12a28..bce84a2e 100644 --- a/include/macis/sd_operations.hpp +++ b/include/macis/sd_operations.hpp @@ -10,6 +10,7 @@ #include #include #include +#include #include namespace macis { @@ -27,13 +28,13 @@ namespace macis { * @returns The bitstring HF state consisting of the specified number of * occupied orbitals. */ -template -std::bitset canonical_hf_determinant(uint32_t nalpha, uint32_t nbeta) { - static_assert((N % 2) == 0, "N Must Be Even"); - std::bitset alpha = full_mask(nalpha); - std::bitset beta = full_mask(nbeta) << (N / 2); - return alpha | beta; -} +//template +//std::bitset canonical_hf_determinant(uint32_t nalpha, uint32_t nbeta) { +// static_assert((N % 2) == 0, "N Must Be Even"); +// std::bitset alpha = full_mask(nalpha); +// std::bitset beta = full_mask(nbeta) << (N / 2); +// return alpha | beta; +//} /** @@ -45,89 +46,51 @@ std::bitset canonical_hf_determinant(uint32_t nalpha, uint32_t nbeta) { * @param[out] occ List of occupied orbitals in `state` * @param[out] vir List of unoccupied orbitals in `state` */ -template -void bitset_to_occ_vir(size_t norb, std::bitset state, - std::vector& occ, std::vector& vir) { - occ = bits_to_indices(state); - const auto nocc = occ.size(); - assert(nocc < norb); - - const auto nvir = norb - nocc; - vir.resize(nvir); - state = ~state; - for(int i = 0; i < nvir; ++i) { - auto a = ffs(state) - 1; - vir[i] = a; - state.flip(a); - } -} - -template -struct spin_wavefunction_type; - -template -struct spin_wavefunction_type> { - using type = std::bitset; -}; -template -using spin_wfn_t = typename spin_wavefunction_type::type; - -enum class Spin { - Alpha, - Beta -}; - -template -auto create_no_check(std::bitset state, unsigned p) { - return state.flip(p); -} - -template -auto single_excitation(std::bitset state, unsigned p, unsigned q) { - return state.flip(p).flip(q); -} - -template -auto single_excitation_spin(std::bitset state, unsigned p, unsigned q) { - static_assert(N%2 == 0, "Num Bits Must Be Even"); - if constexpr (Sigma == Spin::Alpha) - return single_excitation(state,p,q); - else - return single_excitation(state,p+N/2,q+N/2); -} - -template -auto double_excitation(std::bitset state, unsigned p, unsigned q, unsigned r, unsigned s) { - return state.flip(p).flip(q).flip(r).flip(s); -} - -template -auto double_excitation_spin(std::bitset state, unsigned p, unsigned q, unsigned r, unsigned s) { - static_assert(N%2 == 0, "Num Bits Must Be Even"); - if constexpr (Sigma == Spin::Alpha) - return double_excitation(state,p,q,r,s); - else - return double_excitation(state,p+N/2,q+N/2,r+N/2,s+N/2); -} - -template -auto alpha_string(std::bitset state) { return bitset_lo_word(state); } -template -auto beta_string(std::bitset state) { return bitset_hi_word(state); } -template -std::bitset<2*N> from_spin(std::bitset alpha, std::bitset beta) { - auto alpha_expand = expand_bitset<2*N>(alpha); - auto beta_expand = expand_bitset<2*N>(beta) << N; - return alpha_expand | beta_expand; -} - -template -auto from_spin_safe(SpinWfnType s1, SpinWfnType s2) { - if constexpr (Sigma == Spin::Alpha) - return from_spin(s1,s2); - else - return from_spin(s2,s1); -} +//template +//void bitset_to_occ_vir(size_t norb, std::bitset state, +// std::vector& occ, std::vector& vir) { +// occ = bits_to_indices(state); +// const auto nocc = occ.size(); +// assert(nocc < norb); +// +// const auto nvir = norb - nocc; +// vir.resize(nvir); +// state = ~state; +// for(int i = 0; i < nvir; ++i) { +// auto a = ffs(state) - 1; +// vir[i] = a; +// state.flip(a); +// } +//} + + +//template +//auto single_excitation(std::bitset state, unsigned p, unsigned q) { +// return state.flip(p).flip(q); +//} + +//template +//auto single_excitation_spin(std::bitset state, unsigned p, unsigned q) { +// static_assert(N%2 == 0, "Num Bits Must Be Even"); +// if constexpr (Sigma == Spin::Alpha) +// return single_excitation(state,p,q); +// else +// return single_excitation(state,p+N/2,q+N/2); +//} + +//template +//auto double_excitation(std::bitset state, unsigned p, unsigned q, unsigned r, unsigned s) { +// return state.flip(p).flip(q).flip(r).flip(s); +//} + +//template +//auto double_excitation_spin(std::bitset state, unsigned p, unsigned q, unsigned r, unsigned s) { +// static_assert(N%2 == 0, "Num Bits Must Be Even"); +// if constexpr (Sigma == Spin::Alpha) +// return double_excitation(state,p,q,r,s); +// else +// return double_excitation(state,p+N/2,q+N/2,r+N/2,s+N/2); +//} // TODO: Test this function @@ -153,6 +116,7 @@ template void append_singles(WfnType state, const std::vector& occ, const std::vector& vir, WfnContainer& singles) { + using wfn_traits = wavefunction_traits; const size_t nocc = occ.size(); const size_t nvir = vir.size(); @@ -161,7 +125,7 @@ void append_singles(WfnType state, const std::vector& occ, for(size_t a = 0; a < nvir; ++a) for(size_t i = 0; i < nocc; ++i) { - singles.emplace_back(single_excitation(state, occ[i], vir[a])); + singles.emplace_back(wfn_traits::single_excitation_no_check(state, occ[i], vir[a])); } } @@ -169,6 +133,7 @@ template void append_doubles(WfnType state, const std::vector& occ, const std::vector& vir, WfnContainer& doubles) { + using wfn_traits = wavefunction_traits; const size_t nocc = occ.size(); const size_t nvir = vir.size(); @@ -181,14 +146,15 @@ void append_doubles(WfnType state, const std::vector& occ, for(size_t i = 0; i < nocc; ++i) for(size_t b = a + 1; b < nvir; ++b) for(size_t j = i + 1; j < nocc; ++j) { - doubles.emplace_back(double_excitation(state, occ[i], occ[j], vir[a], vir[b])); + doubles.emplace_back(wfn_traits::double_excitation_no_check(state, occ[i], occ[j], vir[a], vir[b])); } } template void generate_singles(size_t norb, WfnType state, WfnContainer& singles) { + using wfn_traits = wavefunction_traits; std::vector occ_orbs, vir_orbs; - bitset_to_occ_vir(norb, state, occ_orbs, vir_orbs); + wfn_traits::state_to_occ_vir(norb, state, occ_orbs, vir_orbs); singles.clear(); append_singles(state, occ_orbs, vir_orbs, singles); @@ -196,8 +162,9 @@ void generate_singles(size_t norb, WfnType state, WfnContainer& singles) { template void generate_doubles(size_t norb, WfnType state, WfnContainer& doubles) { + using wfn_traits = wavefunction_traits; std::vector occ_orbs, vir_orbs; - bitset_to_occ_vir(norb, state, occ_orbs, vir_orbs); + wfn_traits::state_to_occ_vir(norb, state, occ_orbs, vir_orbs); doubles.clear(); append_doubles(state, occ_orbs, vir_orbs, doubles); @@ -206,8 +173,9 @@ void generate_doubles(size_t norb, WfnType state, WfnContainer& doubles) { template void generate_singles_doubles(size_t norb, WfnType state, WfnContainer& singles, WfnContainer& doubles) { + using wfn_traits = wavefunction_traits; std::vector occ_orbs, vir_orbs; - bitset_to_occ_vir(norb, state, occ_orbs, vir_orbs); + wfn_traits::state_to_occ_vir(norb, state, occ_orbs, vir_orbs); singles.clear(); doubles.clear(); @@ -219,8 +187,10 @@ void generate_singles_doubles(size_t norb, WfnType state, template void generate_singles_spin(size_t norb, WfnType state, WfnContainer& singles) { - auto state_alpha = alpha_string(state); - auto state_beta = beta_string (state); + using wfn_traits = wavefunction_traits; + + auto state_alpha = wfn_traits::alpha_string(state); + auto state_beta = wfn_traits::beta_string (state); using spin_wfn_type = spin_wfn_t; std::vector singles_alpha, singles_beta; @@ -234,12 +204,12 @@ void generate_singles_spin(size_t norb, WfnType state, WfnContainer& singles) { // Single Alpha + No Beta for(auto s_alpha : singles_alpha) { - singles.emplace_back(from_spin(s_alpha, state_beta)); + singles.emplace_back(wfn_traits::from_spin(s_alpha, state_beta)); } // No Alpha + Single Beta for(auto s_beta : singles_beta) { - singles.emplace_back(from_spin(state_alpha, s_beta)); + singles.emplace_back(wfn_traits::from_spin(state_alpha, s_beta)); } } @@ -247,8 +217,10 @@ template void generate_singles_doubles_spin(size_t norb, WfnType state, WfnContainer& singles, WfnContainer& doubles) { - auto state_alpha = alpha_string(state); - auto state_beta = beta_string (state); + using wfn_traits = wavefunction_traits; + + auto state_alpha = wfn_traits::alpha_string(state); + auto state_beta = wfn_traits::beta_string (state); using spin_wfn_type = spin_wfn_t; std::vector singles_alpha, singles_beta; @@ -264,12 +236,12 @@ void generate_singles_doubles_spin(size_t norb, WfnType state, // Single Alpha + No Beta for(auto s_alpha : singles_alpha) { - singles.emplace_back(from_spin(s_alpha, state_beta)); + singles.emplace_back(wfn_traits::from_spin(s_alpha, state_beta)); } // No Alpha + Single Beta for(auto s_beta : singles_beta) { - singles.emplace_back(from_spin(state_alpha, s_beta)); + singles.emplace_back(wfn_traits::from_spin(state_alpha, s_beta)); } // Generate Doubles in full space @@ -277,18 +249,18 @@ void generate_singles_doubles_spin(size_t norb, WfnType state, // Double Alpha + No Beta for(auto d_alpha : doubles_alpha) { - doubles.emplace_back(from_spin(d_alpha, state_beta)); + doubles.emplace_back(wfn_traits::from_spin(d_alpha, state_beta)); } // No Alpha + Double Beta for(auto d_beta : doubles_beta) { - doubles.emplace_back(from_spin(state_alpha, d_beta)); + doubles.emplace_back(wfn_traits::from_spin(state_alpha, d_beta)); } // Single Alpha + Single Beta for(auto s_alpha : singles_alpha) for(auto s_beta : singles_beta) { - doubles.emplace_back(from_spin(s_alpha, s_beta)); + doubles.emplace_back(wfn_traits::from_spin(s_alpha, s_beta)); } } @@ -311,6 +283,7 @@ auto generate_cisd_hilbert_space(size_t norb, WfnType state) { template std::vector generate_combs(uint64_t nbits, uint64_t nset) { + using wfn_traits = wavefunction_traits; std::vector v(nbits, false); std::fill_n(v.begin(), nset, true); std::vector store; @@ -319,7 +292,7 @@ std::vector generate_combs(uint64_t nbits, uint64_t nset) { WfnType temp(0ul); for(uint64_t i = 0; i < nbits; ++i) if(v[i]) { - temp = create_no_check(temp, i); + temp = wfn_traits::create_no_check(temp, i); } store.emplace_back(temp); @@ -331,8 +304,10 @@ std::vector generate_combs(uint64_t nbits, uint64_t nset) { template std::vector generate_hilbert_space(size_t norbs, size_t nalpha, size_t nbeta) { - // Get all alpha and beta combs using spin_wfn_type = spin_wfn_t; + using wfn_traits = wavefunction_traits; + + // Get all alpha and beta combs auto alpha_dets = generate_combs(norbs, nalpha); auto beta_dets = generate_combs(norbs, nbeta); @@ -340,7 +315,7 @@ std::vector generate_hilbert_space(size_t norbs, size_t nalpha, states.reserve(alpha_dets.size() * beta_dets.size()); for(auto alpha_det : alpha_dets) for(auto beta_det : beta_dets) { - states.emplace_back(from_spin(alpha_det, beta_det)); + states.emplace_back(wfn_traits::from_spin(alpha_det, beta_det)); } return states; @@ -376,16 +351,14 @@ inline auto single_excitation_sign_indices(WfnType bra, WfnType ket, WfnType ex) // TODO: Test this function template inline auto doubles_sign_indices(WfnType bra, WfnType ket, WfnType ex) { - const auto o1 = first_occupied_flipped(ket, ex); - const auto v1 = first_occupied_flipped(bra, ex); - auto sign = single_excitation_sign(ket, v1, o1); + using wfn_traits = wavefunction_traits; + auto [o1, v1, sign1] = single_excitation_sign_indices(bra, ket, ex); - ket = single_excitation(ket, o1, v1); - ex = single_excitation(ex, o1, v1); + ket = wfn_traits::single_excitation_no_check(ket, o1, v1); + ex = wfn_traits::single_excitation_no_check(ex, o1, v1); - const auto o2 = first_occupied_flipped(ket, ex); - const auto v2 = first_occupied_flipped(bra, ex); - sign *= single_excitation_sign(ket, v2, o2); + auto [o2, v2, sign2] = single_excitation_sign_indices(bra, ket, ex); + auto sign = sign1 * sign2; return std::make_tuple(o1, v1, o2, v2, sign); } @@ -397,57 +370,18 @@ inline auto doubles_sign(WfnType bra, WfnType ket, WfnType ex) { return sign; } -#if 0 -// TODO: Test this function -template -void generate_residues(std::bitset state, std::vector>& res) { - auto state_alpha = bitset_lo_word(state); - auto state_beta = bitset_hi_word(state); - - auto occ_alpha = bits_to_indices(state_alpha); - const int nalpha = occ_alpha.size(); - - auto occ_beta = bits_to_indices(state_beta); - const int nbeta = occ_beta.size(); - - std::bitset state_alpha_full = expand_bitset(state_alpha); - std::bitset state_beta_full = expand_bitset(state_beta); - state_beta_full = state_beta_full << (N / 2); - - std::bitset one = 1ul; - - // Double alpha - for(auto i = 0; i < nalpha; ++i) - for(auto j = i + 1; j < nalpha; ++j) { - auto mask = (one << occ_alpha[i]) | (one << occ_alpha[j]); - std::bitset _r = expand_bitset(state_alpha & ~mask); - res.emplace_back(_r | state_beta_full); - } - - // Double beta - for(auto i = 0; i < nbeta; ++i) - for(auto j = i + 1; j < nbeta; ++j) { - auto mask = (one << occ_beta[i]) | (one << occ_beta[j]); - std::bitset _r = expand_bitset(state_beta & ~mask) << (N / 2); - res.emplace_back(_r | state_alpha_full); - } - - // Mixed - for(auto i = 0; i < nalpha; ++i) - for(auto j = 0; j < nbeta; ++j) { - std::bitset mask = expand_bitset(one << occ_alpha[i]); - mask = mask | (expand_bitset(one << occ_beta[j]) << (N / 2)); - res.emplace_back(state & ~mask); - } -} -#endif template std::string to_canonical_string(WfnType state) { - auto state_alpha = alpha_string(state); - auto state_beta = beta_string (state); + using wfn_traits = wavefunction_traits; + using spin_wfn_type = spin_wfn_t; + using spin_wfn_traits = wavefunction_traits; + + auto state_alpha = wfn_traits::alpha_string(state); + auto state_beta = wfn_traits::beta_string (state); std::string str; - for(size_t i = 0; i < state_alpha.size(); ++i) { + + for(size_t i = 0; i < spin_wfn_traits::size(); ++i) { if(state_alpha[i] and state_beta[i]) str.push_back('2'); else if(state_alpha[i]) @@ -463,18 +397,20 @@ std::string to_canonical_string(WfnType state) { template WfnType from_canonical_string(std::string str) { using spin_wfn_type = spin_wfn_t; + using wfn_traits = wavefunction_traits; + using spin_wfn_traits = wavefunction_traits; spin_wfn_type state_alpha(0), state_beta(0); - for(auto i = 0ul; i < std::min(str.length(),state_alpha.size()); ++i) { + for(auto i = 0ul; i < std::min(str.length(),spin_wfn_traits::size()); ++i) { if(str[i] == '2') { - state_alpha = create_no_check(state_alpha, i); - state_beta = create_no_check(state_beta , i); + state_alpha = spin_wfn_traits::create_no_check(state_alpha, i); + state_beta = spin_wfn_traits::create_no_check(state_beta , i); } else if(str[i] == 'u') { - state_alpha = create_no_check(state_alpha, i); + state_alpha = spin_wfn_traits::create_no_check(state_alpha, i); } else if(str[i] == 'd') { - state_beta = create_no_check(state_beta, i); + state_beta = spin_wfn_traits::create_no_check(state_beta, i); } } - auto state = from_spin(state_alpha, state_beta); + auto state = wfn_traits::from_spin(state_alpha, state_beta); return state; } diff --git a/include/macis/util/rdms.hpp b/include/macis/util/rdms.hpp index 72b55bb3..e10a7cc7 100644 --- a/include/macis/util/rdms.hpp +++ b/include/macis/util/rdms.hpp @@ -103,8 +103,9 @@ inline void rdm_contributions(wfn_t bra_alpha, wfn_t ket_alpha, const IndexType& bra_occ_alpha, const IndexType& bra_occ_beta, T val, matrix_span ordm, rank4_span trdm) { - const uint32_t ex_alpha_count = ex_alpha.count(); - const uint32_t ex_beta_count = ex_beta.count(); + using wfn_traits = wavefunction_traits>; + const uint32_t ex_alpha_count = wfn_traits::count(ex_alpha); + const uint32_t ex_beta_count = wfn_traits::count(ex_beta); if((ex_alpha_count + ex_beta_count) > 4) return; diff --git a/include/macis/util/unused_untested.hpp b/include/macis/util/unused_untested.hpp index 491ee17e..2288c435 100644 --- a/include/macis/util/unused_untested.hpp +++ b/include/macis/util/unused_untested.hpp @@ -191,4 +191,48 @@ void generate_singles_doubles_spin_as(size_t norb, std::bitset state, doubles.emplace_back(d_state_alpha | d_state_beta); } } +#if 0 +// TODO: Test this function +template +void generate_residues(std::bitset state, std::vector>& res) { + auto state_alpha = bitset_lo_word(state); + auto state_beta = bitset_hi_word(state); + + auto occ_alpha = bits_to_indices(state_alpha); + const int nalpha = occ_alpha.size(); + + auto occ_beta = bits_to_indices(state_beta); + const int nbeta = occ_beta.size(); + + std::bitset state_alpha_full = expand_bitset(state_alpha); + std::bitset state_beta_full = expand_bitset(state_beta); + state_beta_full = state_beta_full << (N / 2); + + std::bitset one = 1ul; + + // Double alpha + for(auto i = 0; i < nalpha; ++i) + for(auto j = i + 1; j < nalpha; ++j) { + auto mask = (one << occ_alpha[i]) | (one << occ_alpha[j]); + std::bitset _r = expand_bitset(state_alpha & ~mask); + res.emplace_back(_r | state_beta_full); + } + + // Double beta + for(auto i = 0; i < nbeta; ++i) + for(auto j = i + 1; j < nbeta; ++j) { + auto mask = (one << occ_beta[i]) | (one << occ_beta[j]); + std::bitset _r = expand_bitset(state_beta & ~mask) << (N / 2); + res.emplace_back(_r | state_alpha_full); + } + + // Mixed + for(auto i = 0; i < nalpha; ++i) + for(auto j = 0; j < nbeta; ++j) { + std::bitset mask = expand_bitset(one << occ_alpha[i]); + mask = mask | (expand_bitset(one << occ_beta[j]) << (N / 2)); + res.emplace_back(state & ~mask); + } +} +#endif #endif diff --git a/include/macis/wfn/raw_bitset.hpp b/include/macis/wfn/raw_bitset.hpp new file mode 100644 index 00000000..04c096f2 --- /dev/null +++ b/include/macis/wfn/raw_bitset.hpp @@ -0,0 +1,127 @@ +#pragma once + +#include +#include + +namespace macis { + +enum class Spin { + Alpha, + Beta +}; + +template +struct wavefunction_traits; + +template +using spin_wfn_t = typename wavefunction_traits::spin_wfn_type; + +template +struct wavefunction_traits> { + + using wfn_type = std::bitset; + using spin_wfn_type = std::bitset; + using orbidx_type = uint32_t; + using orbidx_container = std::vector; + + inline static constexpr size_t bit_size = N; + + static constexpr auto size() { return bit_size; } + + static inline auto count(wfn_type state) { return state.count(); } + + static inline spin_wfn_type alpha_string(wfn_type state) { + return bitset_lo_word(state); + } + + static inline spin_wfn_type beta_string(wfn_type state) { + return bitset_hi_word(state); + } + + template + static inline wfn_type from_spin(spin_wfn_type alpha, spin_wfn_type beta) { + if constexpr (Sigma == Spin::Alpha) { + auto alpha_expand = expand_bitset(alpha); + auto beta_expand = expand_bitset(beta) << N/2; + return alpha_expand | beta_expand; + } else { + auto alpha_expand = expand_bitset(alpha) << N/2; + auto beta_expand = expand_bitset(beta); + return alpha_expand | beta_expand; + } + } + + static inline wfn_type canonical_hf_determinant(uint32_t nalpha, uint32_t nbeta) { + + spin_wfn_type alpha = full_mask(nalpha); + spin_wfn_type beta = full_mask(nbeta); + return from_spin(alpha, beta); + + } + + template + static inline wfn_type& flip_bits(wfn_type& state, Inds&&... ); + + template + static inline wfn_type& flip_bits(wfn_type& state) { + return state; + } + + template + static inline wfn_type& flip_bits(wfn_type& state, unsigned p, Inds&&... inds) { + return flip_bits( + state.flip(p + (Sigma == Spin::Alpha ? 0 : N/2)), + std::forward(inds)... + ); + } + + template + static inline wfn_type create_no_check(wfn_type state, unsigned p) { + flip_bits(state, p); + return state; + } + + template + static inline wfn_type single_excitation_no_check(wfn_type state, + unsigned p, + unsigned q) { + flip_bits(state, p, q); + return state; + } + + template + static inline wfn_type double_excitation_no_check(wfn_type state, + unsigned p, + unsigned q, + unsigned r, + unsigned s) { + flip_bits(state, p, q, r, s); + return state; + } + + static inline void state_to_occ(wfn_type state, orbidx_container& occ) { + occ = bits_to_indices(state); + } + + static inline void state_to_occ_vir(size_t norb, wfn_type state, orbidx_container& occ, + orbidx_container& vir) { + + state_to_occ(state, occ); + const auto nocc = occ.size(); + assert(nocc < norb); + + const auto nvir = norb - nocc; + vir.resize(nvir); + state = ~state; + for(int i = 0; i < nvir; ++i) { + auto a = ffs(state) - 1; + vir[i] = a; + state.flip(a); + } + } + +}; + + + +} diff --git a/tests/asci.cxx b/tests/asci.cxx index a6eb65b7..be45f848 100644 --- a/tests/asci.cxx +++ b/tests/asci.cxx @@ -232,7 +232,9 @@ TEST_CASE("ASCI") { macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); // Hamiltonian Genereator - using generator_t = macis::DoubleLoopHamiltonianGenerator>; + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + using generator_t = macis::DoubleLoopHamiltonianGenerator; generator_t ham_gen( macis::matrix_span(T.data(), norb, norb), macis::rank4_span(V.data(), norb, norb, norb, norb)); @@ -243,8 +245,8 @@ TEST_CASE("ASCI") { macis::MCSCFSettings mcscf_settings; // HF guess - std::vector> dets = { - macis::canonical_hf_determinant<64>(nalpha, nbeta)}; + std::vector dets = { + wfn_traits::canonical_hf_determinant(nalpha, nbeta)}; ; std::vector C = {1.0}; double E0 = ham_gen.matrix_element(dets[0], dets[0]); diff --git a/tests/csr_hamiltonian.cxx b/tests/csr_hamiltonian.cxx index fc0a41be..ba4f2417 100644 --- a/tests/csr_hamiltonian.cxx +++ b/tests/csr_hamiltonian.cxx @@ -27,7 +27,9 @@ TEST_CASE("CSR Hamiltonian") { macis::read_fcidump_1body(water_ccpvdz_fcidump, T.data(), norb); macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator>; + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + using generator_type = macis::DoubleLoopHamiltonianGenerator; #if 0 generator_type ham_gen(norb, V.data(), T.data()); @@ -38,7 +40,7 @@ TEST_CASE("CSR Hamiltonian") { #endif // Generate configuration space - const auto hf_det = macis::canonical_hf_determinant<64>(nocc, nocc); + const auto hf_det = wfn_traits::canonical_hf_determinant(nocc, nocc); auto dets = macis::generate_cisd_hilbert_space(norb, hf_det); // Generate CSR Hamiltonian @@ -82,7 +84,9 @@ TEST_CASE("Distributed CSR Hamiltonian") { macis::read_fcidump_1body(water_ccpvdz_fcidump, T.data(), norb); macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator>; + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + using generator_type = macis::DoubleLoopHamiltonianGenerator; #if 0 generator_type ham_gen(norb, V.data(), T.data()); @@ -93,7 +97,7 @@ TEST_CASE("Distributed CSR Hamiltonian") { #endif // Generate configuration space - const auto hf_det = macis::canonical_hf_determinant<64>(nocc, nocc); + const auto hf_det = wfn_traits::canonical_hf_determinant(nocc, nocc); auto dets = macis::generate_cisd_hilbert_space(norb, hf_det); // Generate Distributed CSR Hamiltonian diff --git a/tests/davidson.cxx b/tests/davidson.cxx index 88105c31..db27e85b 100644 --- a/tests/davidson.cxx +++ b/tests/davidson.cxx @@ -32,7 +32,9 @@ TEST_CASE("Davidson") { macis::read_fcidump_1body(water_ccpvdz_fcidump, T.data(), norb); macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator>; + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + using generator_type = macis::DoubleLoopHamiltonianGenerator; #if 0 generator_type ham_gen(norb, V.data(), T.data()); @@ -43,7 +45,7 @@ TEST_CASE("Davidson") { #endif // Generate configuration space - const auto hf_det = macis::canonical_hf_determinant<64>(nocc, nocc); + const auto hf_det = wfn_traits::canonical_hf_determinant(nocc, nocc); auto dets = macis::generate_cisd_hilbert_space(norb, hf_det); auto E0_ref = -7.623197835987e+01; @@ -85,7 +87,9 @@ TEST_CASE("Parallel Davidson") { macis::read_fcidump_1body(water_ccpvdz_fcidump, T.data(), norb); macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator>; + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + using generator_type = macis::DoubleLoopHamiltonianGenerator; #if 0 generator_type ham_gen(norb, V.data(), T.data()); @@ -96,7 +100,7 @@ TEST_CASE("Parallel Davidson") { #endif // Generate configuration space - const auto hf_det = macis::canonical_hf_determinant<64>(nocc, nocc); + const auto hf_det = wfn_traits::canonical_hf_determinant(nocc, nocc); auto dets = macis::generate_cisd_hilbert_space(norb, hf_det); auto E0_ref = -7.623197835987e+01; diff --git a/tests/double_loop.cxx b/tests/double_loop.cxx index fa4ab232..818d2a4e 100644 --- a/tests/double_loop.cxx +++ b/tests/double_loop.cxx @@ -30,7 +30,9 @@ TEST_CASE("Double Loop") { macis::read_fcidump_1body(water_ccpvdz_fcidump, T.data(), norb); macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator>; + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + using generator_type = macis::DoubleLoopHamiltonianGenerator; #if 0 generator_type ham_gen(norb, V.data(), T.data()); @@ -39,7 +41,7 @@ TEST_CASE("Double Loop") { macis::matrix_span(T.data(), norb, norb), macis::rank4_span(V.data(), norb, norb, norb, norb)); #endif - const auto hf_det = macis::canonical_hf_determinant<64>(nocc, nocc); + const auto hf_det = wfn_traits::canonical_hf_determinant(nocc, nocc); std::vector eps(norb); for(auto p = 0ul; p < norb; ++p) { @@ -93,7 +95,7 @@ TEST_CASE("Double Loop") { for(size_t i = 0; i < nocc; ++i) for(size_t a = nocc; a < norb; ++a) { // Generate excited determinant - std::bitset<64> state = hf_det; + wfn_type state = hf_det; state.flip(i).flip(a); auto el_1 = ham_gen.matrix_element(hf_det, state); auto el_2 = ham_gen.matrix_element(state, hf_det); @@ -105,7 +107,7 @@ TEST_CASE("Double Loop") { for(size_t i = 0; i < nocc; ++i) for(size_t a = nocc; a < norb; ++a) { // Generate excited determinant - std::bitset<64> state = hf_det; + wfn_type state = hf_det; state.flip(i + 32).flip(a + 32); auto el_1 = ham_gen.matrix_element(hf_det, state); auto el_2 = ham_gen.matrix_element(state, hf_det); @@ -163,8 +165,8 @@ TEST_CASE("Double Loop") { SECTION("RDM") { std::vector ordm(norb * norb, 0.0), trdm(norb3 * norb, 0.0); - std::vector> dets = { - macis::canonical_hf_determinant<64>(nocc, nocc)}; + std::vector dets = { + wfn_traits::canonical_hf_determinant(nocc, nocc)}; std::vector C = {1.}; @@ -196,14 +198,16 @@ TEST_CASE("RDMS") { macis::rank4_span V_span(V.data(), norb, norb, norb, norb); macis::rank4_span trdm_span(trdm.data(), norb, norb, norb, norb); - using generator_type = macis::DoubleLoopHamiltonianGenerator>; + using wfn_type = macis::wfn_t<128>; + using wfn_traits = macis::wavefunction_traits; + using generator_type = macis::DoubleLoopHamiltonianGenerator; generator_type ham_gen(T_span, V_span); auto abs_sum = [](auto a, auto b) { return a + std::abs(b); }; SECTION("HF") { - std::vector> dets = { - macis::canonical_hf_determinant<128>(nocc, nocc)}; + std::vector dets = { + wfn_traits::canonical_hf_determinant(nocc, nocc)}; std::vector C = {1.}; @@ -226,7 +230,7 @@ TEST_CASE("RDMS") { } SECTION("CI") { - std::vector> states; + std::vector states; std::vector coeffs; macis::read_wavefunction<128>(ch4_wfn_fname, states, coeffs); diff --git a/tests/sd_operations.cxx b/tests/sd_operations.cxx index 3635eff2..68e62c28 100644 --- a/tests/sd_operations.cxx +++ b/tests/sd_operations.cxx @@ -16,7 +16,9 @@ TEST_CASE("Slater Det Operations") { SECTION("HF Determinant") { SECTION("Canonical Ordering") { - auto hf = macis::canonical_hf_determinant<32>(4, 2); + using wfn_type = macis::wfn_t<32>; + using wfn_traits = macis::wavefunction_traits; + auto hf = wfn_traits::canonical_hf_determinant(4, 2); REQUIRE(hf == 0x0003000F); } @@ -31,12 +33,14 @@ TEST_CASE("Slater Det Operations") { SECTION("Occupied / Unoccupied Conversion") { SECTION("Default") { - macis::wfn_t<64> state = 0x00000000000000AF; + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + wfn_type state = 0x00000000000000AF; std::vector ref_occ = {0, 1, 2, 3, 5, 7}; std::vector ref_vir = {4, 6, 8, 9, 10, 11}; std::vector occ, vir; - macis::bitset_to_occ_vir(12, state, occ, vir); + wfn_traits::state_to_occ_vir(12, state, occ, vir); REQUIRE(occ == ref_occ); REQUIRE(vir == ref_vir); @@ -47,14 +51,16 @@ TEST_CASE("Slater Det Operations") { SECTION("Singles") { SECTION("Single Spin") { - std::vector> ref_singles = { + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + std::vector ref_singles = { 0b00011110, 0b00101110, 0b01001110, 0b10001110, 0b00011101, 0b00101101, 0b01001101, 0b10001101, 0b00011011, 0b00101011, 0b01001011, 0b10001011, 0b00010111, 0b00100111, 0b01000111, 0b10000111}; - std::vector> singles; - auto state = macis::canonical_hf_determinant<64>(4, 0); // all alpha + std::vector singles; + auto state = wfn_traits::canonical_hf_determinant(4, 0); // all alpha macis::generate_singles(8, state, singles); auto cmp = macis::bitset_less_comparator<64>{}; @@ -65,7 +71,9 @@ TEST_CASE("Slater Det Operations") { } SECTION("Both Spin") { - std::vector> ref_singles = { + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + std::vector ref_singles = { 0x0F0000001E, 0x0F0000001D, 0x0F0000001B, 0x0F00000017, 0x0F0000002E, 0x0F0000002D, 0x0F0000002B, 0x0F00000027, 0x0F0000004E, 0x0F0000004D, 0x0F0000004B, 0x0F00000047, 0x0F0000008E, 0x0F0000008D, 0x0F0000008B, @@ -74,8 +82,8 @@ TEST_CASE("Slater Det Operations") { 0x4D0000000F, 0x4B0000000F, 0x470000000F, 0x8E0000000F, 0x8D0000000F, 0x8B0000000f, 0x870000000f}; - auto state = macis::canonical_hf_determinant<64>(4, 4); - std::vector> singles; + auto state = wfn_traits::canonical_hf_determinant(4, 4); + std::vector singles; macis::generate_singles_spin(8, state, singles); auto cmp = macis::bitset_less_comparator<64>{}; @@ -88,7 +96,9 @@ TEST_CASE("Slater Det Operations") { SECTION("Doubles") { SECTION("Single Spin") { - std::vector> ref_doubles = { + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + std::vector ref_doubles = { 0b00111100, 0b01011100, 0b10011100, 0b01101100, 0b10101100, 0b11001100, 0b00111010, 0b01011010, 0b10011010, 0b01101010, 0b10101010, 0b11001010, 0b00111001, 0b01011001, 0b10011001, @@ -98,8 +108,8 @@ TEST_CASE("Slater Det Operations") { 0b00110011, 0b01010011, 0b10010011, 0b01100011, 0b10100011, 0b11000011}; - std::vector> doubles; - auto state = macis::canonical_hf_determinant<64>(4, 0); // all alpha + std::vector doubles; + auto state = wfn_traits::canonical_hf_determinant(4, 0); // all alpha macis::generate_doubles(8, state, doubles); auto cmp = macis::bitset_less_comparator<64>{}; @@ -110,7 +120,9 @@ TEST_CASE("Slater Det Operations") { } SECTION("Both Spins") { - std::vector> ref_doubles = { + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + std::vector ref_doubles = { 0x0F0000003C, 0x0F0000003A, 0x0F00000036, 0x0F0000005C, 0x0F0000005A, 0x0F00000056, 0x0F0000009C, 0x0F0000009A, 0x0F00000096, 0x0F00000039, 0x0F00000035, 0x0F00000059, 0x0F00000055, 0x0F00000099, 0x0F00000095, @@ -177,8 +189,8 @@ TEST_CASE("Slater Det Operations") { 0x1700000087, 0x2E00000087, 0x2D00000087, 0x2B00000087, 0x2700000087, 0x4E00000087, 0x4D00000087, 0x4B00000087, 0x4700000087, 0x8E00000087, 0x8D00000087, 0x8B00000087, 0x8700000087}; - auto state = macis::canonical_hf_determinant<64>(4, 4); - std::vector> singles, doubles; + auto state = wfn_traits::canonical_hf_determinant(4, 4); + std::vector singles, doubles; macis::generate_singles_doubles_spin(8, state, singles, doubles); auto cmp = macis::bitset_less_comparator<64>{}; @@ -190,8 +202,10 @@ TEST_CASE("Slater Det Operations") { } SECTION("CIS") { - auto state = macis::canonical_hf_determinant<64>(4, 4); - std::vector> singles; + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + auto state = wfn_traits::canonical_hf_determinant(4, 4); + std::vector singles; macis::generate_singles_spin(8, state, singles); singles.push_back(state); auto cis = macis::generate_cis_hilbert_space(8, state); @@ -203,8 +217,10 @@ TEST_CASE("Slater Det Operations") { } SECTION("CISD") { - auto state = macis::canonical_hf_determinant<64>(4, 4); - std::vector> singles, doubles; + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + auto state = wfn_traits::canonical_hf_determinant(4, 4); + std::vector singles, doubles; macis::generate_singles_doubles_spin(8, state, singles, doubles); singles.insert(singles.end(), doubles.begin(), doubles.end()); singles.push_back(state); @@ -240,7 +256,9 @@ TEST_CASE("Slater Det Operations") { } SECTION("String Conversions") { - auto state = macis::canonical_hf_determinant<64>(2, 2).flip(3).flip(4 + 32); + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + auto state = wfn_traits::canonical_hf_determinant(2, 2).flip(3).flip(4 + 32); SECTION("To String") { auto str = macis::to_canonical_string(state); @@ -250,13 +268,13 @@ TEST_CASE("Slater Det Operations") { SECTION("From String") { SECTION("Full String") { std::string str = "220ud000000000000000000000000000"; - auto det = macis::from_canonical_string>(str); + auto det = macis::from_canonical_string(str); REQUIRE(det == state); } SECTION("Short String") { std::string str = "220ud"; - auto det = macis::from_canonical_string>(str); + auto det = macis::from_canonical_string(str); REQUIRE(det == state); } } diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index e8926d69..55f47ae7 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -64,6 +64,7 @@ int main(int argc, char** argv) { constexpr size_t nwfn_bits = 64; using wfn_type = macis::wfn_t; + using wfn_traits = macis::wavefunction_traits; MACIS_MPI_CODE(MPI_Init(&argc, &argv);) @@ -342,7 +343,7 @@ int main(int argc, char** argv) { } else { // HF Guess console->info("Generating HF Guess for ASCI"); - dets = {macis::canonical_hf_determinant(nalpha, nalpha)}; + dets = {wfn_traits::canonical_hf_determinant(nalpha, nalpha)}; // std::cout << dets[0].to_ullong() << std::endl; E0 = ham_gen.matrix_element(dets[0], dets[0]); C = {1.0}; From 3bbd61b785372760602871b423151a91b5d6faad Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Mon, 11 Sep 2023 11:26:48 -0700 Subject: [PATCH 18/73] Work on generic constraints, added templates over constraint type --- include/macis/asci/determinant_search.hpp | 11 ++- include/macis/asci/mask_constraints.hpp | 112 ++++++++++------------ include/macis/asci/pt2.hpp | 10 +- tests/asci.cxx | 23 ++++- 4 files changed, 77 insertions(+), 79 deletions(-) diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index 8fd017fd..447d95d2 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -281,7 +281,8 @@ asci_contrib_container> asci_contributions_constraint( const double h_el_tol = asci_settings.h_el_tol; const auto& [C, B, C_min] = con; - wfn_t O = full_mask(norb); + wfn_constraint alpha_con{ wfn_traits::alpha_string(C), wfn_traits::alpha_string(B), C_min}; + //wfn_t O = full_mask(norb); // Loop over unique alpha strings for(size_t i_alpha = 0; i_alpha < nuniq_alpha; ++i_alpha) { @@ -296,7 +297,7 @@ asci_contrib_container> asci_contributions_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_singles_contributions_ss( - coeff, det|beta, C, O, B, occ_alpha, occ_beta, + coeff, det|beta, alpha_con, occ_alpha, occ_beta, orb_ens_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -309,7 +310,7 @@ asci_contrib_container> asci_contributions_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_doubles_contributions_ss( - coeff, det|beta, C, O, B, occ_alpha, occ_beta, + coeff, det|beta, alpha_con, occ_alpha, occ_beta, orb_ens_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -324,14 +325,14 @@ asci_contrib_container> asci_contributions_constraint( const auto& orb_ens_alpha = bcd.orb_ens_alpha; const auto& orb_ens_beta = bcd.orb_ens_beta; generate_constraint_doubles_contributions_os( - coeff, det|beta, C, O, B, occ_alpha, occ_beta, vir_beta, + coeff, det|beta, alpha_con, occ_alpha, occ_beta, vir_beta, orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } // If the alpha determinant satisfies the constraint, // append BB and BBBB excitations - if(satisfies_constraint(det, C, C_min)) { + if(satisfies_constraint(det, con)) { for(const auto& bcd : uad[i_alpha].bcd) { const auto& beta = bcd.beta_string; const auto& coeff = bcd.coeff; diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index a02a3479..b8866cf9 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -22,47 +22,20 @@ struct wfn_constraint { }; template -auto make_triplet(unsigned i, unsigned j, unsigned k) { - wfn_constraint con; - - con.C = 0; - con.C.flip(i).flip(j).flip(k); - con.B = 1; - con.B <<= k; - con.B = con.B.to_ullong() - 1; - con.C_min = k; - - return con; -} - -template -auto make_quad(unsigned i, unsigned j, unsigned k, unsigned l) { - wfn_constraint con; - - con.C = 0; - con.C.flip(i).flip(j).flip(k).flip(l); - con.B = 1; - con.B <<= l; - con.B = con.B.to_ullong() - 1; - con.C_min = l; - - return con; -} - -template -bool satisfies_constraint(wfn_t det, wfn_t C, unsigned C_min) { +bool satisfies_constraint(wfn_t det, wfn_constraint constraint) { + auto C = constraint.C; auto C_min = constraint.C_min; return (det & C).count() == C.count() and ((det ^ C) >> C_min).count() == 0; } template -auto generate_constraint_single_excitations(wfn_t det, wfn_t C, - wfn_t O_mask, wfn_t B) { +auto generate_constraint_single_excitations(wfn_t det, wfn_constraint constraint) { + const auto C = constraint.C; const auto B = constraint.B; if((det & C).count() < (C.count() - 1)) // need to have at most one different from the constraint return std::make_pair(wfn_t(0), wfn_t(0)); auto o = det ^ C; - auto v = (~det) & O_mask & B; + auto v = (~det) & B; if((o & C).count() == 1) { // don't have to change this necessarily, but more clear without >= @@ -78,15 +51,15 @@ auto generate_constraint_single_excitations(wfn_t det, wfn_t C, } template -auto generate_constraint_double_excitations(wfn_t det, wfn_t C, - wfn_t O_mask, wfn_t B) { +auto generate_constraint_double_excitations(wfn_t det, wfn_constraint constraint) { + const auto C = constraint.C; const auto B = constraint.B; // Occ/Vir pairs to generate excitations std::vector> O, V; if((det & C) == 0) return std::make_tuple(O, V); auto o = det ^ C; - auto v = (~det) & O_mask & B; + auto v = (~det) & B; if((o & C).count() >= 3) return std::make_tuple(O, V); @@ -130,9 +103,9 @@ auto generate_constraint_double_excitations(wfn_t det, wfn_t C, } template -void generate_constraint_singles(wfn_t det, wfn_t T, wfn_t O_mask, - wfn_t B, std::vector>& t_singles) { - auto [o, v] = generate_constraint_single_excitations(det, T, O_mask, B); +void generate_constraint_singles(wfn_t det, wfn_constraint constraint, + std::vector>& t_singles) { + auto [o, v] = generate_constraint_single_excitations(det, constraint); const auto oc = o.count(); const auto vc = v.count(); if(!oc or !vc) return; @@ -156,9 +129,9 @@ unsigned count_constraint_singles(Args&&... args) { } template -void generate_constraint_doubles(wfn_t det, wfn_t T, wfn_t O_mask, - wfn_t B, std::vector>& t_doubles) { - auto [O, V] = generate_constraint_double_excitations(det, T, O_mask, B); +void generate_constraint_doubles(wfn_t det, wfn_constraint constraint, + std::vector>& t_doubles) { + auto [O, V] = generate_constraint_double_excitations(det, constraint); t_doubles.clear(); for(auto ij : O) { @@ -172,16 +145,15 @@ void generate_constraint_doubles(wfn_t det, wfn_t T, wfn_t O_mask, /** * @param[in] det Input root determinant * @param[in] T Triplet constraint mask - * @param[in] O Overfill mask (full mask 0 -> norb) * @param[in] B B mask (?) */ template -unsigned count_constraint_doubles(wfn_t det, wfn_t C, wfn_t O, - wfn_t B) { +unsigned count_constraint_doubles(wfn_t det, wfn_constraint constraint) { + const auto C = constraint.C; const auto B = constraint.B; if((det & C) == 0) return 0; auto o = det ^ C; - auto v = (~det) & O & B; + auto v = (~det) & B; if((o & C).count() >= 3) return 0; @@ -223,26 +195,24 @@ unsigned count_constraint_doubles(wfn_t det, wfn_t C, wfn_t O, template size_t constraint_histogram(wfn_t det, size_t n_os_singles, - size_t n_os_doubles, wfn_t T, wfn_t O_mask, - wfn_t B) { - auto ns = count_constraint_singles(det, T, O_mask, B); - auto nd = count_constraint_doubles(det, T, O_mask, B); + size_t n_os_doubles, wfn_constraint constraint){ + auto ns = count_constraint_singles(det, constraint); + auto nd = count_constraint_doubles(det, constraint); size_t ndet = 0; ndet += ns; // AA ndet += nd; // AAAA ndet += ns * n_os_singles; // AABB - auto T_min = ffs(T) - 1; - if(satisfies_constraint(det, T, T_min)) { + if(satisfies_constraint(det, constraint)) { ndet += n_os_singles + n_os_doubles + 1; // BB + BBBB + No Excitations } return ndet; } -template +template void generate_constraint_singles_contributions_ss( - double coeff, WfnType det, WfnType T, WfnType O, WfnType B, + double coeff, WfnType det, ConType constraint, const std::vector& occ_same, const std::vector& occ_othr, const double* eps, const double* T_pq, const size_t LDT, const double* G_kpq, const size_t LDG, @@ -250,7 +220,7 @@ void generate_constraint_singles_contributions_ss( double E0, HamiltonianGeneratorBase& ham_gen, asci_contrib_container& asci_contributions) { using wfn_traits = wavefunction_traits; - auto [o, v] = generate_constraint_single_excitations(wfn_traits::alpha_string(det), wfn_traits::alpha_string(T), wfn_traits::alpha_string(O), wfn_traits::alpha_string(B)); + auto [o, v] = generate_constraint_single_excitations(wfn_traits::alpha_string(det), constraint); const auto no = o.count(); const auto nv = v.count(); if(!no or !nv) return; @@ -291,9 +261,9 @@ void generate_constraint_singles_contributions_ss( } } -template +template void generate_constraint_doubles_contributions_ss( - double coeff, WfnType det, WfnType T, WfnType O_mask, WfnType B, + double coeff, WfnType det, ConType constraint, const std::vector& occ_same, const std::vector& occ_othr, const double* eps, const double* G, const size_t LDG, double h_el_tol, double root_diag, double E0, @@ -301,7 +271,7 @@ void generate_constraint_doubles_contributions_ss( asci_contrib_container& asci_contributions) { using wfn_traits = wavefunction_traits; using spin_wfn_traits = wavefunction_traits>; - auto [O, V] = generate_constraint_double_excitations(wfn_traits::alpha_string(det), wfn_traits::alpha_string(T), wfn_traits::alpha_string(O_mask), wfn_traits::alpha_string(B)); + auto [O, V] = generate_constraint_double_excitations(wfn_traits::alpha_string(det), constraint); const auto no_pairs = O.size(); const auto nv_pairs = V.size(); if(!no_pairs or !nv_pairs) return; @@ -346,9 +316,9 @@ void generate_constraint_doubles_contributions_ss( } } -template +template void generate_constraint_doubles_contributions_os( - double coeff, WfnType det, WfnType T, WfnType O, WfnType B, + double coeff, WfnType det, ConType constraint, const std::vector& occ_same, const std::vector& occ_othr, const std::vector& vir_othr, const double* eps_same, @@ -357,7 +327,7 @@ void generate_constraint_doubles_contributions_os( asci_contrib_container& asci_contributions) { using wfn_traits = wavefunction_traits; // Generate Single Excitations that Satisfy the Constraint - auto [o, v] = generate_constraint_single_excitations(wfn_traits::alpha_string(det), wfn_traits::alpha_string(T), wfn_traits::alpha_string(O), wfn_traits::alpha_string(B)); + auto [o, v] = generate_constraint_single_excitations(wfn_traits::alpha_string(det), constraint); const auto no = o.count(); const auto nv = v.count(); if(!no or !nv) return; @@ -488,6 +458,21 @@ auto dist_triplets_histogram(size_t norb, size_t ns_othr, size_t nd_othr, } #endif + +template +auto make_triplet(unsigned i, unsigned j, unsigned k) { + wfn_constraint con; + + con.C = 0; + con.C.flip(i).flip(j).flip(k); + con.B = 1; + con.B <<= k; + con.B = con.B.to_ullong() - 1; + con.C_min = k; + + return con; +} + #ifdef MACIS_ENABLE_MPI template auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, @@ -497,7 +482,7 @@ auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, auto world_rank = comm_rank(comm); auto world_size = comm_size(comm); - wfn_t O = full_mask(norb); + //wfn_t O = full_mask(norb); // Global workloads std::vector workloads(world_size, 0); @@ -514,7 +499,7 @@ auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, size_t nw = 0; for(const auto& alpha : unique_alpha) { - nw += constraint_histogram(alpha, ns_othr, nd_othr, T, O, B); + nw += constraint_histogram(alpha, ns_othr, nd_othr, constraint); } if(nw) constraint_sizes.emplace_back(constraint, nw); total_work += nw; @@ -553,8 +538,7 @@ auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, size_t nw = 0; for(const auto& alpha : unique_alpha) { - nw += constraint_histogram(alpha, ns_othr, nd_othr, c_next.C, O, - c_next.B); + nw += constraint_histogram(alpha, ns_othr, nd_othr, c_next); } if(nw) constraint_sizes.emplace_back(c_next, nw); total_work += nw; diff --git a/include/macis/asci/pt2.hpp b/include/macis/asci/pt2.hpp index 0610a0af..b560597c 100644 --- a/include/macis/asci/pt2.hpp +++ b/include/macis/asci/pt2.hpp @@ -131,7 +131,7 @@ double asci_pt2_constraint( //std::cout << std::distance(&constraints[0], &con) << "/" << constraints.size() << std::endl; const double h_el_tol = 1e-16; const auto& [C, B, C_min] = con; - wfn_t O = full_mask(norb); + wfn_constraint alpha_con{ wfn_traits::alpha_string(C), wfn_traits::alpha_string(B), C_min}; // Loop over unique alpha strings for(size_t i_alpha = 0; i_alpha < nuniq_alpha; ++i_alpha) { @@ -146,7 +146,7 @@ double asci_pt2_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_singles_contributions_ss( - coeff, det|beta, C, O, B, occ_alpha, occ_beta, + coeff, det|beta, alpha_con, occ_alpha, occ_beta, orb_ens_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -159,7 +159,7 @@ double asci_pt2_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_doubles_contributions_ss( - coeff, det|beta, C, O, B, occ_alpha, occ_beta, + coeff, det|beta, alpha_con, occ_alpha, occ_beta, orb_ens_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -174,14 +174,14 @@ double asci_pt2_constraint( const auto& orb_ens_alpha = bcd.orb_ens_alpha; const auto& orb_ens_beta = bcd.orb_ens_beta; generate_constraint_doubles_contributions_os( - coeff, det|beta, C, O, B, occ_alpha, occ_beta, vir_beta, + coeff, det|beta, alpha_con, occ_alpha, occ_beta, vir_beta, orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } // If the alpha determinant satisfies the constraint, // append BB and BBBB excitations - if(satisfies_constraint(det, C, C_min)) { + if(satisfies_constraint(det, con)) { for(const auto& bcd : uad[i_alpha].bcd) { const auto& beta = bcd.beta_string; const auto& coeff = bcd.coeff; diff --git a/tests/asci.cxx b/tests/asci.cxx index be45f848..f088f853 100644 --- a/tests/asci.cxx +++ b/tests/asci.cxx @@ -45,6 +45,20 @@ size_t top_set_ordinal(std::bitset word, size_t NSet) { return ord; } +template +auto make_quad(unsigned i, unsigned j, unsigned k, unsigned l) { + macis::wfn_constraint con; + + con.C = 0; + con.C.flip(i).flip(j).flip(k).flip(l); + con.B = 1; + con.B <<= l; + con.B = con.B.to_ullong() - 1; + con.C_min = l; + + return con; +} + TEST_CASE("Triplets") { constexpr size_t num_bits = 64; size_t norb = 32; @@ -159,12 +173,11 @@ TEST_CASE("Triplets") { triplets.emplace_back(i, j, k); } - const auto overfill = macis::full_mask(norb); std::vector new_triplet_hist(triplet_hist.size(), 0); for(auto [i, j, k] : triplets) { const auto label = i * 32 * 32 + j * 32 + k; - auto [T, B, T_min] = macis::make_triplet(i, j, k); + auto constraint = macis::make_triplet(i, j, k); for(auto det : wfn_a_uniq) { const size_t nocc = det.count(); @@ -173,7 +186,7 @@ TEST_CASE("Triplets") { const size_t n_doubles = (n_singles * (n_singles - nocc - nvir + 1)) / 4; new_triplet_hist[label] += macis::constraint_histogram( - det, n_singles, n_doubles, T, overfill, B); + det, n_singles, n_doubles, constraint); } } @@ -191,7 +204,7 @@ TEST_CASE("Triplets") { for(auto [i, j, k, l] : quads) { const size_t label = i * 32ul * 32ul * 32ul + j * 32ul * 32ul + k * 32ul + l; - auto [Q, B, Q_min] = macis::make_quad(i, j, k, l); + auto constraint = make_quad(i, j, k, l); for(auto det : wfn_a_uniq) { const size_t nocc = det.count(); @@ -200,7 +213,7 @@ TEST_CASE("Triplets") { const size_t n_doubles = (n_singles * (n_singles - nocc - nvir + 1)) / 4; new_quad_hist[label] += macis::constraint_histogram( - det, n_singles, n_doubles, Q, overfill, B); + det, n_singles, n_doubles, constraint); } } From e22433841a11cdcd4ff4bc4369cabb064f15f949 Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Wed, 13 Sep 2023 15:41:01 -0700 Subject: [PATCH 19/73] changed wfn_constraint -> alpha_constraint and made appropriate changes --- include/macis/asci/alpha_constraint.hpp | 70 +++++++++++++++ include/macis/asci/determinant_search.hpp | 13 ++- include/macis/asci/mask_constraints.hpp | 101 +++++++++++----------- include/macis/asci/pt2.hpp | 10 +-- tests/asci.cxx | 24 ++--- 5 files changed, 144 insertions(+), 74 deletions(-) create mode 100644 include/macis/asci/alpha_constraint.hpp diff --git a/include/macis/asci/alpha_constraint.hpp b/include/macis/asci/alpha_constraint.hpp new file mode 100644 index 00000000..4d0ca2be --- /dev/null +++ b/include/macis/asci/alpha_constraint.hpp @@ -0,0 +1,70 @@ +#pragma once + +#include +namespace macis { + +template +class alpha_constraint { + +public: + using wfn_traits = WfnTraits; + using wfn_type = typename WfnTraits::wfn_type; + using spin_wfn_type = spin_wfn_t; + using spin_wfn_traits = wavefunction_traits; + using constraint_type = spin_wfn_type; + +private: + constraint_type C_; + constraint_type B_; + uint32_t C_min_; + uint32_t count_; + +public: + + alpha_constraint(constraint_type C, constraint_type B, uint32_t C_min) : + C_(C), B_(B), C_min_(C_min), count_(spin_wfn_traits::count(C)) {} + + alpha_constraint(const alpha_constraint&) = default; + alpha_constraint& operator=(const alpha_constraint&) = default; + + alpha_constraint(alpha_constraint&& other) noexcept = default; + alpha_constraint& operator=(alpha_constraint&&) noexcept = default; + + + inline auto C() const { return C_; } + inline auto B() const { return B_; } + inline auto C_min() const { return C_min_; } + inline auto count() const { return count_; } + + + inline spin_wfn_type c_mask_union(spin_wfn_type state) const { + return state & C_; + } + inline spin_wfn_type b_mask_union(spin_wfn_type state) const { + return state & B_; + } + + inline spin_wfn_type symmetric_difference(spin_wfn_type state) const { + return state ^ C_; + } + inline spin_wfn_type symmetric_difference(wfn_type state) const { + return symmetric_difference(wfn_traits::alpha_string(state)); + } + + template + inline auto overlap(WfnType state) const { + return spin_wfn_traits::count(c_mask_union(state)); + } + + template + inline bool satisfies_constraint(WfnType state) const { + return overlap(state) == count_ and + spin_wfn_traits::count(symmetric_difference(state) >> C_min_) == 0; + } + + + +}; + + +} diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index 447d95d2..cca0bacb 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -280,9 +280,6 @@ asci_contrib_container> asci_contributions_constraint( auto size_before = asci_pairs.size(); const double h_el_tol = asci_settings.h_el_tol; - const auto& [C, B, C_min] = con; - wfn_constraint alpha_con{ wfn_traits::alpha_string(C), wfn_traits::alpha_string(B), C_min}; - //wfn_t O = full_mask(norb); // Loop over unique alpha strings for(size_t i_alpha = 0; i_alpha < nuniq_alpha; ++i_alpha) { @@ -297,7 +294,7 @@ asci_contrib_container> asci_contributions_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_singles_contributions_ss( - coeff, det|beta, alpha_con, occ_alpha, occ_beta, + coeff, det|beta, con, occ_alpha, occ_beta, orb_ens_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -310,7 +307,7 @@ asci_contrib_container> asci_contributions_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_doubles_contributions_ss( - coeff, det|beta, alpha_con, occ_alpha, occ_beta, + coeff, det|beta, con, occ_alpha, occ_beta, orb_ens_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -325,14 +322,14 @@ asci_contrib_container> asci_contributions_constraint( const auto& orb_ens_alpha = bcd.orb_ens_alpha; const auto& orb_ens_beta = bcd.orb_ens_beta; generate_constraint_doubles_contributions_os( - coeff, det|beta, alpha_con, occ_alpha, occ_beta, vir_beta, + coeff, det|beta, con, occ_alpha, occ_beta, vir_beta, orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } // If the alpha determinant satisfies the constraint, // append BB and BBBB excitations - if(satisfies_constraint(det, con)) { + if(satisfies_constraint(wfn_traits::alpha_string(det), con)) { for(const auto& bcd : uad[i_alpha].bcd) { const auto& beta = bcd.beta_string; const auto& coeff = bcd.coeff; @@ -368,7 +365,7 @@ asci_contrib_container> asci_contributions_constraint( }); asci_pairs.erase(it, asci_pairs.end()); - auto c_indices = bits_to_indices(C); + auto c_indices = bits_to_indices(con.C()); std::string c_string; for(int i = 0; i < c_indices.size(); ++i) c_string += std::to_string(c_indices[i]) + " "; diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index b8866cf9..a184c76a 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -12,33 +12,29 @@ #include #include +#include + namespace macis { -template -struct wfn_constraint { - wfn_t C; - wfn_t B; - unsigned C_min; -}; -template -bool satisfies_constraint(wfn_t det, wfn_constraint constraint) { - auto C = constraint.C; auto C_min = constraint.C_min; - return (det & C).count() == C.count() and ((det ^ C) >> C_min).count() == 0; +template +bool satisfies_constraint(wfn_t det, ConType C) { + return C.satisfies_constraint(det); } -template -auto generate_constraint_single_excitations(wfn_t det, wfn_constraint constraint) { - const auto C = constraint.C; const auto B = constraint.B; - if((det & C).count() < - (C.count() - 1)) // need to have at most one different from the constraint +template +auto generate_constraint_single_excitations(wfn_t det, ConType constraint) { + using spin_wfn_traits = typename ConType::spin_wfn_traits; + const auto C = constraint.C(); const auto B = constraint.B(); + + // need to have at most one different from the constraint + if(constraint.overlap(det) < (constraint.count()-1)) return std::make_pair(wfn_t(0), wfn_t(0)); auto o = det ^ C; auto v = (~det) & B; - if((o & C).count() == - 1) { // don't have to change this necessarily, but more clear without >= + if((o & C).count() == 1) { v = o & C; o ^= v; } @@ -50,9 +46,9 @@ auto generate_constraint_single_excitations(wfn_t det, wfn_constraint cons return std::make_pair(o, v); } -template -auto generate_constraint_double_excitations(wfn_t det, wfn_constraint constraint) { - const auto C = constraint.C; const auto B = constraint.B; +template +auto generate_constraint_double_excitations(wfn_t det, ConType constraint) { + const auto C = constraint.C(); const auto B = constraint.B(); // Occ/Vir pairs to generate excitations std::vector> O, V; @@ -102,8 +98,8 @@ auto generate_constraint_double_excitations(wfn_t det, wfn_constraint cons return std::make_tuple(O, V); } -template -void generate_constraint_singles(wfn_t det, wfn_constraint constraint, +template +void generate_constraint_singles(wfn_t det, ConType constraint, std::vector>& t_singles) { auto [o, v] = generate_constraint_single_excitations(det, constraint); const auto oc = o.count(); @@ -128,8 +124,8 @@ unsigned count_constraint_singles(Args&&... args) { return o.count() * v.count(); } -template -void generate_constraint_doubles(wfn_t det, wfn_constraint constraint, +template +void generate_constraint_doubles(wfn_t det, ConType constraint, std::vector>& t_doubles) { auto [O, V] = generate_constraint_double_excitations(det, constraint); @@ -147,9 +143,9 @@ void generate_constraint_doubles(wfn_t det, wfn_constraint constraint, * @param[in] T Triplet constraint mask * @param[in] B B mask (?) */ -template -unsigned count_constraint_doubles(wfn_t det, wfn_constraint constraint) { - const auto C = constraint.C; const auto B = constraint.B; +template +unsigned count_constraint_doubles(wfn_t det, ConType constraint) { + const auto C = constraint.C(); const auto B = constraint.B(); if((det & C) == 0) return 0; auto o = det ^ C; @@ -193,9 +189,9 @@ unsigned count_constraint_doubles(wfn_t det, wfn_constraint constraint) { return no_pairs * nv_pairs; } -template +template size_t constraint_histogram(wfn_t det, size_t n_os_singles, - size_t n_os_doubles, wfn_constraint constraint){ + size_t n_os_doubles, ConType constraint){ auto ns = count_constraint_singles(det, constraint); auto nd = count_constraint_doubles(det, constraint); @@ -461,16 +457,18 @@ auto dist_triplets_histogram(size_t norb, size_t ns_othr, size_t nd_othr, template auto make_triplet(unsigned i, unsigned j, unsigned k) { - wfn_constraint con; - - con.C = 0; - con.C.flip(i).flip(j).flip(k); - con.B = 1; - con.B <<= k; - con.B = con.B.to_ullong() - 1; - con.C_min = k; - - return con; + using wfn_type = wfn_t; + using wfn_traits = wavefunction_traits; + using constraint_type = alpha_constraint; + using string_type = typename constraint_type::constraint_type; + + string_type C = 0; + C.flip(i).flip(j).flip(k); + string_type B = 1; + B <<= k; + B = B.to_ullong() - 1; + + return constraint_type(C,B,k); } #ifdef MACIS_ENABLE_MPI @@ -479,6 +477,10 @@ auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, size_t nd_othr, const std::vector>& unique_alpha, MPI_Comm comm) { + using wfn_type = wfn_t; + using wfn_traits = wavefunction_traits; + using constraint_type = alpha_constraint; + using string_type = typename constraint_type::constraint_type; auto world_rank = comm_rank(comm); auto world_size = comm_size(comm); @@ -488,18 +490,17 @@ auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, std::vector workloads(world_size, 0); // Generate triplets + heuristic - std::vector, size_t>> constraint_sizes; + std::vector> constraint_sizes; constraint_sizes.reserve(norb * norb * norb); size_t total_work = 0; for(int t_i = 0; t_i < norb; ++t_i) for(int t_j = 0; t_j < t_i; ++t_j) for(int t_k = 0; t_k < t_j; ++t_k) { auto constraint = make_triplet(t_i, t_j, t_k); - const auto& [T, B, _] = constraint; size_t nw = 0; for(const auto& alpha : unique_alpha) { - nw += constraint_histogram(alpha, ns_othr, nd_othr, constraint); + nw += constraint_histogram(wfn_traits::alpha_string(alpha), ns_othr, nd_othr, constraint); } if(nw) constraint_sizes.emplace_back(constraint, nw); total_work += nw; @@ -509,7 +510,7 @@ auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, for(size_t ilevel = 0; ilevel < nlevels; ++ilevel) { // Select constraints larger than average to be broken apart - std::vector, size_t>> tps_to_next; + std::vector> tps_to_next; { auto it = std::partition( constraint_sizes.begin(), constraint_sizes.end(), @@ -525,20 +526,20 @@ auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, // Break apart constraints for(auto [c, nw_trip] : tps_to_next) { - const auto C_min = c.C_min; + const auto C_min = c.C_min(); // Loop over possible constraints with one more element for(auto q_l = 0; q_l < C_min; ++q_l) { // Generate masks / counts - wfn_constraint c_next = c; - c_next.C.flip(q_l); - c_next.B >>= (C_min - q_l); - c_next.C_min = q_l; + string_type cn_C = c.C(); + cn_C.flip(q_l); + string_type cn_B = c.B() >> (C_min - q_l); + constraint_type c_next(cn_C, cn_B, q_l); size_t nw = 0; for(const auto& alpha : unique_alpha) { - nw += constraint_histogram(alpha, ns_othr, nd_othr, c_next); + nw += constraint_histogram(wfn_traits::alpha_string(alpha), ns_othr, nd_othr, c_next); } if(nw) constraint_sizes.emplace_back(c_next, nw); total_work += nw; @@ -569,7 +570,7 @@ auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, [](const auto& a, const auto& b) { return a.second > b.second; }); // Assign work - std::vector> constraints; + std::vector constraints; constraints.reserve(constraint_sizes.size() / world_size); for(auto [c, nw] : constraint_sizes) { diff --git a/include/macis/asci/pt2.hpp b/include/macis/asci/pt2.hpp index b560597c..d7cf7c46 100644 --- a/include/macis/asci/pt2.hpp +++ b/include/macis/asci/pt2.hpp @@ -130,8 +130,6 @@ double asci_pt2_constraint( const auto& con = constraints[ic]; //std::cout << std::distance(&constraints[0], &con) << "/" << constraints.size() << std::endl; const double h_el_tol = 1e-16; - const auto& [C, B, C_min] = con; - wfn_constraint alpha_con{ wfn_traits::alpha_string(C), wfn_traits::alpha_string(B), C_min}; // Loop over unique alpha strings for(size_t i_alpha = 0; i_alpha < nuniq_alpha; ++i_alpha) { @@ -146,7 +144,7 @@ double asci_pt2_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_singles_contributions_ss( - coeff, det|beta, alpha_con, occ_alpha, occ_beta, + coeff, det|beta, con, occ_alpha, occ_beta, orb_ens_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -159,7 +157,7 @@ double asci_pt2_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_doubles_contributions_ss( - coeff, det|beta, alpha_con, occ_alpha, occ_beta, + coeff, det|beta, con, occ_alpha, occ_beta, orb_ens_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -174,14 +172,14 @@ double asci_pt2_constraint( const auto& orb_ens_alpha = bcd.orb_ens_alpha; const auto& orb_ens_beta = bcd.orb_ens_beta; generate_constraint_doubles_contributions_os( - coeff, det|beta, alpha_con, occ_alpha, occ_beta, vir_beta, + coeff, det|beta, con, occ_alpha, occ_beta, vir_beta, orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } // If the alpha determinant satisfies the constraint, // append BB and BBBB excitations - if(satisfies_constraint(det, con)) { + if(satisfies_constraint(wfn_traits::alpha_string(det), con)) { for(const auto& bcd : uad[i_alpha].bcd) { const auto& beta = bcd.beta_string; const auto& coeff = bcd.coeff; diff --git a/tests/asci.cxx b/tests/asci.cxx index f088f853..05ef72c0 100644 --- a/tests/asci.cxx +++ b/tests/asci.cxx @@ -47,16 +47,18 @@ size_t top_set_ordinal(std::bitset word, size_t NSet) { template auto make_quad(unsigned i, unsigned j, unsigned k, unsigned l) { - macis::wfn_constraint con; + using wfn_type = macis::wfn_t; + using wfn_traits = macis::wavefunction_traits; + using constraint_type = macis::alpha_constraint; + using string_type = typename constraint_type::constraint_type; - con.C = 0; - con.C.flip(i).flip(j).flip(k).flip(l); - con.B = 1; - con.B <<= l; - con.B = con.B.to_ullong() - 1; - con.C_min = l; + string_type C = 0; + C.flip(i).flip(j).flip(k).flip(l); + string_type B = 1; + B <<= l; + B = B.to_ullong() - 1; - return con; + return constraint_type(C,B,l); } TEST_CASE("Triplets") { @@ -64,6 +66,8 @@ TEST_CASE("Triplets") { size_t norb = 32; using wfn_less_comparator = macis::bitset_less_comparator; + using wfn_type = macis::wfn_t; + using wfn_traits = macis::wavefunction_traits; // Generate ficticious wfns std::vector> wfn_a = { @@ -186,7 +190,7 @@ TEST_CASE("Triplets") { const size_t n_doubles = (n_singles * (n_singles - nocc - nvir + 1)) / 4; new_triplet_hist[label] += macis::constraint_histogram( - det, n_singles, n_doubles, constraint); + wfn_traits::alpha_string(det), n_singles, n_doubles, constraint); } } @@ -213,7 +217,7 @@ TEST_CASE("Triplets") { const size_t n_doubles = (n_singles * (n_singles - nocc - nvir + 1)) / 4; new_quad_hist[label] += macis::constraint_histogram( - det, n_singles, n_doubles, constraint); + wfn_traits::alpha_string(det), n_singles, n_doubles, constraint); } } From 29e8fc80c8e6910e41a70cbac790050d5129de1e Mon Sep 17 00:00:00 2001 From: "license[bot]" Date: Wed, 13 Sep 2023 22:46:20 +0000 Subject: [PATCH 20/73] Committing license headers --- include/macis/asci/alpha_constraint.hpp | 8 ++++++++ include/macis/util/unused_untested.hpp | 8 ++++++++ include/macis/wfn/raw_bitset.hpp | 8 ++++++++ src/macis/hamiltonian_generator/base.cxx | 8 ++++++++ 4 files changed, 32 insertions(+) diff --git a/include/macis/asci/alpha_constraint.hpp b/include/macis/asci/alpha_constraint.hpp index 4d0ca2be..330e3bd7 100644 --- a/include/macis/asci/alpha_constraint.hpp +++ b/include/macis/asci/alpha_constraint.hpp @@ -1,3 +1,11 @@ +/* + * MACIS Copyright (c) 2023, The Regents of the University of California, + * through Lawrence Berkeley National Laboratory (subject to receipt of + * any required approvals from the U.S. Dept. of Energy). All rights reserved. + * + * See LICENSE.txt for details + */ + #pragma once #include diff --git a/include/macis/util/unused_untested.hpp b/include/macis/util/unused_untested.hpp index 2288c435..f348e00a 100644 --- a/include/macis/util/unused_untested.hpp +++ b/include/macis/util/unused_untested.hpp @@ -1,3 +1,11 @@ +/* + * MACIS Copyright (c) 2023, The Regents of the University of California, + * through Lawrence Berkeley National Laboratory (subject to receipt of + * any required approvals from the U.S. Dept. of Energy). All rights reserved. + * + * See LICENSE.txt for details + */ + #if 0 /** diff --git a/include/macis/wfn/raw_bitset.hpp b/include/macis/wfn/raw_bitset.hpp index 04c096f2..4da3bf26 100644 --- a/include/macis/wfn/raw_bitset.hpp +++ b/include/macis/wfn/raw_bitset.hpp @@ -1,3 +1,11 @@ +/* + * MACIS Copyright (c) 2023, The Regents of the University of California, + * through Lawrence Berkeley National Laboratory (subject to receipt of + * any required approvals from the U.S. Dept. of Energy). All rights reserved. + * + * See LICENSE.txt for details + */ + #pragma once #include diff --git a/src/macis/hamiltonian_generator/base.cxx b/src/macis/hamiltonian_generator/base.cxx index e96ce11a..e376fae7 100644 --- a/src/macis/hamiltonian_generator/base.cxx +++ b/src/macis/hamiltonian_generator/base.cxx @@ -1,3 +1,11 @@ +/* + * MACIS Copyright (c) 2023, The Regents of the University of California, + * through Lawrence Berkeley National Laboratory (subject to receipt of + * any required approvals from the U.S. Dept. of Energy). All rights reserved. + * + * See LICENSE.txt for details + */ + #include "base.ipp" #include "fast_diagonals.ipp" From 840e80e6ec84b93c362c80f6e312eeb7abf2d89b Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Fri, 22 Sep 2023 15:33:42 -0700 Subject: [PATCH 21/73] Added serious unit tests for constraint generation code + misc consistency changes --- include/macis/asci/alpha_constraint.hpp | 11 +- include/macis/asci/mask_constraints.hpp | 58 ++++++---- include/macis/wfn/raw_bitset.hpp | 19 ++++ tests/asci.cxx | 141 +++++++++++++++++++++++- 4 files changed, 198 insertions(+), 31 deletions(-) diff --git a/include/macis/asci/alpha_constraint.hpp b/include/macis/asci/alpha_constraint.hpp index 4d0ca2be..56d19d53 100644 --- a/include/macis/asci/alpha_constraint.hpp +++ b/include/macis/asci/alpha_constraint.hpp @@ -10,8 +10,9 @@ class alpha_constraint { using wfn_traits = WfnTraits; using wfn_type = typename WfnTraits::wfn_type; using spin_wfn_type = spin_wfn_t; - using spin_wfn_traits = wavefunction_traits; - using constraint_type = spin_wfn_type; + + using constraint_type = spin_wfn_type; + using constraint_traits = wavefunction_traits; private: constraint_type C_; @@ -22,7 +23,7 @@ class alpha_constraint { public: alpha_constraint(constraint_type C, constraint_type B, uint32_t C_min) : - C_(C), B_(B), C_min_(C_min), count_(spin_wfn_traits::count(C)) {} + C_(C), B_(B), C_min_(C_min), count_(constraint_traits::count(C)) {} alpha_constraint(const alpha_constraint&) = default; alpha_constraint& operator=(const alpha_constraint&) = default; @@ -53,13 +54,13 @@ class alpha_constraint { template inline auto overlap(WfnType state) const { - return spin_wfn_traits::count(c_mask_union(state)); + return constraint_traits::count(c_mask_union(state)); } template inline bool satisfies_constraint(WfnType state) const { return overlap(state) == count_ and - spin_wfn_traits::count(symmetric_difference(state) >> C_min_) == 0; + constraint_traits::count(symmetric_difference(state) >> C_min_) == 0; } diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index a3c1fa57..251a59e6 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -17,62 +17,71 @@ namespace macis { -template -bool satisfies_constraint(wfn_t det, ConType C) { +template +bool satisfies_constraint(WfnType det, ConType C) { return C.satisfies_constraint(det); } -template -auto generate_constraint_single_excitations(wfn_t det, ConType constraint) { - using spin_wfn_traits = typename ConType::spin_wfn_traits; +template +auto generate_constraint_single_excitations(WfnType det, ConType constraint) { + using constraint_traits = typename ConType::constraint_traits; const auto C = constraint.C(); const auto B = constraint.B(); // need to have at most one different from the constraint if(constraint.overlap(det) < (constraint.count()-1)) - return std::make_pair(wfn_t(0), wfn_t(0)); + return std::make_pair(WfnType(0), WfnType(0)); - auto o = det ^ C; - auto v = (~det) & B; + auto o = constraint.symmetric_difference(det); + auto v = constraint.b_mask_union(~det); - if((o & C).count() == 1) { + if(constraint_traits::count(o & C) == 1) { v = o & C; o ^= v; } - if((o & ~B).count() > 1) return std::make_pair(wfn_t(0), wfn_t(0)); + const auto o_and_not_b = o & ~B; + const auto o_and_not_b_count = constraint_traits::count(o_and_not_b); + if(o_and_not_b_count > 1) return std::make_pair(WfnType(0), WfnType(0)); - if((o & ~B).count() == 1) o &= ~B; + if(o_and_not_b_count == 1) o = o_and_not_b; return std::make_pair(o, v); } template auto generate_constraint_double_excitations(wfn_t det, ConType constraint) { + using constraint_traits = typename ConType::constraint_traits; const auto C = constraint.C(); const auto B = constraint.B(); // Occ/Vir pairs to generate excitations std::vector> O, V; - if((det & C) == 0) return std::make_tuple(O, V); + if(constraint.overlap(det) == 0) return std::make_tuple(O, V); - auto o = det ^ C; - auto v = (~det) & B; + auto o = constraint.symmetric_difference(det); + auto v = constraint.b_mask_union(~det); - if((o & C).count() >= 3) return std::make_tuple(O, V); + auto o_and_c = o & C; + auto o_and_c_count = constraint_traits::count(o_and_c); + if(o_and_c_count >= 3) return std::make_tuple(O, V); // Generate Virtual Pairs - if((o & C).count() == 2) { - v = o & C; + if(o_and_c_count == 2) { + v = o_and_c; o ^= v; + // Regenerate since o changed + // XXX: This apparently is not needed, but leaving because + o_and_c = o & C; + o_and_c_count = constraint_traits::count(o_and_c); } + const auto virt_ind = bits_to_indices(v); - const auto o_and_t = o & C; - switch((o & C).count()) { + switch(o_and_c_count) { case 1: for(auto a : virt_ind) { - V.emplace_back(o_and_t).flip(a); + V.emplace_back(o_and_c).flip(a); } - o ^= o_and_t; + o ^= o_and_c; break; default: generate_pairs(virt_ind, V); @@ -81,16 +90,17 @@ auto generate_constraint_double_excitations(wfn_t det, ConType constraint) { // Generate Occupied Pairs const auto o_and_not_b = o & ~B; - if(o_and_not_b.count() > 2) return std::make_tuple(O, V); + const auto o_and_not_b_count = constraint_traits::count(o_and_not_b); + if(o_and_not_b_count > 2) return std::make_tuple(O, V); - switch(o_and_not_b.count()) { + switch(o_and_not_b_count) { case 1: for(auto i : bits_to_indices(o & B)) { O.emplace_back(o_and_not_b).flip(i); } break; default: - if(o_and_not_b.count() == 2) o = o_and_not_b; + if(o_and_not_b_count == 2) o = o_and_not_b; generate_pairs(bits_to_indices(o), O); break; } diff --git a/include/macis/wfn/raw_bitset.hpp b/include/macis/wfn/raw_bitset.hpp index 04c096f2..356c1c3b 100644 --- a/include/macis/wfn/raw_bitset.hpp +++ b/include/macis/wfn/raw_bitset.hpp @@ -38,6 +38,25 @@ struct wavefunction_traits> { return bitset_hi_word(state); } + using wfn_comparator = bitset_less_comparator; + + + struct spin_comparator { + using spin_wfn_comparator = bitset_less_comparator; + bool operator()(wfn_type x, wfn_type y) const { + auto s_comp = spin_wfn_comparator{}; + const auto x_a = alpha_string(x); + const auto y_a = alpha_string(y); + if( x_a == y_a ) { + const auto x_b = beta_string(x); + const auto y_b = beta_string(y); + return s_comp(x_b, y_b); + } else return s_comp(x_a, y_a); + } + }; + + + template static inline wfn_type from_spin(spin_wfn_type alpha, spin_wfn_type beta) { if constexpr (Sigma == Spin::Alpha) { diff --git a/tests/asci.cxx b/tests/asci.cxx index 05ef72c0..829b0357 100644 --- a/tests/asci.cxx +++ b/tests/asci.cxx @@ -224,6 +224,143 @@ TEST_CASE("Triplets") { REQUIRE(quad_hist == new_quad_hist); } + +TEST_CASE("Constraints") { + + using wfn_type = macis::wfn_t<64>; + using wfn_traits = macis::wavefunction_traits; + using spin_wfn_type = typename wfn_traits::spin_wfn_type; + using spin_wfn_traits = macis::wavefunction_traits; + using wfn_comparator = typename wfn_traits::spin_comparator; + using spin_wfn_comparator = typename spin_wfn_traits::wfn_comparator; + + using constraint_type = macis::alpha_constraint; + + const size_t norb = 10; + size_t nalpha, nbeta; + + SECTION("Closed Shell") { + nalpha = 6; + nbeta = 6; + } + + SECTION("Open Shell") { + nalpha = 6; + nbeta = 3; + } + + // Generate Hilbert Space + auto dets = macis::generate_hilbert_space(norb, nalpha, nbeta); + std::sort(dets.begin(), dets.end(), wfn_comparator{}); // lex sort + + // Get Alpha Compression Data + std::vector> unique_alpha; + unique_alpha.push_back( {wfn_traits::alpha_string(dets[0]), 1} ); + for(size_t i = 1; i < dets.size(); ++i) { + auto& [cur_alpha, cur_count] = unique_alpha.back(); + auto alpha_i = wfn_traits::alpha_string(dets[i]); + if(alpha_i == cur_alpha) { cur_count++; } + else { + unique_alpha.push_back({alpha_i, 1}); + } + } + + // Get offsets + std::vector unique_alpha_offsets(unique_alpha.size()); + std::transform_exclusive_scan(unique_alpha.begin(), unique_alpha.end(), + unique_alpha_offsets.begin(), 0ul, std::plus(), + [](auto p){ return p.second; } ); + + //size_t ntot = std::accumulate( unique_alpha.begin(), unique_alpha.end(), + // 0ul, [](auto s, auto a){ return s + a.second; } ); + //REQUIRE(ntot == dets.size()); + + // Generate constraints + std::vector triplets, quads; + for(int i = 0; i < norb; ++i) + for(int j = 0; j < i; ++j) + for(int k = 0; k < j; ++k) { + triplets.emplace_back(macis::make_triplet<64>(i,j,k)); + for(int l = 0; l < k; ++l) { + quads.emplace_back(make_quad<64>(i,j,k,l)); + } + } + + // Check doubles + auto check_doubles = []( auto det, auto C, auto& doubles ) { + // Sanity check + auto [_O, _V] = macis::generate_constraint_double_excitations(det, C); + REQUIRE(std::all_of(_O.begin(), _O.end(), [](auto e){ return spin_wfn_traits::count(e) == 2; })); + REQUIRE(std::all_of(_V.begin(), _V.end(), [](auto e){ return spin_wfn_traits::count(e) == 2; })); + + // Extract all double excitations that satisfy the constraint + std::vector doubles_c; + std::copy_if(doubles.begin(), doubles.end(), std::back_inserter(doubles_c), + [=](auto d){ return C.satisfies_constraint(d); }); + + // Generate all double excitations that satisfy the constraint + std::vector doubles_g; + macis::generate_constraint_doubles(det, C, doubles_g); + + // Compare and check counting + std::sort(doubles_c.begin(), doubles_c.end(), spin_wfn_comparator{}); + std::sort(doubles_g.begin(), doubles_g.end(), spin_wfn_comparator{}); + REQUIRE( doubles_c == doubles_g ); + REQUIRE( doubles_g.size() == macis::count_constraint_doubles(det, C) ); + }; + + // Check singles + auto check_singles = []( auto det, auto C, auto& singles ) { + // Extract all double excitations that satisfy the constraint + std::vector singles_c; + std::copy_if(singles.begin(), singles.end(), std::back_inserter(singles_c), + [=](auto d){ return C.satisfies_constraint(d); }); + + // Generate all double excitations that satisfy the constraint + std::vector singles_g; + macis::generate_constraint_singles(det, C, singles_g); + + // Compare and check counting + std::sort(singles_c.begin(), singles_c.end(), spin_wfn_comparator{}); + std::sort(singles_g.begin(), singles_g.end(), spin_wfn_comparator{}); + REQUIRE( singles_c == singles_g ); + REQUIRE( singles_g.size() == macis::count_constraint_singles(det, C) ); + }; + + for(auto i = 0; i < unique_alpha.size(); ++i) { + auto det = unique_alpha[i].first; + + auto det_triplet = top_set_indices<3>(det); + auto det_quad = top_set_indices<4>(det); + + std::vector singles, doubles; + macis::generate_singles(norb, det, singles); + macis::generate_doubles(norb, det, doubles); + + for( auto C : triplets ) { + // Check validity of constraint check + auto inds = top_set_indices<3>(C.C()); + REQUIRE(C.C_min() == inds.back()); + REQUIRE(C.satisfies_constraint(det) == (inds == det_triplet)); + + check_singles(det, C, singles); + check_doubles(det, C, doubles); + } + + for( auto C : quads ) { + // Check validity of constraint check + auto inds = top_set_indices<4>(C.C()); + REQUIRE(C.C_min() == inds.back()); + REQUIRE(C.satisfies_constraint(det) == (inds == det_quad)); + + check_singles(det, C, singles); + check_doubles(det, C, doubles); + } + } + + +} + TEST_CASE("ASCI") { MACIS_MPI_CODE(MPI_Barrier(MPI_COMM_WORLD);) using macis::NumActive; @@ -297,8 +434,8 @@ TEST_CASE("ASCI") { ham_gen.T(), ham_gen.G_red(), ham_gen.V_red(),ham_gen.G(), ham_gen.V(), ham_gen MACIS_MPI_CODE(, MPI_COMM_WORLD)); - std::cout << std::scientific << std::setprecision(12); - std::cout << EPT2 << std::endl; + //std::cout << std::scientific << std::setprecision(12); + //std::cout << EPT2 << std::endl; REQUIRE(std::abs(EPT2 - -5.701585096318e-03) < 1e-10); MACIS_MPI_CODE(MPI_Barrier(MPI_COMM_WORLD);) From 4555334ea51b6ca924e8c27073a773d01ec0b5c6 Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Fri, 22 Sep 2023 15:56:22 -0700 Subject: [PATCH 22/73] Further generalizations of ASCI constraint code --- include/macis/asci/alpha_constraint.hpp | 6 +-- include/macis/asci/mask_constraints.hpp | 54 ++++++++++++++----------- 2 files changed, 34 insertions(+), 26 deletions(-) diff --git a/include/macis/asci/alpha_constraint.hpp b/include/macis/asci/alpha_constraint.hpp index 56d19d53..000e9619 100644 --- a/include/macis/asci/alpha_constraint.hpp +++ b/include/macis/asci/alpha_constraint.hpp @@ -48,9 +48,9 @@ class alpha_constraint { inline spin_wfn_type symmetric_difference(spin_wfn_type state) const { return state ^ C_; } - inline spin_wfn_type symmetric_difference(wfn_type state) const { - return symmetric_difference(wfn_traits::alpha_string(state)); - } + //inline spin_wfn_type symmetric_difference(wfn_type state) const { + // return symmetric_difference(wfn_traits::alpha_string(state)); + //} template inline auto overlap(WfnType state) const { diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index 251a59e6..02596c30 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -48,12 +48,13 @@ auto generate_constraint_single_excitations(WfnType det, ConType constraint) { return std::make_pair(o, v); } -template -auto generate_constraint_double_excitations(wfn_t det, ConType constraint) { +template +auto generate_constraint_double_excitations(WfnType det, ConType constraint) { using constraint_traits = typename ConType::constraint_traits; + using constraint_type = typename ConType::constraint_type; const auto C = constraint.C(); const auto B = constraint.B(); // Occ/Vir pairs to generate excitations - std::vector> O, V; + std::vector O, V; if(constraint.overlap(det) == 0) return std::make_tuple(O, V); @@ -108,9 +109,9 @@ auto generate_constraint_double_excitations(wfn_t det, ConType constraint) { return std::make_tuple(O, V); } -template -void generate_constraint_singles(wfn_t det, ConType constraint, - std::vector>& t_singles) { +template +void generate_constraint_singles(WfnType det, ConType constraint, + std::vector& t_singles) { auto [o, v] = generate_constraint_single_excitations(det, constraint); const auto oc = o.count(); const auto vc = v.count(); @@ -134,9 +135,9 @@ unsigned count_constraint_singles(Args&&... args) { return o.count() * v.count(); } -template -void generate_constraint_doubles(wfn_t det, ConType constraint, - std::vector>& t_doubles) { +template +void generate_constraint_doubles(WfnType det, ConType constraint, + std::vector& t_doubles) { auto [O, V] = generate_constraint_double_excitations(det, constraint); t_doubles.clear(); @@ -155,25 +156,31 @@ void generate_constraint_doubles(wfn_t det, ConType constraint, */ template unsigned count_constraint_doubles(wfn_t det, ConType constraint) { + using constraint_traits = typename ConType::constraint_traits; const auto C = constraint.C(); const auto B = constraint.B(); if((det & C) == 0) return 0; auto o = det ^ C; auto v = (~det) & B; - if((o & C).count() >= 3) return 0; + auto o_and_c = o & C; + auto o_and_c_count = constraint_traits::count(o_and_c); + if(o_and_c_count >= 3) return 0; // Generate Virtual Pairs - if((o & C).count() == 2) { - v = o & C; + if(o_and_c_count == 2) { + v = o_and_c; o ^= v; + // Regenerate since o changed + // XXX: This apparently is not needed, but leaving because + o_and_c = o & C; + o_and_c_count = constraint_traits::count(o_and_c); } - unsigned nv_pairs = v.count(); - const auto o_and_t = o & C; - switch((o & C).count()) { + unsigned nv_pairs = constraint_traits::count(v); + switch(o_and_c_count) { case 1: - o ^= o_and_t; + o ^= o_and_c; break; default: nv_pairs = (nv_pairs * (nv_pairs - 1)) / 2; @@ -182,16 +189,17 @@ unsigned count_constraint_doubles(wfn_t det, ConType constraint) { // Generate Occupied Pairs const auto o_and_not_b = o & ~B; - if(o_and_not_b.count() > 2) return 0; + const auto o_and_not_b_count = constraint_traits::count(o_and_not_b); + if(o_and_not_b_count > 2) return 0; unsigned no_pairs = 0; - switch(o_and_not_b.count()) { + switch(o_and_not_b_count) { case 1: - no_pairs = (o & B).count(); + no_pairs = constraint_traits::count(o & B); break; default: - if(o_and_not_b.count() == 2) o = o_and_not_b; - no_pairs = o.count(); + if(o_and_not_b_count == 2) o = o_and_not_b; + no_pairs = constraint_traits::count(o); no_pairs = (no_pairs * (no_pairs - 1)) / 2; break; } @@ -199,8 +207,8 @@ unsigned count_constraint_doubles(wfn_t det, ConType constraint) { return no_pairs * nv_pairs; } -template -size_t constraint_histogram(wfn_t det, size_t n_os_singles, +template +size_t constraint_histogram(WfnType det, size_t n_os_singles, size_t n_os_doubles, ConType constraint){ auto ns = count_constraint_singles(det, constraint); auto nd = count_constraint_doubles(det, constraint); From 947a351d381db730d9f44d842f76b7bf10cedb2d Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Fri, 22 Sep 2023 16:17:31 -0700 Subject: [PATCH 23/73] More generalization of constraint code: removal of most bitset::flip invocations --- include/macis/asci/mask_constraints.hpp | 58 ++++++++++++++----------- include/macis/wfn/raw_bitset.hpp | 4 ++ 2 files changed, 36 insertions(+), 26 deletions(-) diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index 02596c30..07cf196f 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -80,7 +80,7 @@ auto generate_constraint_double_excitations(WfnType det, ConType constraint) { switch(o_and_c_count) { case 1: for(auto a : virt_ind) { - V.emplace_back(o_and_c).flip(a); + V.emplace_back(constraint_traits::create_no_check(o_and_c,a)); } o ^= o_and_c; break; @@ -97,7 +97,7 @@ auto generate_constraint_double_excitations(WfnType det, ConType constraint) { switch(o_and_not_b_count) { case 1: for(auto i : bits_to_indices(o & B)) { - O.emplace_back(o_and_not_b).flip(i); + O.emplace_back(constraint_traits::create_no_check(o_and_not_b,i)); } break; default: @@ -112,27 +112,31 @@ auto generate_constraint_double_excitations(WfnType det, ConType constraint) { template void generate_constraint_singles(WfnType det, ConType constraint, std::vector& t_singles) { + using constraint_traits = typename ConType::constraint_traits; auto [o, v] = generate_constraint_single_excitations(det, constraint); - const auto oc = o.count(); - const auto vc = v.count(); + const auto oc = constraint_traits::count(o); + const auto vc = constraint_traits::count(v); if(!oc or !vc) return; t_singles.clear(); t_singles.reserve(oc * vc); - const auto occ = bits_to_indices(o); - const auto vir = bits_to_indices(v); + const auto occ = constraint_traits::state_to_occ(o); + const auto vir = constraint_traits::state_to_occ(v); for(auto i : occ) { - auto temp = det; - temp.flip(i); - for(auto a : vir) t_singles.emplace_back(temp).flip(a); + auto temp = constraint_traits::create_no_check(det, i); + for(auto a : vir) + t_singles.emplace_back(constraint_traits::create_no_check(temp, a)); } } -template -unsigned count_constraint_singles(Args&&... args) { +template +unsigned count_constraint_singles(WfnType det, ConType constraint) { + using constraint_traits = typename ConType::constraint_traits; auto [o, v] = - generate_constraint_single_excitations(std::forward(args)...); - return o.count() * v.count(); + generate_constraint_single_excitations(det, constraint); + const auto oc = constraint_traits::count(o); + const auto vc = constraint_traits::count(v); + return oc * vc; } template @@ -154,14 +158,14 @@ void generate_constraint_doubles(WfnType det, ConType constraint, * @param[in] T Triplet constraint mask * @param[in] B B mask (?) */ -template -unsigned count_constraint_doubles(wfn_t det, ConType constraint) { +template +unsigned count_constraint_doubles(WfnType det, ConType constraint) { using constraint_traits = typename ConType::constraint_traits; const auto C = constraint.C(); const auto B = constraint.B(); - if((det & C) == 0) return 0; + if(constraint.overlap(det) == 0) return 0; - auto o = det ^ C; - auto v = (~det) & B; + auto o = constraint.symmetric_difference(det); + auto v = constraint.b_mask_union(~det); auto o_and_c = o & C; auto o_and_c_count = constraint_traits::count(o_and_c); @@ -234,20 +238,21 @@ void generate_constraint_singles_contributions_ss( double E0, HamiltonianGeneratorBase& ham_gen, asci_contrib_container& asci_contributions) { using wfn_traits = wavefunction_traits; + using constraint_traits = typename ConType::constraint_traits; auto [o, v] = generate_constraint_single_excitations(wfn_traits::alpha_string(det), constraint); - const auto no = o.count(); - const auto nv = v.count(); + const auto no = constraint_traits::count(o); + const auto nv = constraint_traits::count(v); if(!no or !nv) return; const size_t LDG2 = LDG * LDG; const size_t LDV2 = LDV * LDV; for(int ii = 0; ii < no; ++ii) { const auto i = fls(o); - o.flip(i); // Disable "i"-bit so it's not used in FLS next iteration + o = constraint_traits::create_no_check(o, i); // o.flip(i) auto v_cpy = v; for(int aa = 0; aa < nv; ++aa) { const auto a = fls(v_cpy); - v_cpy.flip(a); // Disable "a"-bit so it's not used in FLS next iteration + v_cpy = constraint_traits::create_no_check(v_cpy, a); // v_cpy.flip(a) double h_el = T_pq[a + i * LDT]; const double* G_ov = G_kpq + a * LDG + i * LDG2; @@ -340,20 +345,21 @@ void generate_constraint_doubles_contributions_os( double root_diag, double E0, HamiltonianGeneratorBase& ham_gen, asci_contrib_container& asci_contributions) { using wfn_traits = wavefunction_traits; + using constraint_traits = typename ConType::constraint_traits; // Generate Single Excitations that Satisfy the Constraint auto [o, v] = generate_constraint_single_excitations(wfn_traits::alpha_string(det), constraint); - const auto no = o.count(); - const auto nv = v.count(); + const auto no = constraint_traits::count(o); + const auto nv = constraint_traits::count(v); if(!no or !nv) return; const size_t LDV2 = LDV * LDV; for(int ii = 0; ii < no; ++ii) { const auto i = fls(o); - o.flip(i); + o = constraint_traits::create_no_check(o, i); // o.flip(i) auto v_cpy = v; for(int aa = 0; aa < nv; ++aa) { const auto a = fls(v_cpy); - v_cpy.flip(a); + v_cpy = constraint_traits::create_no_check(v_cpy, a); // v_cpy.flip(a) const auto* V_ai = V + a + i * LDV; double sign_same = single_excitation_sign(det, a, i); diff --git a/include/macis/wfn/raw_bitset.hpp b/include/macis/wfn/raw_bitset.hpp index 356c1c3b..114d6f24 100644 --- a/include/macis/wfn/raw_bitset.hpp +++ b/include/macis/wfn/raw_bitset.hpp @@ -122,6 +122,10 @@ struct wavefunction_traits> { occ = bits_to_indices(state); } + static inline orbidx_container state_to_occ(wfn_type state) { + return bits_to_indices(state); + } + static inline void state_to_occ_vir(size_t norb, wfn_type state, orbidx_container& occ, orbidx_container& vir) { From 3eb8f139aef086e814d335df93abd8231903a035 Mon Sep 17 00:00:00 2001 From: Clang Robot Date: Mon, 25 Sep 2023 20:35:31 +0000 Subject: [PATCH 24/73] Committing clang-format changes --- include/macis/asci/alpha_constraint.hpp | 44 ++-- .../macis/asci/determinant_contributions.hpp | 32 +-- include/macis/asci/determinant_search.hpp | 28 +-- include/macis/asci/iteration.hpp | 2 +- include/macis/asci/mask_constraints.hpp | 105 +++++---- include/macis/asci/pt2.hpp | 217 +++++++++--------- include/macis/csr_hamiltonian.hpp | 9 +- include/macis/hamiltonian_generator.hpp | 11 +- include/macis/hamiltonian_generator/base.hpp | 13 +- .../hamiltonian_generator/matrix_elements.hpp | 9 +- include/macis/mcscf/cas.hpp | 11 +- include/macis/mcscf/mcscf_impl.hpp | 5 +- include/macis/mcscf/orbital_hessian.hpp | 2 +- include/macis/sd_operations.hpp | 152 ++++++------ include/macis/util/rdms.hpp | 2 +- include/macis/util/unused_untested.hpp | 1 - include/macis/wfn/raw_bitset.hpp | 78 +++---- src/macis/hamiltonian_generator/base.cxx | 1 + src/macis/moller_plesset.cxx | 2 +- tests/asci.cxx | 97 ++++---- tests/double_loop.cxx | 3 +- tests/fcidump.cxx | 2 +- tests/fock_matrices.cxx | 2 +- tests/mcscf.cxx | 2 +- tests/sd_operations.cxx | 5 +- tests/standalone_driver.cxx | 8 +- 26 files changed, 415 insertions(+), 428 deletions(-) diff --git a/include/macis/asci/alpha_constraint.hpp b/include/macis/asci/alpha_constraint.hpp index d5c9337d..2daec074 100644 --- a/include/macis/asci/alpha_constraint.hpp +++ b/include/macis/asci/alpha_constraint.hpp @@ -13,39 +13,35 @@ namespace macis { template class alpha_constraint { + public: + using wfn_traits = WfnTraits; + using wfn_type = typename WfnTraits::wfn_type; + using spin_wfn_type = spin_wfn_t; -public: - using wfn_traits = WfnTraits; - using wfn_type = typename WfnTraits::wfn_type; - using spin_wfn_type = spin_wfn_t; - - using constraint_type = spin_wfn_type; + using constraint_type = spin_wfn_type; using constraint_traits = wavefunction_traits; -private: + private: constraint_type C_; constraint_type B_; - uint32_t C_min_; - uint32_t count_; - -public: + uint32_t C_min_; + uint32_t count_; - alpha_constraint(constraint_type C, constraint_type B, uint32_t C_min) : - C_(C), B_(B), C_min_(C_min), count_(constraint_traits::count(C)) {} + public: + alpha_constraint(constraint_type C, constraint_type B, uint32_t C_min) + : C_(C), B_(B), C_min_(C_min), count_(constraint_traits::count(C)) {} alpha_constraint(const alpha_constraint&) = default; alpha_constraint& operator=(const alpha_constraint&) = default; alpha_constraint(alpha_constraint&& other) noexcept = default; alpha_constraint& operator=(alpha_constraint&&) noexcept = default; - - inline auto C() const { return C_; } - inline auto B() const { return B_; } + inline auto C() const { return C_; } + inline auto B() const { return B_; } inline auto C_min() const { return C_min_; } inline auto count() const { return count_; } - inline spin_wfn_type c_mask_union(spin_wfn_type state) const { return state & C_; } @@ -56,9 +52,9 @@ class alpha_constraint { inline spin_wfn_type symmetric_difference(spin_wfn_type state) const { return state ^ C_; } - //inline spin_wfn_type symmetric_difference(wfn_type state) const { - // return symmetric_difference(wfn_traits::alpha_string(state)); - //} + // inline spin_wfn_type symmetric_difference(wfn_type state) const { + // return symmetric_difference(wfn_traits::alpha_string(state)); + // } template inline auto overlap(WfnType state) const { @@ -67,13 +63,9 @@ class alpha_constraint { template inline bool satisfies_constraint(WfnType state) const { - return overlap(state) == count_ and + return overlap(state) == count_ and constraint_traits::count(symmetric_difference(state) >> C_min_) == 0; } - - - }; - -} +} // namespace macis diff --git a/include/macis/asci/determinant_contributions.hpp b/include/macis/asci/determinant_contributions.hpp index d29af033..301dd084 100644 --- a/include/macis/asci/determinant_contributions.hpp +++ b/include/macis/asci/determinant_contributions.hpp @@ -25,7 +25,6 @@ struct asci_contrib { template using asci_contrib_container = std::vector>; - template void append_singles_asci_contributions( double coeff, WfnType state_full, SpinWfnType state_same, @@ -52,7 +51,8 @@ void append_singles_asci_contributions( if(std::abs(h_el) < h_el_tol) continue; // Calculate Excited Determinant - auto ex_det = wfn_traits::template single_excitation_no_check(state_full, i, a); + auto ex_det = wfn_traits::template single_excitation_no_check( + state_full, i, a); // Calculate Excitation Sign in a Canonical Way auto sign = single_excitation_sign(state_same, a, i); @@ -72,10 +72,10 @@ void append_singles_asci_contributions( template void append_ss_doubles_asci_contributions( double coeff, WfnType state_full, SpinWfnType state_same, - SpinWfnType state_other, - const std::vector& ss_occ, const std::vector& vir, - const std::vector& os_occ, const double* eps_same, - const double* G, size_t LDG, double h_el_tol, double root_diag, double E0, + SpinWfnType state_other, const std::vector& ss_occ, + const std::vector& vir, const std::vector& os_occ, + const double* eps_same, const double* G, size_t LDG, double h_el_tol, + double root_diag, double E0, const HamiltonianGeneratorBase& ham_gen, asci_contrib_container& asci_contributions) { using wfn_traits = wavefunction_traits; @@ -114,14 +114,16 @@ void append_ss_doubles_asci_contributions( // TODO: Can this be made faster since the orbital indices are known // in advance? // Compute excited determinant (spin) - const auto full_ex_spin = spin_wfn_traits::double_excitation_no_check(SpinWfnType(0), i,j,a,b); + const auto full_ex_spin = spin_wfn_traits::double_excitation_no_check( + SpinWfnType(0), i, j, a, b); const auto ex_det_spin = state_same ^ full_ex_spin; // Calculate the sign in a canonical way double sign = doubles_sign(state_same, ex_det_spin, full_ex_spin); // Calculate full excited determinant - auto ex_det = wfn_traits::template from_spin(ex_det_spin, state_other); + auto ex_det = + wfn_traits::template from_spin(ex_det_spin, state_other); #endif // Update sign of matrix element @@ -148,7 +150,8 @@ void append_os_doubles_asci_contributions( const std::vector& vir_alpha, const std::vector& vir_beta, const double* eps_alpha, const double* eps_beta, const double* V, size_t LDV, double h_el_tol, - double root_diag, double E0, const HamiltonianGeneratorBase& ham_gen, + double root_diag, double E0, + const HamiltonianGeneratorBase& ham_gen, asci_contrib_container& asci_contributions) { using wfn_traits = wavefunction_traits; const size_t LDV2 = LDV * LDV; @@ -166,10 +169,13 @@ void append_os_doubles_asci_contributions( double sign_beta = single_excitation_sign(state_beta, b, j); double sign = sign_alpha * sign_beta; - //auto ex_det = state_full; - //ex_det.flip(a).flip(i).flip(j + N).flip(b + N); - auto ex_det = wfn_traits::template single_excitation_no_check(state_full, a, i); - ex_det = wfn_traits::template single_excitation_no_check(ex_det, b, j); + // auto ex_det = state_full; + // ex_det.flip(a).flip(i).flip(j + N).flip(b + N); + auto ex_det = + wfn_traits::template single_excitation_no_check( + state_full, a, i); + ex_det = wfn_traits::template single_excitation_no_check( + ex_det, b, j); auto h_el = sign * V_aibj; // Evaluate fast diagonal element diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index 9b83768e..e2ad3f55 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -72,7 +72,7 @@ asci_contrib_container> asci_contributions_standard( // Alias state data auto state = *(cdets_begin + i); auto state_alpha = wfn_traits::alpha_string(state); - auto state_beta = wfn_traits::beta_string(state); + auto state_beta = wfn_traits::beta_string(state); auto coeff = C[i]; // Get occupied and virtual indices @@ -150,10 +150,11 @@ asci_contrib_container> asci_contributions_constraint( wavefunction_iterator_t cdets_end, const double E_ASCI, const std::vector& C, size_t norb, const double* T_pq, const double* G_red, const double* V_red, const double* G_pqrs, - const double* V_pqrs, HamiltonianGenerator>& ham_gen, MPI_Comm comm) { + const double* V_pqrs, HamiltonianGenerator>& ham_gen, + MPI_Comm comm) { using clock_type = std::chrono::high_resolution_clock; using duration_type = std::chrono::duration; - using wfn_traits = wavefunction_traits>; + using wfn_traits = wavefunction_traits>; using spin_wfn_type = spin_wfn_t>; using spin_wfn_traits = wavefunction_traits; @@ -300,9 +301,9 @@ asci_contrib_container> asci_contributions_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_singles_contributions_ss( - coeff, det|beta, con, occ_alpha, occ_beta, - orb_ens_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, - h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); + coeff, det | beta, con, occ_alpha, occ_beta, orb_ens_alpha.data(), + T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, + ham_gen, asci_pairs); } // AAAA excitations @@ -313,9 +314,8 @@ asci_contrib_container> asci_contributions_constraint( const auto& occ_beta = bcd.occ_beta; const auto& orb_ens_alpha = bcd.orb_ens_alpha; generate_constraint_doubles_contributions_ss( - coeff, det|beta, con, occ_alpha, occ_beta, - orb_ens_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, - ham_gen, asci_pairs); + coeff, det | beta, con, occ_alpha, occ_beta, orb_ens_alpha.data(), + G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } // AABB excitations @@ -328,7 +328,7 @@ asci_contrib_container> asci_contributions_constraint( const auto& orb_ens_alpha = bcd.orb_ens_alpha; const auto& orb_ens_beta = bcd.orb_ens_beta; generate_constraint_doubles_contributions_os( - coeff, det|beta, con, occ_alpha, occ_beta, vir_beta, + coeff, det | beta, con, occ_alpha, occ_beta, vir_beta, orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); } @@ -346,7 +346,7 @@ asci_contrib_container> asci_contributions_constraint( const auto state = det | beta; const auto state_alpha = wfn_traits::alpha_string(state); - const auto state_beta = wfn_traits::beta_string(beta); + const auto state_beta = wfn_traits::beta_string(beta); // BB Excitations append_singles_asci_contributions( coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, @@ -355,9 +355,9 @@ asci_contrib_container> asci_contributions_constraint( // BBBB Excitations append_ss_doubles_asci_contributions( - coeff, state, state_beta, state_alpha, occ_beta, vir_beta, occ_alpha, - eps_beta.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, - asci_pairs); + coeff, state, state_beta, state_alpha, occ_beta, vir_beta, + occ_alpha, eps_beta.data(), G_pqrs, norb, h_el_tol, h_diag, + E_ASCI, ham_gen, asci_pairs); } // Beta Loop } // Triplet Check diff --git a/include/macis/asci/iteration.hpp b/include/macis/asci/iteration.hpp index dd913c43..742fe321 100644 --- a/include/macis/asci/iteration.hpp +++ b/include/macis/asci/iteration.hpp @@ -8,8 +8,8 @@ #pragma once #include -#include #include +#include namespace macis { diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index 07cf196f..899d14f7 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -7,16 +7,14 @@ */ #pragma once +#include #include #include #include #include -#include - namespace macis { - template bool satisfies_constraint(WfnType det, ConType C) { return C.satisfies_constraint(det); @@ -25,16 +23,17 @@ bool satisfies_constraint(WfnType det, ConType C) { template auto generate_constraint_single_excitations(WfnType det, ConType constraint) { using constraint_traits = typename ConType::constraint_traits; - const auto C = constraint.C(); const auto B = constraint.B(); + const auto C = constraint.C(); + const auto B = constraint.B(); // need to have at most one different from the constraint - if(constraint.overlap(det) < (constraint.count()-1)) + if(constraint.overlap(det) < (constraint.count() - 1)) return std::make_pair(WfnType(0), WfnType(0)); auto o = constraint.symmetric_difference(det); auto v = constraint.b_mask_union(~det); - if(constraint_traits::count(o & C) == 1) { + if(constraint_traits::count(o & C) == 1) { v = o & C; o ^= v; } @@ -52,7 +51,8 @@ template auto generate_constraint_double_excitations(WfnType det, ConType constraint) { using constraint_traits = typename ConType::constraint_traits; using constraint_type = typename ConType::constraint_type; - const auto C = constraint.C(); const auto B = constraint.B(); + const auto C = constraint.C(); + const auto B = constraint.B(); // Occ/Vir pairs to generate excitations std::vector O, V; @@ -69,18 +69,17 @@ auto generate_constraint_double_excitations(WfnType det, ConType constraint) { if(o_and_c_count == 2) { v = o_and_c; o ^= v; - // Regenerate since o changed + // Regenerate since o changed // XXX: This apparently is not needed, but leaving because o_and_c = o & C; o_and_c_count = constraint_traits::count(o_and_c); } - const auto virt_ind = bits_to_indices(v); switch(o_and_c_count) { case 1: for(auto a : virt_ind) { - V.emplace_back(constraint_traits::create_no_check(o_and_c,a)); + V.emplace_back(constraint_traits::create_no_check(o_and_c, a)); } o ^= o_and_c; break; @@ -97,7 +96,7 @@ auto generate_constraint_double_excitations(WfnType det, ConType constraint) { switch(o_and_not_b_count) { case 1: for(auto i : bits_to_indices(o & B)) { - O.emplace_back(constraint_traits::create_no_check(o_and_not_b,i)); + O.emplace_back(constraint_traits::create_no_check(o_and_not_b, i)); } break; default: @@ -110,7 +109,7 @@ auto generate_constraint_double_excitations(WfnType det, ConType constraint) { } template -void generate_constraint_singles(WfnType det, ConType constraint, +void generate_constraint_singles(WfnType det, ConType constraint, std::vector& t_singles) { using constraint_traits = typename ConType::constraint_traits; auto [o, v] = generate_constraint_single_excitations(det, constraint); @@ -124,7 +123,7 @@ void generate_constraint_singles(WfnType det, ConType constraint, const auto vir = constraint_traits::state_to_occ(v); for(auto i : occ) { auto temp = constraint_traits::create_no_check(det, i); - for(auto a : vir) + for(auto a : vir) t_singles.emplace_back(constraint_traits::create_no_check(temp, a)); } } @@ -132,15 +131,14 @@ void generate_constraint_singles(WfnType det, ConType constraint, template unsigned count_constraint_singles(WfnType det, ConType constraint) { using constraint_traits = typename ConType::constraint_traits; - auto [o, v] = - generate_constraint_single_excitations(det, constraint); + auto [o, v] = generate_constraint_single_excitations(det, constraint); const auto oc = constraint_traits::count(o); const auto vc = constraint_traits::count(v); return oc * vc; } -template -void generate_constraint_doubles(WfnType det, ConType constraint, +template +void generate_constraint_doubles(WfnType det, ConType constraint, std::vector& t_doubles) { auto [O, V] = generate_constraint_double_excitations(det, constraint); @@ -161,7 +159,8 @@ void generate_constraint_doubles(WfnType det, ConType constraint, template unsigned count_constraint_doubles(WfnType det, ConType constraint) { using constraint_traits = typename ConType::constraint_traits; - const auto C = constraint.C(); const auto B = constraint.B(); + const auto C = constraint.C(); + const auto B = constraint.B(); if(constraint.overlap(det) == 0) return 0; auto o = constraint.symmetric_difference(det); @@ -175,7 +174,7 @@ unsigned count_constraint_doubles(WfnType det, ConType constraint) { if(o_and_c_count == 2) { v = o_and_c; o ^= v; - // Regenerate since o changed + // Regenerate since o changed // XXX: This apparently is not needed, but leaving because o_and_c = o & C; o_and_c_count = constraint_traits::count(o_and_c); @@ -213,7 +212,7 @@ unsigned count_constraint_doubles(WfnType det, ConType constraint) { template size_t constraint_histogram(WfnType det, size_t n_os_singles, - size_t n_os_doubles, ConType constraint){ + size_t n_os_doubles, ConType constraint) { auto ns = count_constraint_singles(det, constraint); auto nd = count_constraint_doubles(det, constraint); @@ -239,7 +238,8 @@ void generate_constraint_singles_contributions_ss( asci_contrib_container& asci_contributions) { using wfn_traits = wavefunction_traits; using constraint_traits = typename ConType::constraint_traits; - auto [o, v] = generate_constraint_single_excitations(wfn_traits::alpha_string(det), constraint); + auto [o, v] = generate_constraint_single_excitations( + wfn_traits::alpha_string(det), constraint); const auto no = constraint_traits::count(o); const auto nv = constraint_traits::count(v); if(!no or !nv) return; @@ -248,11 +248,11 @@ void generate_constraint_singles_contributions_ss( const size_t LDV2 = LDV * LDV; for(int ii = 0; ii < no; ++ii) { const auto i = fls(o); - o = constraint_traits::create_no_check(o, i); // o.flip(i) + o = constraint_traits::create_no_check(o, i); // o.flip(i) auto v_cpy = v; for(int aa = 0; aa < nv; ++aa) { const auto a = fls(v_cpy); - v_cpy = constraint_traits::create_no_check(v_cpy, a); // v_cpy.flip(a) + v_cpy = constraint_traits::create_no_check(v_cpy, a); // v_cpy.flip(a) double h_el = T_pq[a + i * LDT]; const double* G_ov = G_kpq + a * LDG + i * LDG2; @@ -264,8 +264,9 @@ void generate_constraint_singles_contributions_ss( if(std::abs(coeff * h_el) < h_el_tol) continue; // Calculate Excited Determinant - auto ex_det = wfn_traits::template single_excitation_no_check(det, i, a ); - + auto ex_det = + wfn_traits::template single_excitation_no_check(det, i, + a); // Compute Sign in a Canonical Way auto sign = single_excitation_sign(det, a, i); @@ -290,7 +291,8 @@ void generate_constraint_doubles_contributions_ss( asci_contrib_container& asci_contributions) { using wfn_traits = wavefunction_traits; using spin_wfn_traits = wavefunction_traits>; - auto [O, V] = generate_constraint_double_excitations(wfn_traits::alpha_string(det), constraint); + auto [O, V] = generate_constraint_double_excitations( + wfn_traits::alpha_string(det), constraint); const auto no_pairs = O.size(); const auto nv_pairs = V.size(); if(!no_pairs or !nv_pairs) return; @@ -301,7 +303,9 @@ void generate_constraint_doubles_contributions_ss( const auto i = ffs(ij) - 1; const auto j = fls(ij); const auto G_ij = G + (j + i * LDG2) * LDG; - const auto ex_ij = wfn_traits::template single_excitation_no_check(det,i,j); // det ^ ij; + const auto ex_ij = + wfn_traits::template single_excitation_no_check( + det, i, j); // det ^ ij; for(int _ab = 0; _ab < nv_pairs; ++_ab) { const auto ab = V[_ab]; const auto a = ffs(ab) - 1; @@ -313,14 +317,20 @@ void generate_constraint_doubles_contributions_ss( if(std::abs(coeff * G_aibj) < h_el_tol) continue; // Calculate Excited Determinant (spin) - const auto full_ex_spin = spin_wfn_traits::template single_excitation_no_check(ij,a,b); // ij | ab; - const auto ex_det_spin = wfn_traits::template single_excitation_no_check(ex_ij,a,b); // ex_ij | ab; + const auto full_ex_spin = + spin_wfn_traits::template single_excitation_no_check( + ij, a, b); // ij | ab; + const auto ex_det_spin = + wfn_traits::template single_excitation_no_check( + ex_ij, a, b); // ex_ij | ab; // Compute Sign in a Canonical Way - auto sign = doubles_sign(wfn_traits::alpha_string(det), wfn_traits::alpha_string(ex_det_spin), full_ex_spin); + auto sign = + doubles_sign(wfn_traits::alpha_string(det), + wfn_traits::alpha_string(ex_det_spin), full_ex_spin); // Calculate Full Excited Determinant - const auto full_ex = ex_det_spin;// | os_det; + const auto full_ex = ex_det_spin; // | os_det; // Update Sign of Matrix Element auto h_el = sign * G_aibj; @@ -347,7 +357,8 @@ void generate_constraint_doubles_contributions_os( using wfn_traits = wavefunction_traits; using constraint_traits = typename ConType::constraint_traits; // Generate Single Excitations that Satisfy the Constraint - auto [o, v] = generate_constraint_single_excitations(wfn_traits::alpha_string(det), constraint); + auto [o, v] = generate_constraint_single_excitations( + wfn_traits::alpha_string(det), constraint); const auto no = constraint_traits::count(o); const auto nv = constraint_traits::count(v); if(!no or !nv) return; @@ -355,11 +366,11 @@ void generate_constraint_doubles_contributions_os( const size_t LDV2 = LDV * LDV; for(int ii = 0; ii < no; ++ii) { const auto i = fls(o); - o = constraint_traits::create_no_check(o, i); // o.flip(i) + o = constraint_traits::create_no_check(o, i); // o.flip(i) auto v_cpy = v; for(int aa = 0; aa < nv; ++aa) { const auto a = fls(v_cpy); - v_cpy = constraint_traits::create_no_check(v_cpy, a); // v_cpy.flip(a) + v_cpy = constraint_traits::create_no_check(v_cpy, a); // v_cpy.flip(a) const auto* V_ai = V + a + i * LDV; double sign_same = single_excitation_sign(det, a, i); @@ -379,10 +390,13 @@ void generate_constraint_doubles_contributions_os( double sign = sign_same * sign_othr; // Compute Excited Determinant - //auto ex_det = det | os_det; - //ex_det.flip(i).flip(a).flip(j + N / 2).flip(b + N / 2); - auto ex_det = wfn_traits::template single_excitation_no_check(det,i,a); - ex_det = wfn_traits::template single_excitation_no_check(ex_det,j,b); + // auto ex_det = det | os_det; + // ex_det.flip(i).flip(a).flip(j + N / 2).flip(b + N / 2); + auto ex_det = + wfn_traits::template single_excitation_no_check( + det, i, a); + ex_det = wfn_traits::template single_excitation_no_check( + ex_det, j, b); // Finalize Matrix Element auto h_el = sign * V_aibj; @@ -478,13 +492,12 @@ auto dist_triplets_histogram(size_t norb, size_t ns_othr, size_t nd_othr, } #endif - template auto make_triplet(unsigned i, unsigned j, unsigned k) { using wfn_type = wfn_t; using wfn_traits = wavefunction_traits; using constraint_type = alpha_constraint; - using string_type = typename constraint_type::constraint_type; + using string_type = typename constraint_type::constraint_type; string_type C = 0; C.flip(i).flip(j).flip(k); @@ -492,7 +505,7 @@ auto make_triplet(unsigned i, unsigned j, unsigned k) { B <<= k; B = B.to_ullong() - 1; - return constraint_type(C,B,k); + return constraint_type(C, B, k); } #ifdef MACIS_ENABLE_MPI @@ -504,11 +517,11 @@ auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, using wfn_type = wfn_t; using wfn_traits = wavefunction_traits; using constraint_type = alpha_constraint; - using string_type = typename constraint_type::constraint_type; + using string_type = typename constraint_type::constraint_type; auto world_rank = comm_rank(comm); auto world_size = comm_size(comm); - //wfn_t O = full_mask(norb); + // wfn_t O = full_mask(norb); // Global workloads std::vector workloads(world_size, 0); @@ -524,7 +537,8 @@ auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, size_t nw = 0; for(const auto& alpha : unique_alpha) { - nw += constraint_histogram(wfn_traits::alpha_string(alpha), ns_othr, nd_othr, constraint); + nw += constraint_histogram(wfn_traits::alpha_string(alpha), ns_othr, + nd_othr, constraint); } if(nw) constraint_sizes.emplace_back(constraint, nw); total_work += nw; @@ -563,7 +577,8 @@ auto dist_constraint_general(size_t nlevels, size_t norb, size_t ns_othr, size_t nw = 0; for(const auto& alpha : unique_alpha) { - nw += constraint_histogram(wfn_traits::alpha_string(alpha), ns_othr, nd_othr, c_next); + nw += constraint_histogram(wfn_traits::alpha_string(alpha), ns_othr, + nd_othr, c_next); } if(nw) constraint_sizes.emplace_back(c_next, nw); total_work += nw; diff --git a/include/macis/asci/pt2.hpp b/include/macis/asci/pt2.hpp index d7cf7c46..3cea33a8 100644 --- a/include/macis/asci/pt2.hpp +++ b/include/macis/asci/pt2.hpp @@ -12,23 +12,23 @@ namespace macis { - template -double asci_pt2_constraint( - wavefunction_iterator_t cdets_begin, wavefunction_iterator_t cdets_end, - const double E_ASCI, const std::vector& C, size_t norb, - const double* T_pq, const double* G_red, const double* V_red, - const double* G_pqrs, const double* V_pqrs, HamiltonianGenerator>& ham_gen, - MPI_Comm comm) { - +double asci_pt2_constraint(wavefunction_iterator_t cdets_begin, + wavefunction_iterator_t cdets_end, + const double E_ASCI, const std::vector& C, + size_t norb, const double* T_pq, const double* G_red, + const double* V_red, const double* G_pqrs, + const double* V_pqrs, + HamiltonianGenerator>& ham_gen, + MPI_Comm comm) { using clock_type = std::chrono::high_resolution_clock; using duration_type = std::chrono::duration; using wfn_traits = wavefunction_traits>; auto logger = spdlog::get("asci_search"); const size_t ncdets = std::distance(cdets_begin, cdets_end); - //std::cout << "NDETS PT = " << ncdets << " " << C.size() << std::endl; - //std::cout << "PT E0 = " << E_ASCI << std::endl; + // std::cout << "NDETS PT = " << ncdets << " " << C.size() << std::endl; + // std::cout << "PT E0 = " << E_ASCI << std::endl; std::vector occ_alpha, vir_alpha; std::vector occ_beta, vir_beta; @@ -106,9 +106,8 @@ double asci_pt2_constraint( logger->info(" * NS = {} ND = {}", n_sing_alpha, n_doub_alpha); auto gen_c_st = clock_type::now(); - auto constraints = - dist_constraint_general(0, norb, - n_sing_alpha, n_doub_alpha, uniq_alpha_wfn, comm); + auto constraints = dist_constraint_general( + 0, norb, n_sing_alpha, n_doub_alpha, uniq_alpha_wfn, comm); auto gen_c_en = clock_type::now(); duration_type gen_c_dur = gen_c_en - gen_c_st; logger->info(" * GEN_DUR = {:.2e} ms", gen_c_dur.count()); @@ -120,114 +119,116 @@ double asci_pt2_constraint( )); double EPT2 = 0.0; - // Process ASCI pair contributions for each constraint - #pragma omp parallel +// Process ASCI pair contributions for each constraint +#pragma omp parallel { - asci_contrib_container> asci_pairs; - asci_pairs.reserve(max_size); - #pragma omp for reduction(+:EPT2) - for(size_t ic = 0; ic < constraints.size(); ++ic) { - const auto& con = constraints[ic]; - //std::cout << std::distance(&constraints[0], &con) << "/" << constraints.size() << std::endl; - const double h_el_tol = 1e-16; - - // Loop over unique alpha strings - for(size_t i_alpha = 0; i_alpha < nuniq_alpha; ++i_alpha) { - const auto& det = uniq_alpha_wfn[i_alpha]; - const auto occ_alpha = bits_to_indices(det); - - // AA excitations - for(const auto& bcd : uad[i_alpha].bcd) { - const auto& beta = bcd.beta_string; - const auto& coeff = bcd.coeff; - const auto& h_diag = bcd.h_diag; - const auto& occ_beta = bcd.occ_beta; - const auto& orb_ens_alpha = bcd.orb_ens_alpha; - generate_constraint_singles_contributions_ss( - coeff, det|beta, con, occ_alpha, occ_beta, - orb_ens_alpha.data(), T_pq, norb, G_red, norb, V_red, norb, - h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); - } - - // AAAA excitations - for(const auto& bcd : uad[i_alpha].bcd) { - const auto& beta = bcd.beta_string; - const auto& coeff = bcd.coeff; - const auto& h_diag = bcd.h_diag; - const auto& occ_beta = bcd.occ_beta; - const auto& orb_ens_alpha = bcd.orb_ens_alpha; - generate_constraint_doubles_contributions_ss( - coeff, det|beta, con, occ_alpha, occ_beta, - orb_ens_alpha.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, - ham_gen, asci_pairs); - } - - // AABB excitations - for(const auto& bcd : uad[i_alpha].bcd) { - const auto& beta = bcd.beta_string; - const auto& coeff = bcd.coeff; - const auto& h_diag = bcd.h_diag; - const auto& occ_beta = bcd.occ_beta; - const auto& vir_beta = bcd.vir_beta; - const auto& orb_ens_alpha = bcd.orb_ens_alpha; - const auto& orb_ens_beta = bcd.orb_ens_beta; - generate_constraint_doubles_contributions_os( - coeff, det|beta, con, occ_alpha, occ_beta, vir_beta, - orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, - h_diag, E_ASCI, ham_gen, asci_pairs); - } + asci_contrib_container> asci_pairs; + asci_pairs.reserve(max_size); +#pragma omp for reduction(+ : EPT2) + for(size_t ic = 0; ic < constraints.size(); ++ic) { + const auto& con = constraints[ic]; + // std::cout << std::distance(&constraints[0], &con) << "/" << + // constraints.size() << std::endl; + const double h_el_tol = 1e-16; + + // Loop over unique alpha strings + for(size_t i_alpha = 0; i_alpha < nuniq_alpha; ++i_alpha) { + const auto& det = uniq_alpha_wfn[i_alpha]; + const auto occ_alpha = bits_to_indices(det); + + // AA excitations + for(const auto& bcd : uad[i_alpha].bcd) { + const auto& beta = bcd.beta_string; + const auto& coeff = bcd.coeff; + const auto& h_diag = bcd.h_diag; + const auto& occ_beta = bcd.occ_beta; + const auto& orb_ens_alpha = bcd.orb_ens_alpha; + generate_constraint_singles_contributions_ss( + coeff, det | beta, con, occ_alpha, occ_beta, orb_ens_alpha.data(), + T_pq, norb, G_red, norb, V_red, norb, h_el_tol, h_diag, E_ASCI, + ham_gen, asci_pairs); + } + + // AAAA excitations + for(const auto& bcd : uad[i_alpha].bcd) { + const auto& beta = bcd.beta_string; + const auto& coeff = bcd.coeff; + const auto& h_diag = bcd.h_diag; + const auto& occ_beta = bcd.occ_beta; + const auto& orb_ens_alpha = bcd.orb_ens_alpha; + generate_constraint_doubles_contributions_ss( + coeff, det | beta, con, occ_alpha, occ_beta, orb_ens_alpha.data(), + G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); + } - // If the alpha determinant satisfies the constraint, - // append BB and BBBB excitations - if(satisfies_constraint(wfn_traits::alpha_string(det), con)) { + // AABB excitations for(const auto& bcd : uad[i_alpha].bcd) { const auto& beta = bcd.beta_string; const auto& coeff = bcd.coeff; const auto& h_diag = bcd.h_diag; const auto& occ_beta = bcd.occ_beta; const auto& vir_beta = bcd.vir_beta; - const auto& eps_beta = bcd.orb_ens_beta; - - const auto state = det | beta; - const auto state_alpha = wfn_traits::alpha_string(state); - const auto state_beta = wfn_traits::beta_string(beta); - // BB Excitations - append_singles_asci_contributions( - coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, - eps_beta.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, + const auto& orb_ens_alpha = bcd.orb_ens_alpha; + const auto& orb_ens_beta = bcd.orb_ens_beta; + generate_constraint_doubles_contributions_os( + coeff, det | beta, con, occ_alpha, occ_beta, vir_beta, + orb_ens_alpha.data(), orb_ens_beta.data(), V_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, asci_pairs); + } + + // If the alpha determinant satisfies the constraint, + // append BB and BBBB excitations + if(satisfies_constraint(wfn_traits::alpha_string(det), con)) { + for(const auto& bcd : uad[i_alpha].bcd) { + const auto& beta = bcd.beta_string; + const auto& coeff = bcd.coeff; + const auto& h_diag = bcd.h_diag; + const auto& occ_beta = bcd.occ_beta; + const auto& vir_beta = bcd.vir_beta; + const auto& eps_beta = bcd.orb_ens_beta; + + const auto state = det | beta; + const auto state_alpha = wfn_traits::alpha_string(state); + const auto state_beta = wfn_traits::beta_string(beta); + // BB Excitations + append_singles_asci_contributions( + coeff, state, state_beta, occ_beta, vir_beta, occ_alpha, + eps_beta.data(), T_pq, norb, G_red, norb, V_red, norb, h_el_tol, + h_diag, E_ASCI, ham_gen, asci_pairs); + + // BBBB Excitations + append_ss_doubles_asci_contributions( + coeff, state, state_beta, state_alpha, occ_beta, vir_beta, + occ_alpha, eps_beta.data(), G_pqrs, norb, h_el_tol, h_diag, + E_ASCI, ham_gen, asci_pairs); + + // No excition - to remove for PT2 + asci_pairs.push_back( + {state, std::numeric_limits::infinity(), 1.0}); + } // Beta Loop + } // Triplet Check + + } // Unique Alpha Loop + + double EPT2_local = 0.0; + // Local S&A for each quad + update EPT2 + { + auto uit = sort_and_accumulate_asci_pairs(asci_pairs.begin(), + asci_pairs.end()); + for(auto it = asci_pairs.begin(); it != uit; ++it) { + // if(std::find(cdets_begin, cdets_end, it->state) == cdets_end) + if(!std::isinf(it->c_times_matel)) + EPT2_local += (it->c_times_matel * it->c_times_matel) / it->h_diag; + } + asci_pairs.clear(); + } - // BBBB Excitations - append_ss_doubles_asci_contributions( - coeff, state, state_beta, state_alpha, occ_beta, vir_beta, occ_alpha, - eps_beta.data(), G_pqrs, norb, h_el_tol, h_diag, E_ASCI, ham_gen, - asci_pairs); - - // No excition - to remove for PT2 - asci_pairs.push_back({state, std::numeric_limits::infinity(), 1.0}); - } // Beta Loop - } // Triplet Check - - } // Unique Alpha Loop - - double EPT2_local = 0.0; - // Local S&A for each quad + update EPT2 - { - auto uit = sort_and_accumulate_asci_pairs(asci_pairs.begin(), asci_pairs.end()); - for(auto it = asci_pairs.begin(); it != uit; ++it) { - //if(std::find(cdets_begin, cdets_end, it->state) == cdets_end) - if(!std::isinf(it->c_times_matel)) - EPT2_local += (it->c_times_matel * it->c_times_matel) / it->h_diag; - } - asci_pairs.clear(); - } - - EPT2 += EPT2_local; - } // Constraint Loop + EPT2 += EPT2_local; + } // Constraint Loop } EPT2 = allreduce(EPT2, MPI_SUM, comm); return EPT2; } -} +} // namespace macis diff --git a/include/macis/csr_hamiltonian.hpp b/include/macis/csr_hamiltonian.hpp index 903ed1ac..cea646cd 100644 --- a/include/macis/csr_hamiltonian.hpp +++ b/include/macis/csr_hamiltonian.hpp @@ -21,9 +21,9 @@ namespace macis { // Base implementation of CSR hamiltonian generation template sparsexx::csr_matrix make_csr_hamiltonian_block( - WfnIterator bra_begin, WfnIterator bra_end, - WfnIterator ket_begin, WfnIterator ket_end, - HamiltonianGenerator& ham_gen, double H_thresh) { + WfnIterator bra_begin, WfnIterator bra_end, WfnIterator ket_begin, + WfnIterator ket_end, HamiltonianGenerator& ham_gen, + double H_thresh) { size_t nbra = std::distance(bra_begin, bra_end); size_t nket = std::distance(ket_begin, ket_end); @@ -47,7 +47,8 @@ sparsexx::csr_matrix make_csr_hamiltonian( // Base implementation of dist-CSR H construction for bitsets template sparsexx::dist_sparse_matrix> -make_dist_csr_hamiltonian(MPI_Comm comm, WfnIterator sd_begin, WfnIterator sd_end, +make_dist_csr_hamiltonian(MPI_Comm comm, WfnIterator sd_begin, + WfnIterator sd_end, HamiltonianGenerator& ham_gen, const double H_thresh) { using namespace sparsexx; diff --git a/include/macis/hamiltonian_generator.hpp b/include/macis/hamiltonian_generator.hpp index f34b2fb8..4c828ded 100644 --- a/include/macis/hamiltonian_generator.hpp +++ b/include/macis/hamiltonian_generator.hpp @@ -7,16 +7,14 @@ */ #pragma once -#include #include +#include namespace macis { template class HamiltonianGenerator : public HamiltonianGeneratorBase { - public: - using full_det_t = WfnType; using spin_det_t = spin_wfn_t; @@ -32,9 +30,8 @@ class HamiltonianGenerator : public HamiltonianGeneratorBase { full_det_iterator, double) = 0; public: - - HamiltonianGenerator(matrix_span_t T, rank4_span_t V) : - HamiltonianGeneratorBase(T,V) {}; + HamiltonianGenerator(matrix_span_t T, rank4_span_t V) + : HamiltonianGeneratorBase(T, V){}; virtual ~HamiltonianGenerator() noexcept = default; @@ -101,7 +98,7 @@ class HamiltonianGenerator : public HamiltonianGeneratorBase { virtual void SetJustSingles(bool /*_js*/) {} virtual bool GetJustSingles() { return false; } - //virtual size_t GetNimp() const { return N / 2; } + // virtual size_t GetNimp() const { return N / 2; } }; } // namespace macis diff --git a/include/macis/hamiltonian_generator/base.hpp b/include/macis/hamiltonian_generator/base.hpp index e96cf9e8..64dcb67f 100644 --- a/include/macis/hamiltonian_generator/base.hpp +++ b/include/macis/hamiltonian_generator/base.hpp @@ -14,15 +14,13 @@ namespace macis { template class HamiltonianGeneratorBase { - protected: - template using sparse_matrix_type = sparsexx::csr_matrix; using matrix_span_t = matrix_span; - using rank3_span_t = rank3_span; - using rank4_span_t = rank4_span; + using rank3_span_t = rank3_span; + using rank4_span_t = rank4_span; size_t norb_; size_t norb2_; @@ -53,7 +51,6 @@ class HamiltonianGeneratorBase { void generate_integral_intermediates_(rank4_span_t V); public: - HamiltonianGeneratorBase(matrix_span_t T, rank4_span_t V); virtual ~HamiltonianGeneratorBase() noexcept = default; @@ -67,7 +64,6 @@ class HamiltonianGeneratorBase { generate_integral_intermediates_(V_pqrs_); } - double single_orbital_en(uint32_t orb, const std::vector& ss_occ, const std::vector& os_occ) const; @@ -104,10 +100,7 @@ class HamiltonianGeneratorBase { uint32_t orb_paru, uint32_t orb_pard, double orig_det_Hii) const; - - void rotate_hamiltonian_ordm(const Scalar* ordm); - }; -} +} // namespace macis diff --git a/include/macis/hamiltonian_generator/matrix_elements.hpp b/include/macis/hamiltonian_generator/matrix_elements.hpp index f34637b6..36c80b9d 100644 --- a/include/macis/hamiltonian_generator/matrix_elements.hpp +++ b/include/macis/hamiltonian_generator/matrix_elements.hpp @@ -13,7 +13,7 @@ namespace macis { template double HamiltonianGenerator::matrix_element(full_det_t bra, - full_det_t ket) const { + full_det_t ket) const { using wfn_traits = wavefunction_traits; auto bra_alpha = wfn_traits::alpha_string(bra); auto ket_alpha = wfn_traits::alpha_string(ket); @@ -38,7 +38,7 @@ double HamiltonianGenerator::matrix_element( const std::vector& bra_occ_beta) const { using spin_wfn_traits = wavefunction_traits; const uint32_t ex_alpha_count = spin_wfn_traits::count(ex_alpha); - const uint32_t ex_beta_count = spin_wfn_traits::count(ex_beta); + const uint32_t ex_beta_count = spin_wfn_traits::count(ex_beta); if((ex_alpha_count + ex_beta_count) > 4) return 0.; @@ -65,8 +65,9 @@ double HamiltonianGenerator::matrix_element( } template -double HamiltonianGenerator::matrix_element_4(spin_det_t bra, spin_det_t ket, - spin_det_t ex) const { +double HamiltonianGenerator::matrix_element_4(spin_det_t bra, + spin_det_t ket, + spin_det_t ex) const { auto [o1, v1, o2, v2, sign] = doubles_sign_indices(bra, ket, ex); return sign * G_pqrs_(v1, o1, v2, o2); diff --git a/include/macis/mcscf/cas.hpp b/include/macis/mcscf/cas.hpp index 2ca1962b..82a12ec6 100644 --- a/include/macis/mcscf/cas.hpp +++ b/include/macis/mcscf/cas.hpp @@ -7,9 +7,9 @@ */ #pragma once +#include #include #include -#include namespace macis { @@ -34,7 +34,6 @@ double compute_casci_rdms( MCSCFSettings settings, NumOrbital norb, size_t nalpha, size_t nbeta, double* T, double* V, double* ORDM, double* TRDM, std::vector& C MACIS_MPI_CODE(, MPI_Comm comm)) { - using wfn_type = typename HamGen::full_det_t; #ifdef MACIS_ENABLE_MPI int rank; @@ -50,10 +49,10 @@ double compute_casci_rdms( // Compute Lowest Energy Eigenvalue (ED) auto dets = generate_hilbert_space(norb.get(), nalpha, nbeta); - double E0 = - selected_ci_diag(dets.begin(), dets.end(), ham_gen, settings.ci_matel_tol, - settings.ci_max_subspace, settings.ci_res_tol, C, - MACIS_MPI_CODE(comm, ) true); + double E0 = selected_ci_diag( + dets.begin(), dets.end(), ham_gen, settings.ci_matel_tol, + settings.ci_max_subspace, settings.ci_res_tol, C, + MACIS_MPI_CODE(comm, ) true); // Compute RDMs ham_gen.form_rdms(dets.begin(), dets.end(), dets.begin(), dets.end(), diff --git a/include/macis/mcscf/mcscf_impl.hpp b/include/macis/mcscf/mcscf_impl.hpp index 746c9cce..294cae59 100644 --- a/include/macis/mcscf/mcscf_impl.hpp +++ b/include/macis/mcscf/mcscf_impl.hpp @@ -7,9 +7,6 @@ */ #pragma once -#include -#include - #include #include #include @@ -17,6 +14,8 @@ #include #include #include +#include +#include // #include diff --git a/include/macis/mcscf/orbital_hessian.hpp b/include/macis/mcscf/orbital_hessian.hpp index 88b05935..952ae35a 100644 --- a/include/macis/mcscf/orbital_hessian.hpp +++ b/include/macis/mcscf/orbital_hessian.hpp @@ -7,9 +7,9 @@ */ #pragma once -#include #include #include +#include namespace macis { diff --git a/include/macis/sd_operations.hpp b/include/macis/sd_operations.hpp index bce84a2e..d88b02f0 100644 --- a/include/macis/sd_operations.hpp +++ b/include/macis/sd_operations.hpp @@ -28,14 +28,13 @@ namespace macis { * @returns The bitstring HF state consisting of the specified number of * occupied orbitals. */ -//template -//std::bitset canonical_hf_determinant(uint32_t nalpha, uint32_t nbeta) { -// static_assert((N % 2) == 0, "N Must Be Even"); -// std::bitset alpha = full_mask(nalpha); -// std::bitset beta = full_mask(nbeta) << (N / 2); -// return alpha | beta; -//} - +// template +// std::bitset canonical_hf_determinant(uint32_t nalpha, uint32_t nbeta) { +// static_assert((N % 2) == 0, "N Must Be Even"); +// std::bitset alpha = full_mask(nalpha); +// std::bitset beta = full_mask(nbeta) << (N / 2); +// return alpha | beta; +// } /** * @brief Generate the list of (un)occupied orbitals for a paricular state. @@ -46,52 +45,53 @@ namespace macis { * @param[out] occ List of occupied orbitals in `state` * @param[out] vir List of unoccupied orbitals in `state` */ -//template -//void bitset_to_occ_vir(size_t norb, std::bitset state, -// std::vector& occ, std::vector& vir) { -// occ = bits_to_indices(state); -// const auto nocc = occ.size(); -// assert(nocc < norb); +// template +// void bitset_to_occ_vir(size_t norb, std::bitset state, +// std::vector& occ, std::vector& +// vir) { +// occ = bits_to_indices(state); +// const auto nocc = occ.size(); +// assert(nocc < norb); // -// const auto nvir = norb - nocc; -// vir.resize(nvir); -// state = ~state; -// for(int i = 0; i < nvir; ++i) { -// auto a = ffs(state) - 1; -// vir[i] = a; -// state.flip(a); -// } -//} - - -//template -//auto single_excitation(std::bitset state, unsigned p, unsigned q) { -// return state.flip(p).flip(q); -//} - -//template -//auto single_excitation_spin(std::bitset state, unsigned p, unsigned q) { -// static_assert(N%2 == 0, "Num Bits Must Be Even"); -// if constexpr (Sigma == Spin::Alpha) -// return single_excitation(state,p,q); -// else -// return single_excitation(state,p+N/2,q+N/2); -//} - -//template -//auto double_excitation(std::bitset state, unsigned p, unsigned q, unsigned r, unsigned s) { -// return state.flip(p).flip(q).flip(r).flip(s); -//} - -//template -//auto double_excitation_spin(std::bitset state, unsigned p, unsigned q, unsigned r, unsigned s) { -// static_assert(N%2 == 0, "Num Bits Must Be Even"); -// if constexpr (Sigma == Spin::Alpha) -// return double_excitation(state,p,q,r,s); -// else -// return double_excitation(state,p+N/2,q+N/2,r+N/2,s+N/2); -//} - +// const auto nvir = norb - nocc; +// vir.resize(nvir); +// state = ~state; +// for(int i = 0; i < nvir; ++i) { +// auto a = ffs(state) - 1; +// vir[i] = a; +// state.flip(a); +// } +// } + +// template +// auto single_excitation(std::bitset state, unsigned p, unsigned q) { +// return state.flip(p).flip(q); +// } + +// template +// auto single_excitation_spin(std::bitset state, unsigned p, unsigned q) { +// static_assert(N%2 == 0, "Num Bits Must Be Even"); +// if constexpr (Sigma == Spin::Alpha) +// return single_excitation(state,p,q); +// else +// return single_excitation(state,p+N/2,q+N/2); +// } + +// template +// auto double_excitation(std::bitset state, unsigned p, unsigned q, unsigned +// r, unsigned s) { +// return state.flip(p).flip(q).flip(r).flip(s); +// } + +// template +// auto double_excitation_spin(std::bitset state, unsigned p, unsigned q, +// unsigned r, unsigned s) { +// static_assert(N%2 == 0, "Num Bits Must Be Even"); +// if constexpr (Sigma == Spin::Alpha) +// return double_excitation(state,p,q,r,s); +// else +// return double_excitation(state,p+N/2,q+N/2,r+N/2,s+N/2); +// } // TODO: Test this function template @@ -114,8 +114,7 @@ double single_excitation_sign(std::bitset state, unsigned p, unsigned q) { template void append_singles(WfnType state, const std::vector& occ, - const std::vector& vir, - WfnContainer& singles) { + const std::vector& vir, WfnContainer& singles) { using wfn_traits = wavefunction_traits; const size_t nocc = occ.size(); const size_t nvir = vir.size(); @@ -125,14 +124,14 @@ void append_singles(WfnType state, const std::vector& occ, for(size_t a = 0; a < nvir; ++a) for(size_t i = 0; i < nocc; ++i) { - singles.emplace_back(wfn_traits::single_excitation_no_check(state, occ[i], vir[a])); + singles.emplace_back( + wfn_traits::single_excitation_no_check(state, occ[i], vir[a])); } } template void append_doubles(WfnType state, const std::vector& occ, - const std::vector& vir, - WfnContainer& doubles) { + const std::vector& vir, WfnContainer& doubles) { using wfn_traits = wavefunction_traits; const size_t nocc = occ.size(); const size_t nvir = vir.size(); @@ -146,7 +145,8 @@ void append_doubles(WfnType state, const std::vector& occ, for(size_t i = 0; i < nocc; ++i) for(size_t b = a + 1; b < nvir; ++b) for(size_t j = i + 1; j < nocc; ++j) { - doubles.emplace_back(wfn_traits::double_excitation_no_check(state, occ[i], occ[j], vir[a], vir[b])); + doubles.emplace_back(wfn_traits::double_excitation_no_check( + state, occ[i], occ[j], vir[a], vir[b])); } } @@ -171,8 +171,8 @@ void generate_doubles(size_t norb, WfnType state, WfnContainer& doubles) { } template -void generate_singles_doubles(size_t norb, WfnType state, - WfnContainer& singles, WfnContainer& doubles) { +void generate_singles_doubles(size_t norb, WfnType state, WfnContainer& singles, + WfnContainer& doubles) { using wfn_traits = wavefunction_traits; std::vector occ_orbs, vir_orbs; wfn_traits::state_to_occ_vir(norb, state, occ_orbs, vir_orbs); @@ -183,14 +183,12 @@ void generate_singles_doubles(size_t norb, WfnType state, append_doubles(state, occ_orbs, vir_orbs, doubles); } - template void generate_singles_spin(size_t norb, WfnType state, WfnContainer& singles) { - using wfn_traits = wavefunction_traits; auto state_alpha = wfn_traits::alpha_string(state); - auto state_beta = wfn_traits::beta_string (state); + auto state_beta = wfn_traits::beta_string(state); using spin_wfn_type = spin_wfn_t; std::vector singles_alpha, singles_beta; @@ -215,12 +213,12 @@ void generate_singles_spin(size_t norb, WfnType state, WfnContainer& singles) { template void generate_singles_doubles_spin(size_t norb, WfnType state, - WfnContainer& singles, WfnContainer& doubles) { - + WfnContainer& singles, + WfnContainer& doubles) { using wfn_traits = wavefunction_traits; auto state_alpha = wfn_traits::alpha_string(state); - auto state_beta = wfn_traits::beta_string (state); + auto state_beta = wfn_traits::beta_string(state); using spin_wfn_type = spin_wfn_t; std::vector singles_alpha, singles_beta; @@ -230,7 +228,6 @@ void generate_singles_doubles_spin(size_t norb, WfnType state, generate_singles_doubles(norb, state_alpha, singles_alpha, doubles_alpha); generate_singles_doubles(norb, state_beta, singles_beta, doubles_beta); - // Generate Singles in full space singles.clear(); @@ -265,7 +262,8 @@ void generate_singles_doubles_spin(size_t norb, WfnType state, } template -void generate_cisd_hilbert_space(size_t norb, WfnType state, WfnContainer& dets) { +void generate_cisd_hilbert_space(size_t norb, WfnType state, + WfnContainer& dets) { dets.clear(); dets.emplace_back(state); std::vector singles, doubles; @@ -340,7 +338,8 @@ std::vector generate_cis_hilbert_space(size_t norb, WfnType state) { // TODO: Test this function template -inline auto single_excitation_sign_indices(WfnType bra, WfnType ket, WfnType ex) { +inline auto single_excitation_sign_indices(WfnType bra, WfnType ket, + WfnType ex) { auto o1 = first_occupied_flipped(ket, ex); auto v1 = first_occupied_flipped(bra, ex); auto sign = single_excitation_sign(ket, v1, o1); @@ -355,7 +354,7 @@ inline auto doubles_sign_indices(WfnType bra, WfnType ket, WfnType ex) { auto [o1, v1, sign1] = single_excitation_sign_indices(bra, ket, ex); ket = wfn_traits::single_excitation_no_check(ket, o1, v1); - ex = wfn_traits::single_excitation_no_check(ex, o1, v1); + ex = wfn_traits::single_excitation_no_check(ex, o1, v1); auto [o2, v2, sign2] = single_excitation_sign_indices(bra, ket, ex); auto sign = sign1 * sign2; @@ -370,7 +369,6 @@ inline auto doubles_sign(WfnType bra, WfnType ket, WfnType ex) { return sign; } - template std::string to_canonical_string(WfnType state) { using wfn_traits = wavefunction_traits; @@ -378,7 +376,7 @@ std::string to_canonical_string(WfnType state) { using spin_wfn_traits = wavefunction_traits; auto state_alpha = wfn_traits::alpha_string(state); - auto state_beta = wfn_traits::beta_string (state); + auto state_beta = wfn_traits::beta_string(state); std::string str; for(size_t i = 0; i < spin_wfn_traits::size(); ++i) { @@ -397,13 +395,13 @@ std::string to_canonical_string(WfnType state) { template WfnType from_canonical_string(std::string str) { using spin_wfn_type = spin_wfn_t; - using wfn_traits = wavefunction_traits; - using spin_wfn_traits = wavefunction_traits; + using wfn_traits = wavefunction_traits; + using spin_wfn_traits = wavefunction_traits; spin_wfn_type state_alpha(0), state_beta(0); - for(auto i = 0ul; i < std::min(str.length(),spin_wfn_traits::size()); ++i) { + for(auto i = 0ul; i < std::min(str.length(), spin_wfn_traits::size()); ++i) { if(str[i] == '2') { state_alpha = spin_wfn_traits::create_no_check(state_alpha, i); - state_beta = spin_wfn_traits::create_no_check(state_beta , i); + state_beta = spin_wfn_traits::create_no_check(state_beta, i); } else if(str[i] == 'u') { state_alpha = spin_wfn_traits::create_no_check(state_alpha, i); } else if(str[i] == 'd') { diff --git a/include/macis/util/rdms.hpp b/include/macis/util/rdms.hpp index e10a7cc7..875cd968 100644 --- a/include/macis/util/rdms.hpp +++ b/include/macis/util/rdms.hpp @@ -105,7 +105,7 @@ inline void rdm_contributions(wfn_t bra_alpha, wfn_t ket_alpha, matrix_span ordm, rank4_span trdm) { using wfn_traits = wavefunction_traits>; const uint32_t ex_alpha_count = wfn_traits::count(ex_alpha); - const uint32_t ex_beta_count = wfn_traits::count(ex_beta); + const uint32_t ex_beta_count = wfn_traits::count(ex_beta); if((ex_alpha_count + ex_beta_count) > 4) return; diff --git a/include/macis/util/unused_untested.hpp b/include/macis/util/unused_untested.hpp index f348e00a..af7b6639 100644 --- a/include/macis/util/unused_untested.hpp +++ b/include/macis/util/unused_untested.hpp @@ -6,7 +6,6 @@ * See LICENSE.txt for details */ - #if 0 /** * @brief Generate canonical HF determinant. diff --git a/include/macis/wfn/raw_bitset.hpp b/include/macis/wfn/raw_bitset.hpp index 34a7dea7..3bd5f4e0 100644 --- a/include/macis/wfn/raw_bitset.hpp +++ b/include/macis/wfn/raw_bitset.hpp @@ -13,10 +13,7 @@ namespace macis { -enum class Spin { - Alpha, - Beta -}; +enum class Spin { Alpha, Beta }; template struct wavefunction_traits; @@ -26,10 +23,9 @@ using spin_wfn_t = typename wavefunction_traits::spin_wfn_type; template struct wavefunction_traits> { - - using wfn_type = std::bitset; - using spin_wfn_type = std::bitset; - using orbidx_type = uint32_t; + using wfn_type = std::bitset; + using spin_wfn_type = std::bitset; + using orbidx_type = uint32_t; using orbidx_container = std::vector; inline static constexpr size_t bit_size = N; @@ -48,46 +44,43 @@ struct wavefunction_traits> { using wfn_comparator = bitset_less_comparator; - struct spin_comparator { - using spin_wfn_comparator = bitset_less_comparator; + using spin_wfn_comparator = bitset_less_comparator; bool operator()(wfn_type x, wfn_type y) const { auto s_comp = spin_wfn_comparator{}; const auto x_a = alpha_string(x); const auto y_a = alpha_string(y); - if( x_a == y_a ) { + if(x_a == y_a) { const auto x_b = beta_string(x); const auto y_b = beta_string(y); return s_comp(x_b, y_b); - } else return s_comp(x_a, y_a); + } else + return s_comp(x_a, y_a); } }; - - template static inline wfn_type from_spin(spin_wfn_type alpha, spin_wfn_type beta) { - if constexpr (Sigma == Spin::Alpha) { + if constexpr(Sigma == Spin::Alpha) { auto alpha_expand = expand_bitset(alpha); - auto beta_expand = expand_bitset(beta) << N/2; + auto beta_expand = expand_bitset(beta) << N / 2; return alpha_expand | beta_expand; } else { - auto alpha_expand = expand_bitset(alpha) << N/2; - auto beta_expand = expand_bitset(beta); + auto alpha_expand = expand_bitset(alpha) << N / 2; + auto beta_expand = expand_bitset(beta); return alpha_expand | beta_expand; } } - static inline wfn_type canonical_hf_determinant(uint32_t nalpha, uint32_t nbeta) { - - spin_wfn_type alpha = full_mask(nalpha); - spin_wfn_type beta = full_mask(nbeta); + static inline wfn_type canonical_hf_determinant(uint32_t nalpha, + uint32_t nbeta) { + spin_wfn_type alpha = full_mask(nalpha); + spin_wfn_type beta = full_mask(nbeta); return from_spin(alpha, beta); - } template - static inline wfn_type& flip_bits(wfn_type& state, Inds&&... ); + static inline wfn_type& flip_bits(wfn_type& state, Inds&&...); template static inline wfn_type& flip_bits(wfn_type& state) { @@ -95,34 +88,30 @@ struct wavefunction_traits> { } template - static inline wfn_type& flip_bits(wfn_type& state, unsigned p, Inds&&... inds) { - return flip_bits( - state.flip(p + (Sigma == Spin::Alpha ? 0 : N/2)), - std::forward(inds)... - ); + static inline wfn_type& flip_bits(wfn_type& state, unsigned p, + Inds&&... inds) { + return flip_bits(state.flip(p + (Sigma == Spin::Alpha ? 0 : N / 2)), + std::forward(inds)...); } template static inline wfn_type create_no_check(wfn_type state, unsigned p) { - flip_bits(state, p); + flip_bits(state, p); return state; } template - static inline wfn_type single_excitation_no_check(wfn_type state, - unsigned p, + static inline wfn_type single_excitation_no_check(wfn_type state, unsigned p, unsigned q) { - flip_bits(state, p, q); + flip_bits(state, p, q); return state; } template - static inline wfn_type double_excitation_no_check(wfn_type state, - unsigned p, - unsigned q, - unsigned r, + static inline wfn_type double_excitation_no_check(wfn_type state, unsigned p, + unsigned q, unsigned r, unsigned s) { - flip_bits(state, p, q, r, s); + flip_bits(state, p, q, r, s); return state; } @@ -134,13 +123,13 @@ struct wavefunction_traits> { return bits_to_indices(state); } - static inline void state_to_occ_vir(size_t norb, wfn_type state, orbidx_container& occ, - orbidx_container& vir) { - + static inline void state_to_occ_vir(size_t norb, wfn_type state, + orbidx_container& occ, + orbidx_container& vir) { state_to_occ(state, occ); const auto nocc = occ.size(); assert(nocc < norb); - + const auto nvir = norb - nocc; vir.resize(nvir); state = ~state; @@ -150,9 +139,6 @@ struct wavefunction_traits> { state.flip(a); } } - }; - - -} +} // namespace macis diff --git a/src/macis/hamiltonian_generator/base.cxx b/src/macis/hamiltonian_generator/base.cxx index e376fae7..dbfd61ac 100644 --- a/src/macis/hamiltonian_generator/base.cxx +++ b/src/macis/hamiltonian_generator/base.cxx @@ -7,6 +7,7 @@ */ #include "base.ipp" + #include "fast_diagonals.ipp" namespace macis { diff --git a/src/macis/moller_plesset.cxx b/src/macis/moller_plesset.cxx index 902d8b19..49982ed1 100644 --- a/src/macis/moller_plesset.cxx +++ b/src/macis/moller_plesset.cxx @@ -8,8 +8,8 @@ #include #include -#include #include +#include namespace macis { diff --git a/tests/asci.cxx b/tests/asci.cxx index 829b0357..40e8c406 100644 --- a/tests/asci.cxx +++ b/tests/asci.cxx @@ -12,8 +12,8 @@ #include #include #include -#include #include +#include #include #include #include @@ -50,7 +50,7 @@ auto make_quad(unsigned i, unsigned j, unsigned k, unsigned l) { using wfn_type = macis::wfn_t; using wfn_traits = macis::wavefunction_traits; using constraint_type = macis::alpha_constraint; - using string_type = typename constraint_type::constraint_type; + using string_type = typename constraint_type::constraint_type; string_type C = 0; C.flip(i).flip(j).flip(k).flip(l); @@ -58,7 +58,7 @@ auto make_quad(unsigned i, unsigned j, unsigned k, unsigned l) { B <<= l; B = B.to_ullong() - 1; - return constraint_type(C,B,l); + return constraint_type(C, B, l); } TEST_CASE("Triplets") { @@ -177,7 +177,6 @@ TEST_CASE("Triplets") { triplets.emplace_back(i, j, k); } - std::vector new_triplet_hist(triplet_hist.size(), 0); for(auto [i, j, k] : triplets) { const auto label = i * 32 * 32 + j * 32 + k; @@ -224,10 +223,8 @@ TEST_CASE("Triplets") { REQUIRE(quad_hist == new_quad_hist); } - TEST_CASE("Constraints") { - - using wfn_type = macis::wfn_t<64>; + using wfn_type = macis::wfn_t<64>; using wfn_traits = macis::wavefunction_traits; using spin_wfn_type = typename wfn_traits::spin_wfn_type; using spin_wfn_traits = macis::wavefunction_traits; @@ -241,62 +238,65 @@ TEST_CASE("Constraints") { SECTION("Closed Shell") { nalpha = 6; - nbeta = 6; + nbeta = 6; } SECTION("Open Shell") { nalpha = 6; - nbeta = 3; + nbeta = 3; } // Generate Hilbert Space auto dets = macis::generate_hilbert_space(norb, nalpha, nbeta); - std::sort(dets.begin(), dets.end(), wfn_comparator{}); // lex sort + std::sort(dets.begin(), dets.end(), wfn_comparator{}); // lex sort - // Get Alpha Compression Data + // Get Alpha Compression Data std::vector> unique_alpha; - unique_alpha.push_back( {wfn_traits::alpha_string(dets[0]), 1} ); + unique_alpha.push_back({wfn_traits::alpha_string(dets[0]), 1}); for(size_t i = 1; i < dets.size(); ++i) { auto& [cur_alpha, cur_count] = unique_alpha.back(); auto alpha_i = wfn_traits::alpha_string(dets[i]); - if(alpha_i == cur_alpha) { cur_count++; } - else { + if(alpha_i == cur_alpha) { + cur_count++; + } else { unique_alpha.push_back({alpha_i, 1}); } } // Get offsets std::vector unique_alpha_offsets(unique_alpha.size()); - std::transform_exclusive_scan(unique_alpha.begin(), unique_alpha.end(), - unique_alpha_offsets.begin(), 0ul, std::plus(), - [](auto p){ return p.second; } ); + std::transform_exclusive_scan( + unique_alpha.begin(), unique_alpha.end(), unique_alpha_offsets.begin(), + 0ul, std::plus(), [](auto p) { return p.second; }); - //size_t ntot = std::accumulate( unique_alpha.begin(), unique_alpha.end(), - // 0ul, [](auto s, auto a){ return s + a.second; } ); - //REQUIRE(ntot == dets.size()); + // size_t ntot = std::accumulate( unique_alpha.begin(), unique_alpha.end(), + // 0ul, [](auto s, auto a){ return s + a.second; } ); + // REQUIRE(ntot == dets.size()); // Generate constraints std::vector triplets, quads; for(int i = 0; i < norb; ++i) - for(int j = 0; j < i; ++j) - for(int k = 0; k < j; ++k) { - triplets.emplace_back(macis::make_triplet<64>(i,j,k)); - for(int l = 0; l < k; ++l) { - quads.emplace_back(make_quad<64>(i,j,k,l)); - } - } + for(int j = 0; j < i; ++j) + for(int k = 0; k < j; ++k) { + triplets.emplace_back(macis::make_triplet<64>(i, j, k)); + for(int l = 0; l < k; ++l) { + quads.emplace_back(make_quad<64>(i, j, k, l)); + } + } // Check doubles - auto check_doubles = []( auto det, auto C, auto& doubles ) { + auto check_doubles = [](auto det, auto C, auto& doubles) { // Sanity check auto [_O, _V] = macis::generate_constraint_double_excitations(det, C); - REQUIRE(std::all_of(_O.begin(), _O.end(), [](auto e){ return spin_wfn_traits::count(e) == 2; })); - REQUIRE(std::all_of(_V.begin(), _V.end(), [](auto e){ return spin_wfn_traits::count(e) == 2; })); + REQUIRE(std::all_of(_O.begin(), _O.end(), + [](auto e) { return spin_wfn_traits::count(e) == 2; })); + REQUIRE(std::all_of(_V.begin(), _V.end(), + [](auto e) { return spin_wfn_traits::count(e) == 2; })); // Extract all double excitations that satisfy the constraint std::vector doubles_c; std::copy_if(doubles.begin(), doubles.end(), std::back_inserter(doubles_c), - [=](auto d){ return C.satisfies_constraint(d); }); + [=](auto d) { return C.satisfies_constraint(d); }); // Generate all double excitations that satisfy the constraint std::vector doubles_g; @@ -305,16 +305,16 @@ TEST_CASE("Constraints") { // Compare and check counting std::sort(doubles_c.begin(), doubles_c.end(), spin_wfn_comparator{}); std::sort(doubles_g.begin(), doubles_g.end(), spin_wfn_comparator{}); - REQUIRE( doubles_c == doubles_g ); - REQUIRE( doubles_g.size() == macis::count_constraint_doubles(det, C) ); + REQUIRE(doubles_c == doubles_g); + REQUIRE(doubles_g.size() == macis::count_constraint_doubles(det, C)); }; - // Check singles - auto check_singles = []( auto det, auto C, auto& singles ) { + // Check singles + auto check_singles = [](auto det, auto C, auto& singles) { // Extract all double excitations that satisfy the constraint std::vector singles_c; std::copy_if(singles.begin(), singles.end(), std::back_inserter(singles_c), - [=](auto d){ return C.satisfies_constraint(d); }); + [=](auto d) { return C.satisfies_constraint(d); }); // Generate all double excitations that satisfy the constraint std::vector singles_g; @@ -323,21 +323,21 @@ TEST_CASE("Constraints") { // Compare and check counting std::sort(singles_c.begin(), singles_c.end(), spin_wfn_comparator{}); std::sort(singles_g.begin(), singles_g.end(), spin_wfn_comparator{}); - REQUIRE( singles_c == singles_g ); - REQUIRE( singles_g.size() == macis::count_constraint_singles(det, C) ); + REQUIRE(singles_c == singles_g); + REQUIRE(singles_g.size() == macis::count_constraint_singles(det, C)); }; for(auto i = 0; i < unique_alpha.size(); ++i) { auto det = unique_alpha[i].first; auto det_triplet = top_set_indices<3>(det); - auto det_quad = top_set_indices<4>(det); + auto det_quad = top_set_indices<4>(det); std::vector singles, doubles; macis::generate_singles(norb, det, singles); macis::generate_doubles(norb, det, doubles); - for( auto C : triplets ) { + for(auto C : triplets) { // Check validity of constraint check auto inds = top_set_indices<3>(C.C()); REQUIRE(C.C_min() == inds.back()); @@ -347,7 +347,7 @@ TEST_CASE("Constraints") { check_doubles(det, C, doubles); } - for( auto C : quads ) { + for(auto C : quads) { // Check validity of constraint check auto inds = top_set_indices<4>(C.C()); REQUIRE(C.C_min() == inds.back()); @@ -357,8 +357,6 @@ TEST_CASE("Constraints") { check_doubles(det, C, doubles); } } - - } TEST_CASE("ASCI") { @@ -411,7 +409,7 @@ TEST_CASE("ASCI") { asci_settings, mcscf_settings, E0, std::move(dets), std::move(C), ham_gen, norb MACIS_MPI_CODE(, MPI_COMM_WORLD)); - //std::cout << E0 - -8.542926243842e+01 << std::endl; + // std::cout << E0 - -8.542926243842e+01 << std::endl; REQUIRE(std::abs(E0 - -8.542926243842e+01) < 1e-11); REQUIRE(dets.size() == 10000); REQUIRE(C.size() == 10000); @@ -430,12 +428,13 @@ TEST_CASE("ASCI") { Approx(1.0)); // ASCI-PT2 - auto EPT2 = macis::asci_pt2_constraint( dets.begin(), dets.end(), E0, C, norb, - ham_gen.T(), ham_gen.G_red(), ham_gen.V_red(),ham_gen.G(), ham_gen.V(), - ham_gen MACIS_MPI_CODE(, MPI_COMM_WORLD)); + auto EPT2 = macis::asci_pt2_constraint( + dets.begin(), dets.end(), E0, C, norb, ham_gen.T(), ham_gen.G_red(), + ham_gen.V_red(), ham_gen.G(), ham_gen.V(), + ham_gen MACIS_MPI_CODE(, MPI_COMM_WORLD)); - //std::cout << std::scientific << std::setprecision(12); - //std::cout << EPT2 << std::endl; + // std::cout << std::scientific << std::setprecision(12); + // std::cout << EPT2 << std::endl; REQUIRE(std::abs(EPT2 - -5.701585096318e-03) < 1e-10); MACIS_MPI_CODE(MPI_Barrier(MPI_COMM_WORLD);) diff --git a/tests/double_loop.cxx b/tests/double_loop.cxx index 818d2a4e..f1e4b602 100644 --- a/tests/double_loop.cxx +++ b/tests/double_loop.cxx @@ -6,14 +6,13 @@ * See LICENSE.txt for details */ +#include #include #include #include #include #include -#include - #include "ut_common.hpp" TEST_CASE("Double Loop") { diff --git a/tests/fcidump.cxx b/tests/fcidump.cxx index 9d0d08fe..5540564c 100644 --- a/tests/fcidump.cxx +++ b/tests/fcidump.cxx @@ -8,8 +8,8 @@ #include #include -#include #include +#include #include "ut_common.hpp" diff --git a/tests/fock_matrices.cxx b/tests/fock_matrices.cxx index 042a0e05..f4acdffc 100644 --- a/tests/fock_matrices.cxx +++ b/tests/fock_matrices.cxx @@ -7,9 +7,9 @@ */ #include +#include #include #include -#include #include "ut_common.hpp" diff --git a/tests/mcscf.cxx b/tests/mcscf.cxx index c1a372da..c928ff1f 100644 --- a/tests/mcscf.cxx +++ b/tests/mcscf.cxx @@ -10,9 +10,9 @@ #include #include +#include #include #include -#include #include "ut_common.hpp" diff --git a/tests/sd_operations.cxx b/tests/sd_operations.cxx index 68e62c28..ae540c25 100644 --- a/tests/sd_operations.cxx +++ b/tests/sd_operations.cxx @@ -33,7 +33,7 @@ TEST_CASE("Slater Det Operations") { SECTION("Occupied / Unoccupied Conversion") { SECTION("Default") { - using wfn_type = macis::wfn_t<64>; + using wfn_type = macis::wfn_t<64>; using wfn_traits = macis::wavefunction_traits; wfn_type state = 0x00000000000000AF; std::vector ref_occ = {0, 1, 2, 3, 5, 7}; @@ -258,7 +258,8 @@ TEST_CASE("Slater Det Operations") { SECTION("String Conversions") { using wfn_type = macis::wfn_t<64>; using wfn_traits = macis::wavefunction_traits; - auto state = wfn_traits::canonical_hf_determinant(2, 2).flip(3).flip(4 + 32); + auto state = + wfn_traits::canonical_hf_determinant(2, 2).flip(3).flip(4 + 32); SECTION("To String") { auto str = macis::to_canonical_string(state); diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index 0b4dfeb6..c33b2c5b 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -18,10 +18,10 @@ #include #include #include -#include -#include #include #include +#include +#include #include #include #include @@ -304,8 +304,8 @@ int main(int argc, char** argv) { : spdlog::stdout_color_mt("determinants"); det_logger->info("Print leading determinants > {:.2e}", determinants_threshold); - auto dets = macis::generate_hilbert_space( - n_active, nalpha, nbeta); + auto dets = + macis::generate_hilbert_space(n_active, nalpha, nbeta); for(size_t i = 0; i < dets.size(); ++i) { if(std::abs(C_local[i]) > determinants_threshold) { det_logger->info("{:>16.12f} {}", C_local[i], From f91ee6b2070d3398e003e4cf63569293f962bc67 Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Mon, 25 Sep 2023 14:34:18 -0700 Subject: [PATCH 25/73] ASCI nominally works for open shells --- include/macis/asci/determinant_search.hpp | 2 +- tests/standalone_driver.cxx | 8 ++++---- 2 files changed, 5 insertions(+), 5 deletions(-) diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index e2ad3f55..dc3c6256 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -269,7 +269,7 @@ asci_contrib_container> asci_contributions_constraint( auto gen_c_st = clock_type::now(); auto constraints = dist_constraint_general(asci_settings.constraint_level, norb, - n_sing_alpha, n_doub_alpha, uniq_alpha_wfn, comm); + n_sing_beta, n_doub_beta, uniq_alpha_wfn, comm); auto gen_c_en = clock_type::now(); duration_type gen_c_dur = gen_c_en - gen_c_st; logger->info(" * GEN_DUR = {:.2e} ms", gen_c_dur.count()); diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index c33b2c5b..9db44ca8 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -62,7 +62,7 @@ int main(int argc, char** argv) { spdlog::cfg::load_env_levels(); spdlog::set_pattern("[%n] %v"); - constexpr size_t nwfn_bits = 64; + constexpr size_t nwfn_bits = 128; using wfn_type = macis::wfn_t; using wfn_traits = macis::wavefunction_traits; @@ -315,8 +315,8 @@ int main(int argc, char** argv) { } } else { - if(nalpha != nbeta) - throw std::runtime_error("ASCI Only Implemented for Closed-Shell"); + //if(nalpha != nbeta) + // throw std::runtime_error("ASCI Only Implemented for Closed-Shell"); // Generate the Hamiltonian Generator generator_t ham_gen( @@ -348,7 +348,7 @@ int main(int argc, char** argv) { } else { // HF Guess console->info("Generating HF Guess for ASCI"); - dets = {wfn_traits::canonical_hf_determinant(nalpha, nalpha)}; + dets = {wfn_traits::canonical_hf_determinant(nalpha, nbeta)}; // std::cout << dets[0].to_ullong() << std::endl; E0 = ham_gen.matrix_element(dets[0], dets[0]); C = {1.0}; From 36fc52dbbb1ed5efcbeacbaa2849cfa05cbca713 Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Mon, 2 Oct 2023 13:19:31 -0700 Subject: [PATCH 26/73] Fix bugs in UINT128 interfaces --- include/macis/bitset_operations.hpp | 9 +++++---- include/macis/types.hpp | 2 +- 2 files changed, 6 insertions(+), 5 deletions(-) diff --git a/include/macis/bitset_operations.hpp b/include/macis/bitset_operations.hpp index e0f5ec27..50c7c72e 100644 --- a/include/macis/bitset_operations.hpp +++ b/include/macis/bitset_operations.hpp @@ -86,7 +86,8 @@ template uint128_t to_uint128(std::bitset bits) { static_assert(N <= 128, "N > 128"); if constexpr(N == 128) { - auto _x = reinterpret_cast(&bits); + alignas(alignof(uint128_t)) std::bitset cpy = bits; + auto _x = reinterpret_cast(&cpy); return *_x; } else { return fast_to_ullong(bits); @@ -293,9 +294,9 @@ bool bitset_less(std::bitset x, std::bitset y) { else if constexpr(N <= 64) return fast_to_ullong(x) < fast_to_ullong(y); else if constexpr(N == 128) { - auto _x = reinterpret_cast(&x); - auto _y = reinterpret_cast(&y); - return *_x < *_y; + auto _x = to_uint128(x); + auto _y = to_uint128(y); + return _x < _y; } else { for(int i = N - 1; i >= 0; i--) { if(x[i] ^ y[i]) return y[i]; diff --git a/include/macis/types.hpp b/include/macis/types.hpp index 97331b52..45cee79b 100644 --- a/include/macis/types.hpp +++ b/include/macis/types.hpp @@ -50,7 +50,7 @@ using wavefunction_iterator_t = typename std::vector >::iterator; #pragma GCC diagnostic push #pragma GCC diagnostic ignored "-Wpedantic" -using uint128_t = unsigned __int128; +using uint128_t = __uint128_t; #pragma GCC diagnostic pop template From a218f7317bacb57852396c7b768deee846213bf9 Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Mon, 2 Oct 2023 13:21:08 -0700 Subject: [PATCH 27/73] Fix bug in constraint search + pruning --- include/macis/asci/determinant_search.hpp | 35 ++++++++++++++++------- include/macis/asci/mask_constraints.hpp | 1 + 2 files changed, 25 insertions(+), 11 deletions(-) diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index dc3c6256..dbcabf09 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -161,6 +161,9 @@ asci_contrib_container> asci_contributions_constraint( auto logger = spdlog::get("asci_search"); const size_t ncdets = std::distance(cdets_begin, cdets_end); + auto world_rank = comm_rank(comm); + auto world_size = comm_size(comm); + asci_contrib_container> asci_pairs; std::vector occ_alpha, vir_alpha; std::vector occ_beta, vir_beta; @@ -227,8 +230,6 @@ asci_contrib_container> asci_contributions_constraint( } } - auto world_rank = comm_rank(comm); - auto world_size = comm_size(comm); const auto n_occ_alpha = wfn_traits::count(uniq_alpha_wfn[0]); const auto n_vir_alpha = norb - n_occ_alpha; @@ -283,7 +284,8 @@ asci_contrib_container> asci_contributions_constraint( asci_pairs.reserve(max_size); // Process ASCI pair contributions for each constraint - for(auto con : constraints) { + for(const auto& con : constraints) { + //std::cout << std::distance(constraints.data(), &con) << "/" << constraints.size() << std::endl; auto size_before = asci_pairs.size(); const double h_el_tol = asci_settings.h_el_tol; @@ -366,7 +368,7 @@ asci_contrib_container> asci_contributions_constraint( if(asci_pairs.size() > asci_settings.pair_size_max) { // Remove small contributions auto it = std::partition( - asci_pairs.begin(), asci_pairs.end(), [=](const auto& x) { + asci_pairs.begin() + size_before, asci_pairs.end(), [=](const auto& x) { return std::abs(x.rv()) > asci_settings.rv_prune_tol; }); asci_pairs.erase(it, asci_pairs.end()); @@ -390,11 +392,22 @@ asci_contrib_container> asci_contributions_constraint( } // Pruning } // Unique Alpha Loop + // Local S&A for each quad { + if(size_before > asci_pairs.size()) throw std::runtime_error("DIE DIE DIE"); auto uit = sort_and_accumulate_asci_pairs( asci_pairs.begin() + size_before, asci_pairs.end()); asci_pairs.erase(uit, asci_pairs.end()); + + // Remove small contributions + const auto sz_tmp = asci_pairs.size(); + uit = std::partition(asci_pairs.begin() + size_before, + asci_pairs.end(), [=](const auto &x) { + return std::abs(x.rv()) > asci_settings.rv_prune_tol; + }); + asci_pairs.erase(uit, asci_pairs.end()); + //std::cout << "REMOVED " << sz_tmp - asci_pairs.size() << " PAIRS" << std::endl; } } // Constraint Loop @@ -455,16 +468,16 @@ std::vector> asci_search( // Expand Search Space with Connected ASCI Contributions auto pairs_st = clock_type::now(); asci_contrib_container> asci_pairs; - if(world_size == 1) - asci_pairs = asci_contributions_standard( - asci_settings, cdets_begin, cdets_end, E_ASCI, C, norb, T_pq, G_red, - V_red, G_pqrs, V_pqrs, ham_gen); -#ifdef MACIS_ENABLE_MPI - else + //if(world_size == 1) + // asci_pairs = asci_contributions_standard( + // asci_settings, cdets_begin, cdets_end, E_ASCI, C, norb, T_pq, G_red, + // V_red, G_pqrs, V_pqrs, ham_gen); +//#ifdef MACIS_ENABLE_MPI + //else asci_pairs = asci_contributions_constraint( asci_settings, cdets_begin, cdets_end, E_ASCI, C, norb, T_pq, G_red, V_red, G_pqrs, V_pqrs, ham_gen MACIS_MPI_CODE(, comm)); -#endif +//#endif auto pairs_en = clock_type::now(); { diff --git a/include/macis/asci/mask_constraints.hpp b/include/macis/asci/mask_constraints.hpp index 899d14f7..68ee42c6 100644 --- a/include/macis/asci/mask_constraints.hpp +++ b/include/macis/asci/mask_constraints.hpp @@ -502,6 +502,7 @@ auto make_triplet(unsigned i, unsigned j, unsigned k) { string_type C = 0; C.flip(i).flip(j).flip(k); string_type B = 1; + static_assert(B.size() <= 64, "ULLONG NOT POSSIBLE HERE"); B <<= k; B = B.to_ullong() - 1; From e5e99d41d389ec0c767511a3bee38e4cb89e637d Mon Sep 17 00:00:00 2001 From: Clang Robot Date: Tue, 3 Oct 2023 22:38:01 +0000 Subject: [PATCH 28/73] Committing clang-format changes --- include/macis/asci/determinant_search.hpp | 53 ++++++++++++----------- tests/standalone_driver.cxx | 4 +- 2 files changed, 30 insertions(+), 27 deletions(-) diff --git a/include/macis/asci/determinant_search.hpp b/include/macis/asci/determinant_search.hpp index dbcabf09..05d25059 100644 --- a/include/macis/asci/determinant_search.hpp +++ b/include/macis/asci/determinant_search.hpp @@ -230,7 +230,6 @@ asci_contrib_container> asci_contributions_constraint( } } - const auto n_occ_alpha = wfn_traits::count(uniq_alpha_wfn[0]); const auto n_vir_alpha = norb - n_occ_alpha; const auto n_sing_alpha = n_occ_alpha * n_vir_alpha; @@ -269,8 +268,8 @@ asci_contrib_container> asci_contributions_constraint( auto gen_c_st = clock_type::now(); auto constraints = - dist_constraint_general(asci_settings.constraint_level, norb, - n_sing_beta, n_doub_beta, uniq_alpha_wfn, comm); + dist_constraint_general(asci_settings.constraint_level, norb, n_sing_beta, + n_doub_beta, uniq_alpha_wfn, comm); auto gen_c_en = clock_type::now(); duration_type gen_c_dur = gen_c_en - gen_c_st; logger->info(" * GEN_DUR = {:.2e} ms", gen_c_dur.count()); @@ -285,7 +284,8 @@ asci_contrib_container> asci_contributions_constraint( // Process ASCI pair contributions for each constraint for(const auto& con : constraints) { - //std::cout << std::distance(constraints.data(), &con) << "/" << constraints.size() << std::endl; + // std::cout << std::distance(constraints.data(), &con) << "/" << + // constraints.size() << std::endl; auto size_before = asci_pairs.size(); const double h_el_tol = asci_settings.h_el_tol; @@ -367,10 +367,11 @@ asci_contrib_container> asci_contributions_constraint( // Prune Down Contributions if(asci_pairs.size() > asci_settings.pair_size_max) { // Remove small contributions - auto it = std::partition( - asci_pairs.begin() + size_before, asci_pairs.end(), [=](const auto& x) { - return std::abs(x.rv()) > asci_settings.rv_prune_tol; - }); + auto it = std::partition(asci_pairs.begin() + size_before, + asci_pairs.end(), [=](const auto& x) { + return std::abs(x.rv()) > + asci_settings.rv_prune_tol; + }); asci_pairs.erase(it, asci_pairs.end()); auto c_indices = bits_to_indices(con.C()); @@ -392,22 +393,24 @@ asci_contrib_container> asci_contributions_constraint( } // Pruning } // Unique Alpha Loop - // Local S&A for each quad { - if(size_before > asci_pairs.size()) throw std::runtime_error("DIE DIE DIE"); + if(size_before > asci_pairs.size()) + throw std::runtime_error("DIE DIE DIE"); auto uit = sort_and_accumulate_asci_pairs( asci_pairs.begin() + size_before, asci_pairs.end()); asci_pairs.erase(uit, asci_pairs.end()); // Remove small contributions const auto sz_tmp = asci_pairs.size(); - uit = std::partition(asci_pairs.begin() + size_before, - asci_pairs.end(), [=](const auto &x) { - return std::abs(x.rv()) > asci_settings.rv_prune_tol; - }); + uit = + std::partition(asci_pairs.begin() + size_before, asci_pairs.end(), + [=](const auto& x) { + return std::abs(x.rv()) > asci_settings.rv_prune_tol; + }); asci_pairs.erase(uit, asci_pairs.end()); - //std::cout << "REMOVED " << sz_tmp - asci_pairs.size() << " PAIRS" << std::endl; + // std::cout << "REMOVED " << sz_tmp - asci_pairs.size() << " PAIRS" << + // std::endl; } } // Constraint Loop @@ -468,16 +471,16 @@ std::vector> asci_search( // Expand Search Space with Connected ASCI Contributions auto pairs_st = clock_type::now(); asci_contrib_container> asci_pairs; - //if(world_size == 1) - // asci_pairs = asci_contributions_standard( - // asci_settings, cdets_begin, cdets_end, E_ASCI, C, norb, T_pq, G_red, - // V_red, G_pqrs, V_pqrs, ham_gen); -//#ifdef MACIS_ENABLE_MPI - //else - asci_pairs = asci_contributions_constraint( - asci_settings, cdets_begin, cdets_end, E_ASCI, C, norb, T_pq, G_red, - V_red, G_pqrs, V_pqrs, ham_gen MACIS_MPI_CODE(, comm)); -//#endif + // if(world_size == 1) + // asci_pairs = asci_contributions_standard( + // asci_settings, cdets_begin, cdets_end, E_ASCI, C, norb, T_pq, G_red, + // V_red, G_pqrs, V_pqrs, ham_gen); + // #ifdef MACIS_ENABLE_MPI + // else + asci_pairs = asci_contributions_constraint( + asci_settings, cdets_begin, cdets_end, E_ASCI, C, norb, T_pq, G_red, + V_red, G_pqrs, V_pqrs, ham_gen MACIS_MPI_CODE(, comm)); + // #endif auto pairs_en = clock_type::now(); { diff --git a/tests/standalone_driver.cxx b/tests/standalone_driver.cxx index 9db44ca8..82c4bd51 100644 --- a/tests/standalone_driver.cxx +++ b/tests/standalone_driver.cxx @@ -315,8 +315,8 @@ int main(int argc, char** argv) { } } else { - //if(nalpha != nbeta) - // throw std::runtime_error("ASCI Only Implemented for Closed-Shell"); + // if(nalpha != nbeta) + // throw std::runtime_error("ASCI Only Implemented for Closed-Shell"); // Generate the Hamiltonian Generator generator_t ham_gen( From a43e2540522b5150d26f8800ccba181db40cbd2e Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Wed, 4 Oct 2023 17:02:20 -0700 Subject: [PATCH 29/73] Cleanup of bitset operations + UTs, extension of more functions to larger bitsets --- include/macis/bitset_operations.hpp | 99 +++++++++--- tests/bitset_operations.cxx | 241 ++++++++++++++++++++-------- 2 files changed, 250 insertions(+), 90 deletions(-) diff --git a/include/macis/bitset_operations.hpp b/include/macis/bitset_operations.hpp index 50c7c72e..06b7d13b 100644 --- a/include/macis/bitset_operations.hpp +++ b/include/macis/bitset_operations.hpp @@ -157,12 +157,15 @@ uint32_t ffs(std::bitset bits) { return ffsl(fast_to_ulong(bits)); else if constexpr(N <= 64) return ffsll(fast_to_ullong(bits)); - else if constexpr(N <= 128) { + else if constexpr(N % 64 == 0) { auto as_words = reinterpret_cast(&bits); - if(as_words[0]) - return ffsll(as_words[0]); - else - return ffsll(as_words[1]) + 64; + constexpr int n_words = N / 64; + int off = 0; + for(int i = 0; i < n_words; ++i) { + if(as_words[i]) return ffsll(as_words[i]) + off; + off += 64; + } + return 0; } else { uint32_t ind = 0; for(ind = 0; ind < N; ++ind) @@ -188,17 +191,20 @@ uint32_t fls(std::bitset bits) { return fls(fast_to_ulong(bits)); else if constexpr(N <= 64) return fls(fast_to_ullong(bits)); - else if constexpr(N <= 128) { + else if constexpr(N % 64 == 0) { auto as_words = reinterpret_cast(&bits); - if(as_words[1]) - return fls(as_words[1]) + 64; - else - return fls(as_words[0]); + constexpr int n_words = N / 64; + int off = N - 64; + for(int i = n_words-1; i >= 0; --i) { + if(as_words[i]) return fls(as_words[i]) + off; + off -= 64; + } + return UINT32_MAX; } else { uint32_t ind = 0; for(ind = N - 1; ind >= 0; ind--) if(bits[ind]) return ind; - return ind; + return UINT32_MAX; } abort(); } @@ -225,6 +231,7 @@ std::vector bits_to_indices(std::bitset bits) { return indices; } +#if 0 /// Truncate a bitset to one of smaller width template inline std::bitset truncate_bitset(std::bitset bits) { @@ -243,6 +250,7 @@ inline std::bitset truncate_bitset(std::bitset bits) { return trunc_bits; } } +#endif /// Expand a bitset to one of larger width template @@ -265,27 +273,70 @@ inline std::bitset expand_bitset(std::bitset bits) { /// Extract to lo word of a bitset of even width template inline std::bitset bitset_lo_word(std::bitset bits) { - static_assert(N == 128 or N == 64, "Not Supported"); - if constexpr(N == 128) { - return std::bitset<64>(reinterpret_cast(&bits)[0]); - } + static_assert((N % 64 == 0) and (N == 64 or N/2 % 64 == 0), "Not Supported"); if constexpr(N == 64) { return std::bitset<32>(reinterpret_cast(&bits)[0]); + } else { + std::bitset lo; + constexpr int nword = (N/2) / 64; + auto lo_as_words = reinterpret_cast(&lo); + auto bi_as_words = reinterpret_cast(&bits); + for(int i = 0; i < nword; ++i) lo_as_words[i] = bi_as_words[i]; + return lo; + } +} + +template +inline void set_bitset_lo_word(std::bitset& bits, std::bitset word) { + static_assert((N % 64 == 0) and (N == 64 or N/2 % 64 == 0), "Not Supported"); + + if constexpr(N == 64) { + auto bi_as_words = reinterpret_cast(&bits); + auto wo_as_words = reinterpret_cast(&word); + bi_as_words[0] = wo_as_words[0]; + } else { + constexpr int nword = (N/2) / 64; + auto bi_as_words = reinterpret_cast(&bits); + auto wo_as_words = reinterpret_cast(&word); + for(int i = 0; i < nword; ++i) bi_as_words[i] = wo_as_words[i]; } } /// Extract to hi word of a bitset of even width template inline std::bitset bitset_hi_word(std::bitset bits) { - static_assert(N == 128 or N == 64, "Not Supported"); - if constexpr(N == 128) { - return std::bitset<64>(reinterpret_cast(&bits)[1]); - } + static_assert((N % 64 == 0) and (N == 64 or N/2 % 64 == 0), "Not Supported"); if constexpr(N == 64) { return std::bitset<32>(reinterpret_cast(&bits)[1]); + } else { + std::bitset hi; + constexpr int nword = (N/2) / 64; + auto hi_as_words = reinterpret_cast(&hi); + auto bi_as_words = reinterpret_cast(&bits); + for(int i = 0; i < nword; ++i) hi_as_words[i] = bi_as_words[i + nword]; + return hi; + } +} + +template +inline void set_bitset_hi_word(std::bitset& bits, std::bitset word) { + static_assert((N % 64 == 0) and (N == 64 or N/2 % 64 == 0), "Not Supported"); + + if constexpr(N == 64) { + auto bi_as_words = reinterpret_cast(&bits); + auto wo_as_words = reinterpret_cast(&word); + bi_as_words[1] = wo_as_words[0]; + } else { + constexpr int nword = (N/2) / 64; + auto bi_as_words = reinterpret_cast(&bits); + auto wo_as_words = reinterpret_cast(&word); + for(int i = 0; i < nword; ++i) bi_as_words[i+nword] = wo_as_words[i]; } } + + + /// Bitwise less-than operator for bitset template bool bitset_less(std::bitset x, std::bitset y) { @@ -297,6 +348,16 @@ bool bitset_less(std::bitset x, std::bitset y) { auto _x = to_uint128(x); auto _y = to_uint128(y); return _x < _y; + } else if constexpr(N % 64 == 0) { + auto x_as_words = reinterpret_cast(&x); + auto y_as_words = reinterpret_cast(&y); + constexpr auto nwords = N / 64; + for(int i = nwords - 1; i >= 0; --i) { + const auto x_i = x_as_words[i]; + const auto y_i = y_as_words[i]; + if(x_i != y_i) return x_i < y_i; + } + return false; } else { for(int i = N - 1; i >= 0; i--) { if(x[i] ^ y[i]) return y[i]; diff --git a/tests/bitset_operations.cxx b/tests/bitset_operations.cxx index e69516a8..5498351e 100644 --- a/tests/bitset_operations.cxx +++ b/tests/bitset_operations.cxx @@ -11,6 +11,9 @@ #include "ut_common.hpp" +template +using bs = std::bitset; + template void uint128_conversion_test() { using ref_type = macis::uint128_t; @@ -37,7 +40,135 @@ void uint128_conversion_test() { } template -using bs = std::bitset; +void mask_test() { + bs full = ~bs(0); + bs full_128 = N > 128 ? full >> (N-128) : 0; + bs full_64 = N > 64 ? full >> (N-64) : 0; + bs full_32 = N > 32 ? full >> (N-32) : 0; + + REQUIRE(full == macis::full_mask()); + if constexpr (N > 128) REQUIRE(full_128 == macis::full_mask<128,N>()); + if constexpr (N > 64) REQUIRE(full_64 == macis::full_mask<64,N>() ); + if constexpr (N > 32) REQUIRE(full_32 == macis::full_mask<32,N>() ); + + REQUIRE(full == macis::full_mask(N)); + if constexpr (N > 128) REQUIRE(full_128 == macis::full_mask(128)); + if constexpr (N > 64) REQUIRE(full_64 == macis::full_mask(64) ); + if constexpr (N > 32) REQUIRE(full_32 == macis::full_mask(32) ); +} + +template +void ffs_test() { + REQUIRE(macis::ffs(bs()) == 0); + REQUIRE(macis::ffs(bs(1)) == 1); + + bs a(0xABC); + REQUIRE(macis::ffs(a) == 3); + if(N > 32) REQUIRE(macis::ffs(a << 32) == 3 + 32 ); + if(N > 64) REQUIRE(macis::ffs(a << 64) == 3 + 64 ); + if(N > 128) REQUIRE(macis::ffs(a << 128) == 3 + 128); +} + +template +void fls_test() { + REQUIRE(macis::fls(bs()) == UINT32_MAX); + REQUIRE(macis::fls(bs(1)) == 0 ); + + bs a(0xDEADBEEF); + REQUIRE(macis::fls(a) == 31); + if(N > 32) REQUIRE(macis::fls(a << 32) == 31 + 32 ); + if(N > 64) REQUIRE(macis::fls(a << 64) == 31 + 64 ); + if(N > 128) REQUIRE(macis::fls(a << 128) == 31 + 128); +} + +template +void indices_test() { + std::vector indices = {5}; + if (N > 32) indices.emplace_back(6+32); + if (N > 64) indices.emplace_back(7+64); + if (N > 128) indices.emplace_back(8+128); + + bs one(1), a(0); + for(auto i : indices) a |= one << i; + REQUIRE(indices == macis::bits_to_indices(a)); +} + +template +void lo_word_test() { + bs a(0); + bs b(0); + size_t n_32_words = N / 32; + for(int i = 0; i < n_32_words; ++i) { + a |= bs(0xDEADBEEF + i) << (i*32); + } + for(int i = 0; i < n_32_words/2; ++i) { + b |= bs(0xDEADBEEF + i) << (i*32); + } + + REQUIRE(macis::bitset_lo_word(a) == b); + + bs c(0); + macis::set_bitset_lo_word(c, b); + REQUIRE( (a << N/2) >> N/2 == c ); +} + +template +void hi_word_test() { + bs a(0); + bs b(0); + size_t n_32_words = N / 32; + for(int i = 0; i < n_32_words; ++i) { + a |= bs(0xDEADBEEF + i) << (i*32); + } + for(int i = 0; i < n_32_words/2; ++i) { + b |= bs(0xDEADBEEF + (i+n_32_words/2)) << (i*32); + } + + REQUIRE(macis::bitset_hi_word(a) == b); + + bs c(0); + macis::set_bitset_hi_word(c, b); + REQUIRE( (a >> N/2) << N/2 == c ); +} + +template +void bitset_less_test() { + bs a(65), b(42); + REQUIRE(macis::bitset_less(b, a)); + REQUIRE_FALSE(macis::bitset_less(a, a)); + REQUIRE_FALSE(macis::bitset_less(a, b)); + + if(N > 32) { + auto aa = a << 32; + auto bb = b << 32; + REQUIRE(macis::bitset_less(bb, aa)); + REQUIRE_FALSE(macis::bitset_less(aa, aa)); + REQUIRE_FALSE(macis::bitset_less(aa, bb)); + REQUIRE_FALSE(macis::bitset_less(aa, b)); + REQUIRE_FALSE(macis::bitset_less(aa, a)); + } + + if(N > 64) { + auto aa = a << 64; + auto bb = b << 64; + REQUIRE(macis::bitset_less(bb, aa)); + REQUIRE_FALSE(macis::bitset_less(aa, aa)); + REQUIRE_FALSE(macis::bitset_less(aa, bb)); + REQUIRE_FALSE(macis::bitset_less(aa, b)); + REQUIRE_FALSE(macis::bitset_less(aa, a)); + } + + if(N > 128) { + auto aa = a << 128; + auto bb = b << 128; + REQUIRE(macis::bitset_less(bb, aa)); + REQUIRE_FALSE(macis::bitset_less(aa, aa)); + REQUIRE_FALSE(macis::bitset_less(aa, bb)); + REQUIRE_FALSE(macis::bitset_less(aa, b)); + REQUIRE_FALSE(macis::bitset_less(aa, a)); + } +} + TEST_CASE("Bitset Operations") { ROOT_ONLY(MPI_COMM_WORLD); @@ -54,63 +185,34 @@ TEST_CASE("Bitset Operations") { } SECTION("Full Mask") { - bs<128> full_128 = ~bs<128>(0); - bs<128> full_64 = bs<128>(UINT64_MAX); - bs<128> full_32 = bs<128>(UINT32_MAX); - - SECTION("Static") { - REQUIRE(full_128 == macis::full_mask<128>()); - REQUIRE(full_64 == macis::full_mask<64, 128>()); - REQUIRE(full_32 == macis::full_mask<32, 128>()); - } - - SECTION("Dynamic") { - REQUIRE(full_128 == macis::full_mask<128>(128)); - REQUIRE(full_64 == macis::full_mask<128>(64)); - REQUIRE(full_32 == macis::full_mask<128>(32)); - } + SECTION("32" ) { mask_test<32 >(); } + SECTION("64" ) { mask_test<64 >(); } + SECTION("128") { mask_test<128>(); } + SECTION("256") { mask_test<256>(); } } SECTION("FFS") { - SECTION("Zero") { REQUIRE(macis::ffs(bs<64>()) == 0); } - SECTION("One") { REQUIRE(macis::ffs(bs<64>(1)) == 1); } - SECTION("Arbitrary") { - bs<64> a(0x0A0A); - REQUIRE(macis::ffs(a) == 2); - bs<32> b(0x0A0A); - REQUIRE(macis::ffs(b) == 2); - bs<128> c(0xABC); - REQUIRE(macis::ffs(c) == 3); - REQUIRE(macis::ffs(c << 64) == 3 + 64); - bs<256> d(0xABC); - REQUIRE(macis::ffs(d) == 3); - REQUIRE(macis::ffs(d << 64) == 3 + 64); - REQUIRE(macis::ffs(d << 128) == 3 + 128); - } + SECTION("32" ) { ffs_test<32 >(); } + SECTION("64" ) { ffs_test<64 >(); } + SECTION("128") { ffs_test<128>(); } + SECTION("256") { ffs_test<256>(); } } SECTION("FLS") { - bs<64> a(0x0A0A); - REQUIRE(macis::fls(a) == 12 - 1); - bs<32> b(0x0A0A); - REQUIRE(macis::fls(b) == 12 - 1); - bs<128> c(0xDEADBEEF); - REQUIRE(macis::fls(c) == 31); - REQUIRE(macis::fls(c << 64) == 31 + 64); - bs<256> d(0xDEADBEEF); - REQUIRE(macis::fls(d) == 31); - REQUIRE(macis::fls(d << 64) == 31 + 64); - REQUIRE(macis::fls(d << 128) == 31 + 128); + SECTION("32" ) { fls_test<32 >(); } + SECTION("64" ) { fls_test<64 >(); } + SECTION("128") { fls_test<128>(); } + SECTION("256") { fls_test<256>(); } } SECTION("Indices") { - bs<128> one(1); - bs<128> a = (one << 4) | (one << 67) | (one << 118) | (one << 31); - auto ind = macis::bits_to_indices(a); - std::vector ref = {4, 31, 67, 118}; - REQUIRE(ind == ref); + SECTION("32" ) { indices_test<32 >(); } + SECTION("64" ) { indices_test<64 >(); } + SECTION("128") { indices_test<128>(); } + SECTION("256") { indices_test<256>(); } } +#if 0 SECTION("Truncate") { bs<64> a_64(0xCCCCCCCCDEADDEAD); bs<32> ref(0xDEADDEAD); @@ -122,31 +224,28 @@ TEST_CASE("Bitset Operations") { bs<64> ref(0x00000000DEADDEAD); REQUIRE(macis::expand_bitset<64>(a_32) == ref); } +#endif + + SECTION("LO WORDS") { + SECTION("64" ) { lo_word_test<64 >(); } + SECTION("128") { lo_word_test<128>(); } + SECTION("256") { lo_word_test<256>(); } + SECTION("512") { lo_word_test<512>(); } + SECTION("1024") { lo_word_test<1024>(); } + } + + SECTION("HI WORDS") { + SECTION("64" ) { hi_word_test<64 >(); } + SECTION("128") { hi_word_test<128>(); } + SECTION("256") { hi_word_test<256>(); } + SECTION("512") { hi_word_test<512>(); } + SECTION("1024") { hi_word_test<1024>(); } + } SECTION("Compare") { - SECTION("32 bit") { - bs<32> a(65), b(42); - REQUIRE(macis::bitset_less(b, a)); - REQUIRE_FALSE(macis::bitset_less(a, b)); - } - SECTION("64 bit") { - bs<64> a(65ull << 32), b(42ull << 32); - REQUIRE(macis::bitset_less(b, a)); - REQUIRE_FALSE(macis::bitset_less(a, b)); - } - SECTION("128 bit") { - bs<128> a(65ull), b(42ull); - a = a << 64; - b = b << 64; - REQUIRE(macis::bitset_less(b, a)); - REQUIRE_FALSE(macis::bitset_less(a, b)); - } - SECTION("256 bit") { - bs<256> a(65ull), b(42ull); - a = a << 128; - b = b << 128; - REQUIRE(macis::bitset_less(b, a)); - REQUIRE_FALSE(macis::bitset_less(a, b)); - } + SECTION("32" ) { bitset_less_test<32 >(); } + SECTION("64" ) { bitset_less_test<64 >(); } + SECTION("128") { bitset_less_test<128>(); } + SECTION("256") { bitset_less_test<256>(); } } } From 8ae7f33cc633e9d0366ac6eef67a647aa571d535 Mon Sep 17 00:00:00 2001 From: Clang Robot Date: Thu, 5 Oct 2023 00:03:18 +0000 Subject: [PATCH 30/73] Committing clang-format changes --- include/macis/bitset_operations.hpp | 41 +++++----- tests/bitset_operations.cxx | 121 ++++++++++++++-------------- 2 files changed, 81 insertions(+), 81 deletions(-) diff --git a/include/macis/bitset_operations.hpp b/include/macis/bitset_operations.hpp index 06b7d13b..66a56a59 100644 --- a/include/macis/bitset_operations.hpp +++ b/include/macis/bitset_operations.hpp @@ -195,7 +195,7 @@ uint32_t fls(std::bitset bits) { auto as_words = reinterpret_cast(&bits); constexpr int n_words = N / 64; int off = N - 64; - for(int i = n_words-1; i >= 0; --i) { + for(int i = n_words - 1; i >= 0; --i) { if(as_words[i]) return fls(as_words[i]) + off; off -= 64; } @@ -273,12 +273,13 @@ inline std::bitset expand_bitset(std::bitset bits) { /// Extract to lo word of a bitset of even width template inline std::bitset bitset_lo_word(std::bitset bits) { - static_assert((N % 64 == 0) and (N == 64 or N/2 % 64 == 0), "Not Supported"); + static_assert((N % 64 == 0) and (N == 64 or N / 2 % 64 == 0), + "Not Supported"); if constexpr(N == 64) { return std::bitset<32>(reinterpret_cast(&bits)[0]); - } else { - std::bitset lo; - constexpr int nword = (N/2) / 64; + } else { + std::bitset lo; + constexpr int nword = (N / 2) / 64; auto lo_as_words = reinterpret_cast(&lo); auto bi_as_words = reinterpret_cast(&bits); for(int i = 0; i < nword; ++i) lo_as_words[i] = bi_as_words[i]; @@ -287,15 +288,16 @@ inline std::bitset bitset_lo_word(std::bitset bits) { } template -inline void set_bitset_lo_word(std::bitset& bits, std::bitset word) { - static_assert((N % 64 == 0) and (N == 64 or N/2 % 64 == 0), "Not Supported"); +inline void set_bitset_lo_word(std::bitset& bits, std::bitset word) { + static_assert((N % 64 == 0) and (N == 64 or N / 2 % 64 == 0), + "Not Supported"); if constexpr(N == 64) { auto bi_as_words = reinterpret_cast(&bits); auto wo_as_words = reinterpret_cast(&word); bi_as_words[0] = wo_as_words[0]; - } else { - constexpr int nword = (N/2) / 64; + } else { + constexpr int nword = (N / 2) / 64; auto bi_as_words = reinterpret_cast(&bits); auto wo_as_words = reinterpret_cast(&word); for(int i = 0; i < nword; ++i) bi_as_words[i] = wo_as_words[i]; @@ -305,12 +307,13 @@ inline void set_bitset_lo_word(std::bitset& bits, std::bitset word) { /// Extract to hi word of a bitset of even width template inline std::bitset bitset_hi_word(std::bitset bits) { - static_assert((N % 64 == 0) and (N == 64 or N/2 % 64 == 0), "Not Supported"); + static_assert((N % 64 == 0) and (N == 64 or N / 2 % 64 == 0), + "Not Supported"); if constexpr(N == 64) { return std::bitset<32>(reinterpret_cast(&bits)[1]); } else { - std::bitset hi; - constexpr int nword = (N/2) / 64; + std::bitset hi; + constexpr int nword = (N / 2) / 64; auto hi_as_words = reinterpret_cast(&hi); auto bi_as_words = reinterpret_cast(&bits); for(int i = 0; i < nword; ++i) hi_as_words[i] = bi_as_words[i + nword]; @@ -319,24 +322,22 @@ inline std::bitset bitset_hi_word(std::bitset bits) { } template -inline void set_bitset_hi_word(std::bitset& bits, std::bitset word) { - static_assert((N % 64 == 0) and (N == 64 or N/2 % 64 == 0), "Not Supported"); +inline void set_bitset_hi_word(std::bitset& bits, std::bitset word) { + static_assert((N % 64 == 0) and (N == 64 or N / 2 % 64 == 0), + "Not Supported"); if constexpr(N == 64) { auto bi_as_words = reinterpret_cast(&bits); auto wo_as_words = reinterpret_cast(&word); bi_as_words[1] = wo_as_words[0]; - } else { - constexpr int nword = (N/2) / 64; + } else { + constexpr int nword = (N / 2) / 64; auto bi_as_words = reinterpret_cast(&bits); auto wo_as_words = reinterpret_cast(&word); - for(int i = 0; i < nword; ++i) bi_as_words[i+nword] = wo_as_words[i]; + for(int i = 0; i < nword; ++i) bi_as_words[i + nword] = wo_as_words[i]; } } - - - /// Bitwise less-than operator for bitset template bool bitset_less(std::bitset x, std::bitset y) { diff --git a/tests/bitset_operations.cxx b/tests/bitset_operations.cxx index 5498351e..2fd4673e 100644 --- a/tests/bitset_operations.cxx +++ b/tests/bitset_operations.cxx @@ -41,52 +41,52 @@ void uint128_conversion_test() { template void mask_test() { - bs full = ~bs(0); - bs full_128 = N > 128 ? full >> (N-128) : 0; - bs full_64 = N > 64 ? full >> (N-64) : 0; - bs full_32 = N > 32 ? full >> (N-32) : 0; + bs full = ~bs(0); + bs full_128 = N > 128 ? full >> (N - 128) : 0; + bs full_64 = N > 64 ? full >> (N - 64) : 0; + bs full_32 = N > 32 ? full >> (N - 32) : 0; REQUIRE(full == macis::full_mask()); - if constexpr (N > 128) REQUIRE(full_128 == macis::full_mask<128,N>()); - if constexpr (N > 64) REQUIRE(full_64 == macis::full_mask<64,N>() ); - if constexpr (N > 32) REQUIRE(full_32 == macis::full_mask<32,N>() ); + if constexpr(N > 128) REQUIRE(full_128 == macis::full_mask<128, N>()); + if constexpr(N > 64) REQUIRE(full_64 == macis::full_mask<64, N>()); + if constexpr(N > 32) REQUIRE(full_32 == macis::full_mask<32, N>()); REQUIRE(full == macis::full_mask(N)); - if constexpr (N > 128) REQUIRE(full_128 == macis::full_mask(128)); - if constexpr (N > 64) REQUIRE(full_64 == macis::full_mask(64) ); - if constexpr (N > 32) REQUIRE(full_32 == macis::full_mask(32) ); + if constexpr(N > 128) REQUIRE(full_128 == macis::full_mask(128)); + if constexpr(N > 64) REQUIRE(full_64 == macis::full_mask(64)); + if constexpr(N > 32) REQUIRE(full_32 == macis::full_mask(32)); } template void ffs_test() { - REQUIRE(macis::ffs(bs()) == 0); - REQUIRE(macis::ffs(bs(1)) == 1); - - bs a(0xABC); - REQUIRE(macis::ffs(a) == 3); - if(N > 32) REQUIRE(macis::ffs(a << 32) == 3 + 32 ); - if(N > 64) REQUIRE(macis::ffs(a << 64) == 3 + 64 ); - if(N > 128) REQUIRE(macis::ffs(a << 128) == 3 + 128); + REQUIRE(macis::ffs(bs()) == 0); + REQUIRE(macis::ffs(bs(1)) == 1); + + bs a(0xABC); + REQUIRE(macis::ffs(a) == 3); + if(N > 32) REQUIRE(macis::ffs(a << 32) == 3 + 32); + if(N > 64) REQUIRE(macis::ffs(a << 64) == 3 + 64); + if(N > 128) REQUIRE(macis::ffs(a << 128) == 3 + 128); } template void fls_test() { - REQUIRE(macis::fls(bs()) == UINT32_MAX); - REQUIRE(macis::fls(bs(1)) == 0 ); - - bs a(0xDEADBEEF); - REQUIRE(macis::fls(a) == 31); - if(N > 32) REQUIRE(macis::fls(a << 32) == 31 + 32 ); - if(N > 64) REQUIRE(macis::fls(a << 64) == 31 + 64 ); - if(N > 128) REQUIRE(macis::fls(a << 128) == 31 + 128); + REQUIRE(macis::fls(bs()) == UINT32_MAX); + REQUIRE(macis::fls(bs(1)) == 0); + + bs a(0xDEADBEEF); + REQUIRE(macis::fls(a) == 31); + if(N > 32) REQUIRE(macis::fls(a << 32) == 31 + 32); + if(N > 64) REQUIRE(macis::fls(a << 64) == 31 + 64); + if(N > 128) REQUIRE(macis::fls(a << 128) == 31 + 128); } template void indices_test() { std::vector indices = {5}; - if (N > 32) indices.emplace_back(6+32); - if (N > 64) indices.emplace_back(7+64); - if (N > 128) indices.emplace_back(8+128); + if(N > 32) indices.emplace_back(6 + 32); + if(N > 64) indices.emplace_back(7 + 64); + if(N > 128) indices.emplace_back(8 + 128); bs one(1), a(0); for(auto i : indices) a |= one << i; @@ -95,40 +95,40 @@ void indices_test() { template void lo_word_test() { - bs a(0); - bs b(0); + bs a(0); + bs b(0); size_t n_32_words = N / 32; for(int i = 0; i < n_32_words; ++i) { - a |= bs(0xDEADBEEF + i) << (i*32); + a |= bs(0xDEADBEEF + i) << (i * 32); } - for(int i = 0; i < n_32_words/2; ++i) { - b |= bs(0xDEADBEEF + i) << (i*32); + for(int i = 0; i < n_32_words / 2; ++i) { + b |= bs(0xDEADBEEF + i) << (i * 32); } REQUIRE(macis::bitset_lo_word(a) == b); bs c(0); macis::set_bitset_lo_word(c, b); - REQUIRE( (a << N/2) >> N/2 == c ); + REQUIRE((a << N / 2) >> N / 2 == c); } template void hi_word_test() { - bs a(0); - bs b(0); + bs a(0); + bs b(0); size_t n_32_words = N / 32; for(int i = 0; i < n_32_words; ++i) { - a |= bs(0xDEADBEEF + i) << (i*32); + a |= bs(0xDEADBEEF + i) << (i * 32); } - for(int i = 0; i < n_32_words/2; ++i) { - b |= bs(0xDEADBEEF + (i+n_32_words/2)) << (i*32); + for(int i = 0; i < n_32_words / 2; ++i) { + b |= bs(0xDEADBEEF + (i + n_32_words / 2)) << (i * 32); } REQUIRE(macis::bitset_hi_word(a) == b); bs c(0); macis::set_bitset_hi_word(c, b); - REQUIRE( (a >> N/2) << N/2 == c ); + REQUIRE((a >> N / 2) << N / 2 == c); } template @@ -137,7 +137,7 @@ void bitset_less_test() { REQUIRE(macis::bitset_less(b, a)); REQUIRE_FALSE(macis::bitset_less(a, a)); REQUIRE_FALSE(macis::bitset_less(a, b)); - + if(N > 32) { auto aa = a << 32; auto bb = b << 32; @@ -169,7 +169,6 @@ void bitset_less_test() { } } - TEST_CASE("Bitset Operations") { ROOT_ONLY(MPI_COMM_WORLD); @@ -185,29 +184,29 @@ TEST_CASE("Bitset Operations") { } SECTION("Full Mask") { - SECTION("32" ) { mask_test<32 >(); } - SECTION("64" ) { mask_test<64 >(); } + SECTION("32") { mask_test<32>(); } + SECTION("64") { mask_test<64>(); } SECTION("128") { mask_test<128>(); } SECTION("256") { mask_test<256>(); } } SECTION("FFS") { - SECTION("32" ) { ffs_test<32 >(); } - SECTION("64" ) { ffs_test<64 >(); } + SECTION("32") { ffs_test<32>(); } + SECTION("64") { ffs_test<64>(); } SECTION("128") { ffs_test<128>(); } SECTION("256") { ffs_test<256>(); } } SECTION("FLS") { - SECTION("32" ) { fls_test<32 >(); } - SECTION("64" ) { fls_test<64 >(); } + SECTION("32") { fls_test<32>(); } + SECTION("64") { fls_test<64>(); } SECTION("128") { fls_test<128>(); } SECTION("256") { fls_test<256>(); } } SECTION("Indices") { - SECTION("32" ) { indices_test<32 >(); } - SECTION("64" ) { indices_test<64 >(); } + SECTION("32") { indices_test<32>(); } + SECTION("64") { indices_test<64>(); } SECTION("128") { indices_test<128>(); } SECTION("256") { indices_test<256>(); } } @@ -227,24 +226,24 @@ TEST_CASE("Bitset Operations") { #endif SECTION("LO WORDS") { - SECTION("64" ) { lo_word_test<64 >(); } - SECTION("128") { lo_word_test<128>(); } - SECTION("256") { lo_word_test<256>(); } - SECTION("512") { lo_word_test<512>(); } + SECTION("64") { lo_word_test<64>(); } + SECTION("128") { lo_word_test<128>(); } + SECTION("256") { lo_word_test<256>(); } + SECTION("512") { lo_word_test<512>(); } SECTION("1024") { lo_word_test<1024>(); } } SECTION("HI WORDS") { - SECTION("64" ) { hi_word_test<64 >(); } - SECTION("128") { hi_word_test<128>(); } - SECTION("256") { hi_word_test<256>(); } - SECTION("512") { hi_word_test<512>(); } + SECTION("64") { hi_word_test<64>(); } + SECTION("128") { hi_word_test<128>(); } + SECTION("256") { hi_word_test<256>(); } + SECTION("512") { hi_word_test<512>(); } SECTION("1024") { hi_word_test<1024>(); } } SECTION("Compare") { - SECTION("32" ) { bitset_less_test<32 >(); } - SECTION("64" ) { bitset_less_test<64 >(); } + SECTION("32") { bitset_less_test<32>(); } + SECTION("64") { bitset_less_test<64>(); } SECTION("128") { bitset_less_test<128>(); } SECTION("256") { bitset_less_test<256>(); } } From 0fd26cd77027203f87f13923b74d412559645a2a Mon Sep 17 00:00:00 2001 From: David Williams-Young Date: Tue, 10 Oct 2023 13:19:05 -0700 Subject: [PATCH 31/73] Added SortedDoubleLoop + required sparsexx functions and UTs, correct but underperfoming --- include/macis/asci/iteration.hpp | 5 + .../sorted_double_loop.hpp | 256 ++++++++++++++++++ include/macis/sd_operations.hpp | 22 ++ .../sparsexx/matrix_types/coo_matrix.hpp | 10 + src/sparsexx/tests/CMakeLists.txt | 2 +- src/sparsexx/tests/test_types.cxx | 33 +++ tests/csr_hamiltonian.cxx | 28 +- tests/ref_data/h2o.ccpvdz.cisd.colind.bin | Bin 14071264 -> 14071264 bytes tests/ref_data/h2o.ccpvdz.cisd.nzval.bin | Bin 28142528 -> 28142528 bytes tests/ref_data/h2o.ccpvdz.cisd.rowptr.bin | Bin 50548 -> 50548 bytes 10 files changed, 352 insertions(+), 4 deletions(-) create mode 100644 include/macis/hamiltonian_generator/sorted_double_loop.hpp create mode 100644 src/sparsexx/tests/test_types.cxx diff --git a/include/macis/asci/iteration.hpp b/include/macis/asci/iteration.hpp index 742fe321..f9bffc22 100644 --- a/include/macis/asci/iteration.hpp +++ b/include/macis/asci/iteration.hpp @@ -29,6 +29,11 @@ auto asci_iter(ASCISettings asci_settings, MCSCFSettings mcscf_settings, E0, X, norb, ham_gen.T(), ham_gen.G_red(), ham_gen.V_red(), ham_gen.G(), ham_gen.V(), ham_gen MACIS_MPI_CODE(, comm)); + //std::sort(wfn.begin(), wfn.end(), bitset_less_comparator{}); + using wfn_traits = wavefunction_traits>; + using wfn_comp = typename wfn_traits::spin_comparator; + std::sort(wfn.begin(), wfn.end(), wfn_comp{}); + // Rediagonalize std::vector X_local; // Precludes guess reuse auto E = selected_ci_diag( diff --git a/include/macis/hamiltonian_generator/sorted_double_loop.hpp b/include/macis/hamiltonian_generator/sorted_double_loop.hpp new file mode 100644 index 00000000..50050dd6 --- /dev/null +++ b/include/macis/hamiltonian_generator/sorted_double_loop.hpp @@ -0,0 +1,256 @@ +/* + * MACIS Copyright (c) 2023, The Regents of the University of California, + * through Lawrence Berkeley National Laboratory (subject to receipt of + * any required approvals from the U.S. Dept. of Energy). All rights reserved. + * + * See LICENSE.txt for details + */ + +#pragma once +#include +#include +#include +#include + +namespace macis { + +template +class SortedDoubleLoopHamiltonianGenerator : public HamiltonianGenerator { + public: + using base_type = HamiltonianGenerator; + using full_det_t = typename base_type::full_det_t; + using spin_det_t = typename base_type::spin_det_t; + using full_det_iterator = typename base_type::full_det_iterator; + using matrix_span_t = typename base_type::matrix_span_t; + using rank4_span_t = typename base_type::rank4_span_t; + + template + using sparse_matrix_type = sparsexx::csr_matrix; + + protected: + template + sparse_matrix_type make_csr_hamiltonian_block_( + full_det_iterator bra_begin, full_det_iterator bra_end, + full_det_iterator ket_begin, full_det_iterator ket_end, double H_thresh) { + using wfn_traits = wavefunction_traits; + using spin_wfn_type = typename wfn_traits::spin_wfn_type; + using spin_wfn_traits = wavefunction_traits; + const size_t nbra_dets = std::distance(bra_begin, bra_end); + const size_t nket_dets = std::distance(ket_begin, ket_end); + + std::vector bra_occ_alpha, bra_occ_beta; + + + // Get unique alpha strings + auto setup_st = std::chrono::high_resolution_clock::now(); + auto unique_alpha_bra = get_unique_alpha(bra_begin, bra_end); + auto unique_alpha_ket = get_unique_alpha(ket_begin, ket_end); + + const size_t nuniq_bra = unique_alpha_bra.size(); + const size_t nuniq_ket = unique_alpha_ket.size(); + + // Compute offsets + std::vector unique_alpha_bra_idx(nuniq_bra+1); + std::transform_exclusive_scan(unique_alpha_bra.begin(), + unique_alpha_bra.end(), + unique_alpha_bra_idx.begin(), + 0ul, std::plus{}, + [](auto& x){ return x.second; }); + std::vector unique_alpha_ket_idx(nuniq_ket+1); + std::transform_exclusive_scan(unique_alpha_ket.begin(), + unique_alpha_ket.end(), + unique_alpha_ket_idx.begin(), + 0ul, std::plus{}, + [](auto& x){ return x.second; }); + + unique_alpha_bra_idx.back() = nbra_dets; + unique_alpha_ket_idx.back() = nket_dets; + auto setup_en = std::chrono::high_resolution_clock::now(); + + std::cout << "AVERAGE NBETA = " << + std::accumulate(unique_alpha_bra.begin(), unique_alpha_bra.end(), + 0ul, [](auto a, auto b){ return a + b.second; }) / double(nuniq_bra) << std::endl; + + // Populate COO matrix locally + sparsexx::coo_matrix coo_mat(nbra_dets, nket_dets, 0, 0); + + size_t skip1 = 0; + size_t skip2 = 0; + + // Loop over uniq alphas in bra/ket + auto pop_st = std::chrono::high_resolution_clock::now(); + for(size_t ia_bra = 0; ia_bra < nuniq_bra; ++ia_bra) + if(unique_alpha_bra[ia_bra].first.any()) { + // Extract alpha bra + const auto bra_alpha = unique_alpha_bra[ia_bra].first; + const size_t beta_st_bra = unique_alpha_bra_idx[ia_bra]; + const size_t beta_en_bra = unique_alpha_bra_idx[ia_bra+1]; + spin_wfn_traits::state_to_occ(bra_alpha, bra_occ_alpha); + + for(size_t ia_ket = 0; ia_ket < nuniq_ket; ++ia_ket) + if(unique_alpha_ket[ia_ket].first.any()) { + // Extract alpha ket + const auto ket_alpha = unique_alpha_ket[ia_ket].first; + + // Compute alpha excitation + const auto ex_alpha = bra_alpha ^ ket_alpha; + const auto ex_alpha_count = spin_wfn_traits::count(ex_alpha); + + // Early exit + if( ex_alpha_count > 4) { + skip1++; + continue; + } + + // Precompute all-alpha excitation if it will be used + const double mat_el_4_alpha = (ex_alpha_count == 4) ? + this->matrix_element_4(bra_alpha, ket_alpha, ex_alpha) : 0.0; + if(ex_alpha_count == 4 and std::abs(mat_el_4_alpha) < H_thresh) { + // The only possible matrix element is too-small, skip everyhing + skip2++; + continue; + } + + const size_t beta_st_ket = unique_alpha_ket_idx[ia_ket]; + const size_t beta_en_ket = unique_alpha_ket_idx[ia_ket+1]; + + // Loop over local betas according to their global indices + for(size_t ibra = beta_st_bra; ibra < beta_en_bra; ++ibra) { + const auto bra_beta = wfn_traits::beta_string(*(bra_begin+ibra)); + spin_wfn_traits::state_to_occ(bra_beta, bra_occ_beta); + for(size_t iket = beta_st_ket; iket < beta_en_ket; ++iket) { + const auto ket_beta = wfn_traits::beta_string(*(ket_begin+iket)); + + // Compute beta excitation + const auto ex_beta = bra_beta ^ ket_beta; + const auto ex_beta_count = spin_wfn_traits::count(ex_beta); + + if((ex_alpha_count + ex_beta_count) > 4) continue; + + double h_el = 0.0; + if(ex_alpha_count == 4) { + // Use precomputed value + h_el = mat_el_4_alpha; + } else if(ex_beta_count == 4) { + h_el = this->matrix_element_4(bra_beta, ket_beta, ex_beta); + } else if(ex_alpha_count == 2) { + if(ex_beta_count == 2) { + h_el = this->matrix_element_22(bra_alpha, ket_alpha, ex_alpha, bra_beta, + ket_beta, ex_beta); + } else { + h_el = this->matrix_element_2(bra_alpha, ket_alpha, ex_alpha, + bra_occ_alpha, bra_occ_beta); + } + } else if(ex_beta_count == 2) { + h_el = this->matrix_element_2(bra_beta, ket_beta, ex_beta, + bra_occ_beta, bra_occ_alpha); + } else { + // Diagonal matrix element + h_el = this->matrix_element_diag(bra_occ_alpha, bra_occ_beta); + } + + // Insert matrix element + if(std::abs(h_el) > H_thresh) { + coo_mat.template insert(ibra, iket, h_el); + } + + } // ket beta + } // bra beta + + + } // Loop over ket alphas + } // Loop over bra alphas + auto pop_en = std::chrono::high_resolution_clock::now(); + + auto sort_st = std::chrono::high_resolution_clock::now(); + coo_mat.sort_by_row_index(); // Could be slow, but what else can we do?! + auto sort_en = std::chrono::high_resolution_clock::now(); + + auto conv_st = std::chrono::high_resolution_clock::now(); + sparse_matrix_type csr_mat(coo_mat); // Convert to CSR Matrix + auto conv_en = std::chrono::high_resolution_clock::now(); + + printf("Setup %.2e Pop %.2e Sort %.2e Conv %.2e S1 %lu S2 %lu\n", + std::chrono::duration(setup_en - setup_st).count(), + std::chrono::duration(pop_en - pop_st).count(), + std::chrono::duration(sort_en - sort_st).count(), + std::chrono::duration(conv_en - conv_st).count(),skip1,skip2); + + return csr_mat; + } + + sparse_matrix_type make_csr_hamiltonian_block_32bit_( + full_det_iterator bra_begin, full_det_iterator bra_end, + full_det_iterator ket_begin, full_det_iterator ket_end, + double H_thresh) override { + return make_csr_hamiltonian_block_(bra_begin, bra_end, ket_begin, + ket_end, H_thresh); + } + + sparse_matrix_type make_csr_hamiltonian_block_64bit_( + full_det_iterator bra_begin, full_det_iterator bra_end, + full_det_iterator ket_begin, full_det_iterator ket_end, + double H_thresh) override { + return make_csr_hamiltonian_block_(bra_begin, bra_end, ket_begin, + ket_end, H_thresh); + } + + public: + void form_rdms(full_det_iterator bra_begin, full_det_iterator bra_end, + full_det_iterator ket_begin, full_det_iterator ket_end, + double *C, matrix_span_t ordm, rank4_span_t trdm) override { + using wfn_traits = wavefunction_traits; + const size_t nbra_dets = std::distance(bra_begin, bra_end); + const size_t nket_dets = std::distance(ket_begin, ket_end); + + std::vector bra_occ_alpha, bra_occ_beta; + + // Loop over bra determinants + for(size_t i = 0; i < nbra_dets; ++i) { + const auto bra = *(bra_begin + i); + // if( (i%1000) == 0 ) std::cout << i << std::endl; + if(wfn_traits::count(bra)) { + // Separate out into alpha/beta components + spin_det_t bra_alpha = wfn_traits::alpha_string(bra); + spin_det_t bra_beta = wfn_traits::beta_string(bra); + + // Get occupied indices + bits_to_indices(bra_alpha, bra_occ_alpha); + bits_to_indices(bra_beta, bra_occ_beta); + + // Loop over ket determinants + for(size_t j = 0; j < nket_dets; ++j) { + const auto ket = *(ket_begin + j); + if(wfn_traits::count(ket)) { + spin_det_t ket_alpha = wfn_traits::alpha_string(ket); + spin_det_t ket_beta = wfn_traits::beta_string(ket); + + full_det_t ex_total = bra ^ ket; + if(wfn_traits::count(ex_total) <= 4) { + spin_det_t ex_alpha = wfn_traits::alpha_string(ex_total); + spin_det_t ex_beta = wfn_traits::beta_string(ex_total); + + const double val = C[i] * C[j]; + + // Compute Matrix Element + if(std::abs(val) > 1e-16) { + rdm_contributions(bra_alpha, ket_alpha, ex_alpha, bra_beta, + ket_beta, ex_beta, bra_occ_alpha, + bra_occ_beta, val, ordm, trdm); + } + } // Possible non-zero connection (Hamming distance) + + } // Non-zero ket determinant + } // Loop over ket determinants + + } // Non-zero bra determinant + } // Loop over bra determinants + } + + public: + template + SortedDoubleLoopHamiltonianGenerator(Args &&...args) + : HamiltonianGenerator(std::forward(args)...) {} +}; + +} // namespace macis diff --git a/include/macis/sd_operations.hpp b/include/macis/sd_operations.hpp index d88b02f0..f90f8ff3 100644 --- a/include/macis/sd_operations.hpp +++ b/include/macis/sd_operations.hpp @@ -369,6 +369,28 @@ inline auto doubles_sign(WfnType bra, WfnType ket, WfnType ex) { return sign; } + +template +auto get_unique_alpha(WfnIterator begin, WfnIterator end) { + using wfn_type = typename std::iterator_traits::value_type; + using wfn_traits = wavefunction_traits; + using spin_wfn_type = typename wfn_traits::spin_wfn_type; + + std::vector> unique_alpha; + unique_alpha.push_back({wfn_traits::alpha_string(*begin), 1}); + for(auto it = begin+1; it != end; ++it) { + auto& [cur_alpha, cur_count] = unique_alpha.back(); + auto alpha_i = wfn_traits::alpha_string(*it); + if(alpha_i == cur_alpha) { + cur_count++; + } else { + unique_alpha.push_back({alpha_i, 1}); + } + } + + return unique_alpha; +} + template std::string to_canonical_string(WfnType state) { using wfn_traits = wavefunction_traits; diff --git a/src/sparsexx/include/sparsexx/matrix_types/coo_matrix.hpp b/src/sparsexx/include/sparsexx/matrix_types/coo_matrix.hpp index 8e47b9ee..0d371a8c 100644 --- a/src/sparsexx/include/sparsexx/matrix_types/coo_matrix.hpp +++ b/src/sparsexx/include/sparsexx/matrix_types/coo_matrix.hpp @@ -212,6 +212,16 @@ class coo_matrix { void expand_from_triangle(); + template + inline void insert(index_type i, index_type j, value_type v) noexcept { + static_assert(not Check, "insert check NYI"); + rowind_.emplace_back(i); + colind_.emplace_back(j); + nzval_ .emplace_back(v); + nnz_++; + } + + #ifdef SPARSEXX_ENABLE_CEREAL template void serialize(Archive& ar) { diff --git a/src/sparsexx/tests/CMakeLists.txt b/src/sparsexx/tests/CMakeLists.txt index 52e12cdb..17ba4589 100644 --- a/src/sparsexx/tests/CMakeLists.txt +++ b/src/sparsexx/tests/CMakeLists.txt @@ -24,7 +24,7 @@ if( NOT Catch2_FOUND ) endif() -add_executable( sparsexx_test ut_main.cxx test_io.cxx test_util.cxx test_graph.cxx test_spmbv.cxx ) +add_executable( sparsexx_test ut_main.cxx test_types.cxx test_io.cxx test_util.cxx test_graph.cxx test_spmbv.cxx ) target_link_libraries( sparsexx_test PUBLIC sparsexx Catch2::Catch2 ) target_compile_definitions( sparsexx_test PUBLIC "SPARSEXX_DATA_DIR=\"${CMAKE_CURRENT_LIST_DIR}\"" diff --git a/src/sparsexx/tests/test_types.cxx b/src/sparsexx/tests/test_types.cxx new file mode 100644 index 00000000..97ee3463 --- /dev/null +++ b/src/sparsexx/tests/test_types.cxx @@ -0,0 +1,33 @@ +/* + * MACIS Copyright (c) 2023, The Regents of the University of California, + * through Lawrence Berkeley National Laboratory (subject to receipt of + * any required approvals from the U.S. Dept. of Energy). All rights reserved. + * + * See LICENSE.txt for details + */ + + +#include +#include + +#include "catch2/catch.hpp" + +TEST_CASE("COO Matrix", "[matrix_types]") { + using mat_type = sparsexx::coo_matrix; + + SECTION("Insert") { + size_t n = 6; + mat_type A(n,n,0,0); // empty matrix zero-indexing + for(int i = 0; i < n; ++i) { + A.insert(i,i, 2); + if(i < n-1) A.insert(i,i+1, 1); + if(i > 0) A.insert(i,i-1, 1); + } + A.sort_by_row_index(); // Put into canonical order + REQUIRE(A.nnz() == 16); + REQUIRE(A.rowind() == std::vector{0,0,1,1,1,2,2,2,3,3,3,4,4,4,5,5}); + REQUIRE(A.colind() == std::vector{0,1,0,1,2,1,2,3,2,3,4,3,4,5,4,5}); + REQUIRE(A.nzval() == std::vector {2,1,1,2,1,1,2,1,1,2,1,1,2,1,1,2}); + } + +} diff --git a/tests/csr_hamiltonian.cxx b/tests/csr_hamiltonian.cxx index ba4f2417..c6b7148a 100644 --- a/tests/csr_hamiltonian.cxx +++ b/tests/csr_hamiltonian.cxx @@ -11,11 +11,13 @@ #include #include #include +#include #include #include "ut_common.hpp" -TEST_CASE("CSR Hamiltonian") { +using wfn_type = macis::wfn_t<64>; +TEMPLATE_TEST_CASE("CSR Hamiltonian","[ham_gen]", macis::DoubleLoopHamiltonianGenerator, macis::SortedDoubleLoopHamiltonianGenerator ) { ROOT_ONLY(MPI_COMM_WORLD); size_t norb = macis::read_fcidump_norb(water_ccpvdz_fcidump); @@ -27,9 +29,8 @@ TEST_CASE("CSR Hamiltonian") { macis::read_fcidump_1body(water_ccpvdz_fcidump, T.data(), norb); macis::read_fcidump_2body(water_ccpvdz_fcidump, V.data(), norb); - using wfn_type = macis::wfn_t<64>; using wfn_traits = macis::wavefunction_traits; - using generator_type = macis::DoubleLoopHamiltonianGenerator; + using generator_type = TestType; #if 0 generator_type ham_gen(norb, V.data(), T.data()); @@ -42,10 +43,30 @@ TEST_CASE("CSR Hamiltonian") { // Generate configuration space const auto hf_det = wfn_traits::canonical_hf_determinant(nocc, nocc); auto dets = macis::generate_cisd_hilbert_space(norb, hf_det); + std::sort(dets.begin(), dets.end(), wfn_traits::spin_comparator{}); // Generate CSR Hamiltonian + auto st = std::chrono::high_resolution_clock::now(); auto H = macis::make_csr_hamiltonian_block( dets.begin(), dets.end(), dets.begin(), dets.end(), ham_gen, 1e-16); + auto en = std::chrono::high_resolution_clock::now(); + std::cout << std::chrono::duration(en - st).count() << std::endl; + +//#define GENERATE_TESTS +#ifdef GENERATE_TESTS + std::string tmp_rowptr_fname = "tmp_rowptr.bin"; + std::string tmp_colind_fname = "tmp_colind.bin"; + std::string tmp_nzval_fname = "tmp_nzval.bin"; + + std::ofstream rowptr_file(tmp_rowptr_fname, std::ios::binary); + rowptr_file.write((char*)H.rowptr().data(), H.rowptr().size() * sizeof(int32_t)); + std::ofstream colind_file(tmp_colind_fname, std::ios::binary); + colind_file.write((char*)H.colind().data(), H.colind().size() * sizeof(int32_t)); + std::ofstream nzval_file(tmp_nzval_fname, std::ios::binary); + nzval_file.write((char*)H.nzval().data(), H.nzval().size() * sizeof(double)); +#else + + //std::cout << "NEW H " << H.m() << " " 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